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Simulating large-scale coupled-oscillator systems presents substantial computational challenges for classical algorithms, particularly when pursuing first-principles analyses in the thermodynamic limit. Motivated by the quantum algorithm…

While it seems possible that quantum computers may allow for algorithms offering a computational speed-up over classical algorithms for some problems, the issue is poorly understood. We explore this computational speed-up by investigating…

量子物理 · 物理学 2010-06-09 Alastair A. Abbott , Cristian S. Calude

Quantum adiabatic optimization seeks to solve combinatorial problems using quantum dynamics, requiring the Hamiltonian of the system to align with the problem of interest. However, these Hamiltonians are often incompatible with the native…

The implementation of the orbital minimization method (OMM) for solving the self-consistent Kohn-Sham (KS) problem for electronic structure calculations in a basis of non-orthogonal numerical atomic orbitals of finite-range is reported. We…

计算物理 · 物理学 2014-02-06 Fabiano Corsetti

We show how to apply the quantum adiabatic algorithm directly to the quantum computation of molecular properties. We describe a procedure to map electronic structure Hamiltonians to 2-local qubit Hamiltonians with a small set of physically…

量子物理 · 物理学 2015-02-20 Ryan Babbush , Peter J. Love , Alán Aspuru-Guzik

For noisy intermediate-scale quantum (NISQ) devices only a moderate number of qubits with a limited coherence is available thus enabling only shallow circuits and a few time evolution steps in the currently performed quantum computations.…

量子物理 · 物理学 2021-02-04 Diksha Dhawan , Mekena Metcalf , Dominika Zgid

We propose an iterative algorithm to simulate the dynamics generated by any $n$-qubit Hamiltonian. The simulation entails decomposing the unitary time evolution operator $U$ (unitary) into a product of different time-step unitaries. The…

量子物理 · 物理学 2012-04-09 Ashok Ajoy , Rama Koteswara Rao , Anil Kumar , Pranaw Rungta

In electronic structure theory, variational methods offer a valuable paradigm for approximating electronic ground states. However, for historical reasons, this principle is mostly restricted to model chemistries in pre-defined fixed basis…

量子物理 · 物理学 2025-11-17 Fabian Langkabel , Stefan Knecht , Jakob S. Kottmann

Achieving an accurate description of fermionic systems typically requires considerably many more orbitals than fermions. Previous resource analyses of quantum chemistry simulation often failed to exploit this low fermionic number…

量子物理 · 物理学 2022-05-24 Sam McArdle , Earl Campbell , Yuan Su

Quantum algorithms offer significant speedups over their classical counterparts for a variety of problems. The strongest arguments for this advantage are borne by algorithms for quantum search, quantum phase estimation, and Hamiltonian…

量子物理 · 物理学 2021-12-14 John M. Martyn , Zane M. Rossi , Andrew K. Tan , Isaac L. Chuang

Quantum Hamiltonian identification is important for characterizing the dynamics of quantum systems, calibrating quantum devices and achieving precise quantum control. In this paper, an effective two-step optimization (TSO) quantum…

量子物理 · 物理学 2018-06-05 Yuanlong Wang , Daoyi Dong , Bo Qi , Jun Zhang , Ian R. Petersen , Hidehiro Yonezawa

Quantum computing is a promising technology that harnesses the peculiarities of quantum mechanics to deliver computational speedups for some problems that are intractable to solve on a classical computer. Current generation noisy…

Many of the envisioned use-cases for quantum computers involve optimisation processes. While there are many algorithmic primitives to perform the required calculations, all eventually lead to quantum gates operating on quantum bits, with an…

量子物理 · 物理学 2026-03-26 Lukas Schmidbauer , Elisabeth Lobe , Ina Schaefer , Wolfgang Mauerer

The computation of electronic structure properties at the quantum level is a crucial aspect of modern physics research. However, conventional methods can be computationally demanding for larger, more complex systems. To address this issue,…

量子物理 · 物理学 2023-12-05 Nouhaila Innan , Muhammad Al-Zafar Khan , Mohamed Bennai

Optimization of circuits is an essential task for both quantum and classical computers to improve their efficiency. In contrast, classical logic optimization is known to be difficult, and a lot of heuristic approaches have been developed so…

量子物理 · 物理学 2025-05-14 Yusei Mori , Hideaki Hakoshima , Kyohei Sudo , Toshio Mori , Kosuke Mitarai , Keisuke Fujii

Accurate quantum chemistry simulations remain challenging on classical computers for problems of industrially relevant sizes and there is reason for hope that quantum computing may help push the boundaries of what is technically feasible.…

量子物理 · 物理学 2021-03-17 Vincent E. Elfving , Marta Millaruelo , José A. Gámez , Christian Gogolin

Quantum computation appears to offer significant advantages over classical computation and this has generated a tremendous interest in the field. In this thesis we consider the application of quantum computers to scientific computing and…

量子物理 · 物理学 2018-05-10 Stuart Hadfield

The numerical version of the Hamilton-Jacobi quantization method, recently proposed, is applied to the one dimensional quartic oscillator. A suitable quantization condition is formulated and various energy levels and wave functions are…

量子物理 · 物理学 2017-11-28 Mario Fusco Girard

In computer simulations, quantum delocalization of atomic nuclei can be modeled making use of the Path Integral (PI) formulation of quantum statistical mechanics. This approach, however, comes with a large computational cost. By restricting…

统计力学 · 物理学 2015-04-13 Karsten Kreis , Mark E. Tuckerman , Davide Donadio , Kurt Kremer , Raffaello Potestio

Achieving reliable performance on early fault-tolerant quantum hardware will depend on protocols that manage noise without incurring prohibitive overhead. We propose a novel framework that integrates quantum computation with the…

量子物理 · 物理学 2026-03-10 IlKwon Sohn , Changyeol Lee , Wooyeong Song , Kwangil Bae , Wonhyuk Lee