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Strong electric fields can be used to align molecules. However, a non-polar molecule such as H$_2$ has no preference for its orientation. There are thus two equivalent configurations with equal energy separated by a potential-energy…

化学物理 · 物理学 2025-12-02 J. Amira Geuther , Marit R. Fiechter , Jeremy O. Richardson

We study strong-field molecular ionization as a function of pulse duration. Experimental measurements of the photoelectron yield for a number of molecules reveal competition between different ionization continua (cationic states) which…

We study ionization of atoms in strong elliptically-polarized laser fields numerically and analytically. We focus on effects of laser ellipticity on the offset angle in photoelectron momentum distribution. This angle is considered to encode…

原子物理 · 物理学 2023-04-26 J. Y. Che , J. Y. Huang , F. B. Zhang , C. Chen , G. G. Xin , Y. J. Chen

Quantum emitters in solid-state crystals have recently attracted a lot of attention due to their simple applicability in optical quantum technologies. The polarization of single photons generated by quantum emitters is one of the key…

Multiphoton ionization of sodium by laser pulses of 800 nm wavelength and 57 fs duration is studied in the range of laser peak intensities belonging to over-the-barrier ionization regime. Photoelectron momentum distributions (PMD) and the…

原子物理 · 物理学 2019-03-21 Andrej Bunac , Duška B. Popović , Nenad S. Simonović

To measure and control the electron motion in atoms and molecules by the strong laser field on the attosecond time scale is one of the research frontiers of atomic and molecular photophysics. It involves many new phenomena and processes and…

原子物理 · 物理学 2022-03-30 Chao Chen , Jiayin Che , Shang Wang , Guoguo Xin , Yanjun Chen

Previous attoclock experiments measuring the photoelectron momentum distribution (PMD) via strong-field ionization in an elliptically polarized laser field have shown anomalously large offset angles in the nonadiabatic regime with large…

原子物理 · 物理学 2025-01-22 Q. Z. Lv , M. Klaiber , P. -L. He , K. Z. Hatsagortsyan , C. H. Keitel

Using a model methane-like chiral system, we theoretically demonstrate a possibility to access photoelectron circular dichroism (PECD) by a single experiment with two overlapping laser pulses of carrier frequencies $\omega$ and $2\omega$,…

原子与分子团簇 · 物理学 2018-12-20 Philipp V. Demekhin , Anton N. Artemyev , Alexander Kastner , Thomas Baumert

We consider the final stage of double ionization of $\rm O_2$ molecules by short linearly polarized laser pulses. The saddles of the effective adiabatic potential energy close to which simultaneous escape of electrons from a molecule takes…

原子物理 · 物理学 2007-05-23 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt

We propose a very sensitive method for measuring the electric dipole moment of the electron using polar molecules embedded in a cryogenic solid matrix of inert-gas atoms. The polar molecules can be oriented in the $\hat{\rm{z}}$ direction…

原子物理 · 物理学 2018-01-29 A. C. Vutha , M. Horbatsch , E. A. Hessels

Recent advances in strong x-ray laser techniques enable the study of nonlinear multiphoton ionization in extreme high-frequency fields. Although the stabilization regime in such fields is theoretically established, its modified properties…

原子物理 · 物理学 2026-02-17 Aleksandr V. Boitsov , Karen Z. Hatsagortsyan , Christoph H. Keitel

We discuss the final stages of double ionization of atoms in a strong linearly polarized laser field within a classical model. We propose that all trajectories leading to non-sequential double ionization pass close to a saddle in phase…

原子物理 · 物理学 2009-11-06 Krzysztof Sacha , Bruno Eckhardt

Double ionization of diatomic molecules by short linearly polarized laser pulses is analyzed. We consider the final stage of the ionization process, that is the decay of a highly excited two electron molecule, which is formed after…

原子物理 · 物理学 2016-09-08 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt , Jakub Zakrzewski

D$_2$ molecules, excited by linearly cross-polarized femtosecond extreme ultraviolet (XUV) and near-infrared (NIR) light pulses, reveal highly structured D$^+$ ion fragment momenta and angular distributions that originate from two different…

Ferroelectric materials with switchable spontaneous polarization underpin non-volatile memories, transistors, sensors, and emerging neuromorphic chips. Their performance and stability are governed by polarization dynamics and domain…

材料科学 · 物理学 2026-03-20 Dongyu Bai , Ri He , Junxian Liu , Liangzhi Kou

The dynamics of electric field generation and radial acceleration of ions by a laser pulse of relativistic intensity propagating in an underdense plasma has been investigated using an one-dimensional electrostatic, ponderomotive model…

等离子体物理 · 物理学 2008-07-30 A. Macchi , F. Ceccherini , F. Cornolti , S. Kar , M. Borghesi

Recent theoretical investigations have indicated that rapid optical cycling should be feasible in complex polyatomic molecules with diverse constituents, geometries and symmetries. However, as a composite molecular mass grows, so does the…

原子物理 · 物理学 2020-12-18 Konrad Wenz , Ivan Kozyryev , Rees L. McNally , Leland Aldridge , Tanya Zelevinsky

Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an…

化学物理 · 物理学 2016-07-27 Markus Kowalewski , Kochise Bennett , Jérémy R. Rouxel , Shaul Mukamel

In a spherically symmetric plasma constrained by its own gravity, the ionization degree lags behind changes in temperature and density. The ambipolar electric field accelerates ions radially and cools electrons. Ions lose energy and angular…

星系天体物理 · 物理学 2024-08-13 Haibin Chen , Rong Wu

Dynamic stabilization of atomic hydrogen against ionization in high-frequency single- and two-color, circularly polarized laser pulses is observed by numerically solving the three-dimensional, time-dependent Schr\"odinger equation. The…

原子物理 · 物理学 2009-11-07 D. Bauer , F. Ceccherini