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Quantum spin liquids are materials that feature quantum entangled spin correlations and avoid magnetic long-range order at T = 0 K. Particularly interesting are two-dimensional honeycomb spin lattices where a plethora of exotic quantum spin…

强关联电子 · 物理学 2020-11-20 C. Wessler , B. Roessli , K. W. Krämer , B. Delley , O. Waldmann , L. Keller , D. Cheptiakov , H. B. Braun , M. Kenzelmann

Despite the exciting implications of the Kitaev spin-Hamiltonian, finding and confirming the quantum spin liquid state has proven incredibly difficult. Recently the applicability of the model has been expanded through the development of a…

In addition to the Kitaev ($K$) interaction, candidate Kitaev materials also possess Heisenberg ($J$) and off-diagonal symmetric ($\Gamma$) couplings. We investigate the quantum ($S = 1/2$) $K$-$J$-$\Gamma$ model on the honeycomb lattice by…

强关联电子 · 物理学 2019-11-14 Jiucai Wang , B. Normand , Zheng-Xin Liu

The physics of spin-orbit entangled magnetic moments of $4d$ and $5d$ transition metal ions on a honeycomb lattice has been much explored in search for unconventional magnetic orders or quantum spin liquids expected for compass spin models,…

Motivated by the rich physics of honeycomb magnetic materials, we obtain the phase diagram and analyze magnetic properties of the spin-1/2 and spin-1 J1-J2-J3 Heisenberg model on the honeycomb lattice. Based on the SU(2) and SU(3) symmetry…

强关联电子 · 物理学 2018-05-16 J. Merino , A. Ralko

Motivated by the recently synthesized insulating nickelate Ni$_2$Mo$_3$O$_8$, which has been reported to have an unusual non-collinear magnetic order of Ni$^{2+}$ $S=1$ moments with a nontrivial angle between adjacent spins, we construct an…

强关联电子 · 物理学 2021-08-17 Shuyi Li , Manh Duc Le , Vaideesh Loganathan , Andriy H. Nevidomskyy

Na$_2$IrO$_3$, a honeycomb 5$d^5$ oxide, has been recently identified as a potential realization of the Kitaev spin lattice. The basic feature of this spin model is that for each of the three metal-metal links emerging out of a metal site,…

Anderson proposed structural topology in frustrated magnets hosting novel quantum spin liquids (QSLs). The QSL state is indeed exactly derived by fractionalizing the spin excitation into spinless Majorana fermions in a perfect two…

We have combined single crystal neutron and x-ray diffractions to investigate the magnetic and crystal structures of the honeycomb lattice $\rm Na_2IrO_3$. The system orders magnetically below $18.1(2)$ K with Ir$^{4+}$ ions forming zigzag…

Recently it was realized that the zigzag magnetic order in Kitaev materials can be stabilized by small negative off-diagonal interactions called the $\Gamma'$ terms. To fully understand the effect of the $\Gamma'$ interactions, we…

强关联电子 · 物理学 2020-10-21 Jiucai Wang , Qirong Zhao , Xiaoqun Wang , Zheng-Xin Liu

The nature of the effective spin Hamiltonian and magnetic order in the honeycomb iridates is explored by considering a trigonal crystal field effect and spin-orbit coupling. Starting from a Hubbard model, an effective spin Hamiltonian is…

强关联电子 · 物理学 2012-07-10 Subhro Bhattacharjee , Sung-Sik Lee , Yong Baek Kim

Most of the searches for Kitaev materials deal with $4d/5d$ magnets with spin-orbit-coupled ${J=1/2}$ local moments such as iridates and $\alpha$-RuCl$_3$. Here we propose the monoclinic YbCl$_3$ with a Yb$^{3+}$ honeycomb lattice for the…

We investigate the ground-state and finite-temperature properties of the bond-random $s=1/2$ Heisenberg model on a honeycomb lattice with frustrated nearest- and next-nearest-neighbor antiferromagnetic interactions, $J_1$ and $J_2$, by the…

强关联电子 · 物理学 2018-10-24 Kazuki Uematsu , Hikaru Kawamura

Rare-earth (RE) based honeycomb-lattice materials with strong spin-orbit coupled Jeff=1/2 moments have attracted great interest as a platform to realize Kitaev quantum spin liquid (QSL) state. Herein, we report the discovery of a new family…

Quantum magnets based on honeycomb lattices with low-coordination number offer a viable ground to realize exotic emergent quantum excitations and phenomena arising from the interplay between competing magnetic interactions, spin…

强关联电子 · 物理学 2024-11-14 J. Khatua , M. Gomilsek , Kwang-Yong Choi , P. Khuntia

Two-dimensional honeycomb lattices, characterized by their low coordination numbers, provide a fertile platform for exploring various quantum phenomena due to the intricate interplay between competing magnetic interactions, spin-orbit…

One main theme in current condensed matter physics is the search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature without static order. However, there is no…

强关联电子 · 物理学 2023-01-10 Chengpeng Tu , Dongzhe Dai , Xu Zhang , Chengcheng Zhao , Xiaobo Jin , Bin Gao , Tong Chen , Pengcheng Dai , Shiyan Li

We report on band structure calculations and a microscopic model of the low-dimensional magnet beta-Cu2V2O7. Magnetic properties of this compound can be described by a spin-1/2 anisotropic honeycomb lattice model with the averaged coupling…

强关联电子 · 物理学 2010-10-12 Alexander A. Tsirlin , Oleg Janson , Helge Rosner

Layered honeycomb magnets are of interest as potential realizations of the Kitaev quantum spin liquid (KQSL), a quantum state with long-range spin entanglement and an exactly solvable Hamiltonian. Conventional magnetically ordered states…

强关联电子 · 物理学 2020-01-28 Ruidan Zhong , Tong Gao , Nai Phuan Ong , Robert J. Cava

Contrasting ground states of quantum magnets with the integer and half-integer spin moments are the manifestation of many-body quantum interference effects. In this work, we investigate the distinct nature of the integer and half-integer…

强关联电子 · 物理学 2021-07-21 Hyun-Yong Lee , Takafumi Suzuki , Yong Baek Kim , Naoki Kawashima
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