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The nonlinear processes of frequency conversion like second harmonic generation (SHG) usually obey certain selection rules, resulting from the preservation of different kind of physical quantities, e.g., the angular momentum. For SHG…

光学 · 物理学 2020-04-09 Florian Spreyer , Ruizhe Zhao , Lingling Huang , Thomas Zentgraf

Strong light-matter coupling within electromagnetic environments provides a promising path to modify and control chemical and physical processes. The origin of the enhancement of nonlinear optical processes such as second-harmonic and…

光学 · 物理学 2022-03-03 Davis M. Welakuh , Prineha Narang

Polaritons can provide strong optical field enhancement allowing to boost light-matter interaction. Here, we experimentally observe enhancement of mid-infrared second-harmonic generation (SHG) using grating-coupled surface phonon polaritons…

Boosting nonlinear frequency conversion in extremely confined volumes remains a key challenge in nano-optics, nanomedicine, photocatalysis, and background-free biosensing. To this aim, field enhancements in plasmonic nanostructures are…

Since the first observation of second harmonic generation (SHG), there have been extensive studies on this nonlinear phenomenon not only to clarify its physical origin but also to realize unconventional functionalities. Nonetheless, a…

Second harmonic generation (SHG), as one of the most significant \c{hi}(2) nonlinear optical processes, plays crucial roles in a broad variety of optical and photonic applications. Designing various delicate schemes to achieve highly…

光学 · 物理学 2021-09-01 Lei Wang , XiuQuan Zhang , Feng Chen

We theoretically study high-order harmonic generation (HHG) from solid-phase systems in spatially inhomogeneous strong laser fields originated by resonant plasmons within a metallic nanostructure. The intensity of the second plateau in HHG…

光学 · 物理学 2016-09-12 Tao-Yuan Du , Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

It is of fundamental importance but challenging to simultaneously identify atomic and magnetic configurations of two-dimensional van der Waals materials. In this work, we show that the nonreciprocal second-harmonic generation (SHG) can be a…

材料科学 · 物理学 2020-07-15 Wenshen Song , Ruixiang Fei , Li Yang

Second harmonic generation (SHG) is a nonlinear optical response arising exclusively from broken inversion symmetry in the electric-dipole limit. Recently, SHG has attracted widespread interest as a versatile and noninvasive tool for…

The efficient optical second-harmonic generation (SHG) of two-dimensional (2D) crystals, coupled with their atomic thickness that circumvents the phase-match problem, has garnered considerable attention. While various 2D heterostructures…

材料科学 · 物理学 2023-10-31 Wontaek Kim , Gyouil Jeong , Juseung Oh , Jihun Kim , Kenji Watanabe , Takashi Taniguchi , Sunmin Ryu

We theoretically investigate the second harmonic generation (SHG) of topological insulator surface states in a perpendicular magnetic field. Our theory is based on the microscopic expression of the second-order magneto-optical conductivity…

介观与纳米尺度物理 · 物理学 2024-11-27 Kainan Chang , Muhammad Zubair , Jin Luo Cheng , Wang-Kong Tse

We theoretically demonstrate x-ray second harmonic generation (SHG) with strong-field-driven high harmonic generation (HHG) from core electrons in gas-phase atoms, highlighting its potential as a powerful spectroscopic tool for studying…

原子物理 · 物理学 2025-03-31 Xinhua Xie

Nonlinear optics of semiconductors is an important field of fundamental and applied research, but surprisingly the role of excitons in the coherent processes leading to harmonics generation has remained essentially unexplored. Here we…

介观与纳米尺度物理 · 物理学 2015-06-17 M. Lafrentz , D. Brunne , A. V. Rodina , V. V. Pavlov , R. V. Pisarev , D. R. Yakovlev , A. Bakin , M. Bayer

In nonlinear nanophotonics, cascaded second-harmonic generation (SHG) in pure plasmonic waveguides for sequential signal transformation and complex on-chip functionality remains a long-standing challenge. Precise phase matching becomes…

光学 · 物理学 2025-08-22 Komal Gupta , Anand Hegde , Xiaofei Wu , Jer-Shing Huang , Chen-Bin Huang

Chip-scale nonlinear optics enables strong light-matter interactions within compact devices, serving as a fundamental platform for multifunctional integrated photonics from classical optical signal processing to quantum information…

We conduct a theoretical and numerical study on the second-harmonic (SH) optical response of a nano-structured metamaterial composed of a periodic array of inclusions. Both the inclusions and their surrounding matrix are made of…

介观与纳米尺度物理 · 物理学 2019-03-13 Ulises R. Meza , Bernardo S. Mendoza , W. Luis Mochán

We study surface second-harmonic generation (SHG) from a singular plasmonic structure consisting of touching metallic wires. We use the technique of transformation optics and relate the structure to a rather simpler geometry, a slab…

We show that the second harmonic generation (SHG) is enhanced in the chiral one-dimensional electron currents in a broad frequency range. The origin of the enhancement is two-fold: first, the linear dispersion of the current and the…

介观与纳米尺度物理 · 物理学 2020-04-17 Ivan Iorsh , Gulnaz Rakhmanova

We report second-harmonic generation (SHG) from thick hexagonal boron nitride (hBN) flakes with approximately 109-111 layers. The resulting effective second-order susceptibility is similar to previously reported few-layer experiments. This…

Exciton effects on conjugated polymers and the resulting optical nonlinearities are investigated in soliton lattice states. We use the Su-Schrieffer-Heeger model with long-range Coulomb interactions for electrons. The third-harmonic…

凝聚态物理 · 物理学 2008-02-03 Kikuo Harigaya