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The electronic ground state in many iridate materials is described by a complex wave-function in which spin and orbital angular momenta are entangled due to relativistic spin-orbit coupling (SOC). Such a localized electronic state carries…

Quantum spin liquids attract great interest due to their exceptional magnetic properties characterized by the absence of long-range order down to low temperatures despite the strong magnetic interaction. Commonly, these compounds are…

强关联电子 · 物理学 2018-05-01 Martin Dressel , Andrej Pustogow

Using quantum chemistry calculations we shed fresh light on the electronic structure and magnetic properties of RuCl3, a proposed realization of the honeycomb Kitaev spin model. It is found that the nearest-neighbor Kitaev exchange K is…

Muon spin rotation measurements have been performed on a powder sample of a-RuCl3, a layered material which previously has been proposed to be a quantum magnet on a honeycomb lattice close to a quantum spin liquid ground state. Our data…

强关联电子 · 物理学 2016-07-20 F. Lang , P. J. Baker , A. A. Haghighirad , Y. Li , D. Prabhakaran , R. Valenti , S. J. Blundell

The layered honeycomb magnet $\alpha$-Li$_2$IrO$_3$ has been theoretically proposed as a candidate to display novel magnetic behaviour associated with Kitaev interactions between spin-orbit entangled $j_{\rm eff}=1/2$ magnetic moments on a…

We show that the topological Kitaev spin liquid on the honeycomb lattice is extremely fragile against the second-neighbor Kitaev coupling $K_2$, which has recently been shown to be the dominant perturbation away from the nearest-neighbor…

强关联电子 · 物理学 2015-12-08 Ioannis Rousochatzakis , Johannes Reuther , Ronny Thomale , Stephan Rachel , N. B. Perkins

Recent experiment on a honeycomb-lattice Heisenberg antiferromagnet (AF) Bi$_3$Mn$_4$O$_{12}$(NO$_3$) revealed a novel spin-liquid-like behavior down to low temperature, which was ascribed to the frustration effect due to the competition…

强关联电子 · 物理学 2015-05-18 Soichiro Okumura , Hikaru Kawamura , Tsuyoshi Okubo , Yukitoshi Motome

The honeycomb-lattice cobaltate Na$_3$Co$_2$SbO$_6$ has recently been proposed to be a proximate Kitaev quantum spin liquid~(QSL) candidate. However, non-Kitaev terms in the Hamiltonian lead to a zigzag-type antiferromagnetic~(AFM) order at…

YbOCl is a representative member of the van der Waals layered honeycomb rare-earth chalcohalide REChX (RE = rare earth, Ch = O, S, Se, and Te, and X = F, Cl, Br, and I) family reported recently. Its spin ground state remains to be explored…

By including a material-relevant off-diagonal interaction called the $\Gamma$ term into the Kitaev model and introducing spatial anisotropy in the interaction strength on the honeycomb lattice, we obtain a series of nodal Z$_2$ quantum spin…

强关联电子 · 物理学 2020-09-15 Jiucai Wang , Zheng-Xin Liu

With large spin-orbit coupling, the $t_{2g}^5$ electron configuration in $d$-metal oxides is prone to highly anisotropic exchange interactions and exotic magnetic properties. In $5d^5$ iridates, given the existing variety of crystal…

Nearest-neighbor interacting S = 1/2 spins on the ideal Kagom\'{e} lattice are predicted to form a variety of novel quantum entangled states, including quantum spin-liquid (SL) and valence bond solid (VBS) phases. In real materials, the…

Motivated by the recent theoretical study by Okubo $et \ al$ [Phys. Rev. Lett. ${\bf 108}$, 017206 (2012)] on the possible realization of the frustration-induced $ symmetric$ skyrmion-lattice state in the $J_1$-$J_2$ (or $J_1$-$J_3$)…

强关联电子 · 物理学 2019-12-05 Tokuro Shimokawa , Tsuyoshi Okubo , Hikaru Kawamura

The 5d-electron honeycomb compound H$_3$LiIr$_2$O$_3$ [K. Kitagawa $et$ $al.$, Nature 554, 341-345 (2018)] exhibits an apparent quantum spin liquid (QSL) state. In this intercalated spin-orbital compound, a remarkable pile up of low-energy…

强关联电子 · 物理学 2019-02-07 Johannes Knolle , Roderich Moessner , Natalia B. Perkins

Cobaltates with 3$d$ based layered honeycomb structure were recently proposed as Kitaev magnets and putative candidates to host the long-sought Kitaev spin liquid. Here we present inelastic neutron scattering results down to 50 mK for…

强关联电子 · 物理学 2023-01-18 Alaric L. Sanders , Richard A. Mole , Jiatu Liu , Alex J. Brown , Dehong Yu , Chris D. Ling , Stephan Rachel

Material realizations of the bond-dependent Kitaev interactions with $S$=1/2 local moments have vitalized the research in quantum spin liquids. Recently, it has been proposed that higher-spin analogues of the Kitaev interactions may also…

强关联电子 · 物理学 2021-02-24 Ilia Khait , P. Peter Stavropoulos , Hae-Young Kee , Yong Baek Kim

In the quest to find quantum spin liquids, layered cobalt oxides Na2Co2TeO6 and Na3Co2SbO6 have been proposed as promising candidates for approximating the Kitaev honeycomb model. Yet, their suitability has been thrown into question due to…

We report the magnetic properties of the double perovskites SrLaCuSbO$_6$ (SLCSO) and SrLaCuNbO$_6$ (SLCNO). The temperature dependence of the magnetic susceptibilities of both compounds shows a broad maximum characteristic of an…

Using modified spin wave (MSW) method, we study the $J_1-J_2$ Heisenberg model with first and second neighbor antiferromagnetic exchange interactions. For symmetric $S=1/2$ model, with the same couplings for all the equivalent neighbors, we…

强关联电子 · 物理学 2016-08-24 Elaheh Ghorbani , Farhad Shahbazi , Hamid Mosadeq

The Kitaev honeycomb model plays a pivotal role in the quest for quantum spin liquids, in which fractional quasiparticles would provide applications in decoherence-free topological quantum computing. The key ingredient is the bond-dependent…

强关联电子 · 物理学 2024-10-11 Seong-Hoon Jang , Yukitoshi Motome