相关论文: Laboratory-based sticking coefficients for ices on…
In laboratory experiments, we study the motion of levitated, sedimenting clouds of sub-mm grains at low ambient pressure and at high solid-to-gas ratios $\epsilon$. The experiments show a collective behavior of particles, i.e. grains in…
The typical amount of molecular hydrogen (${\rm H_2}$) in interstellar ices is not known, but significant freeze-out of ${\rm H_2}$ on dust grains is not expected. However, chemical models ubiquitously predict large amounts of $\rm H_2$…
Gas-grain and gas-phase reactions dominate the formation of molecules in the interstellar medium (ISM). Gas-grain reactions require a substrate (e.g. a dust or ice grain) on which the reaction is able to occur. The formation of molecular…
Ice is ubiquitous in the interstellar medium. We model the formation of the main constituents of interstellar ices, including H2O, CO2 , CO, and CH3 OH. We strive to understand what physical or chemical parameters influence the final…
Physical conditions in dense and cold regions of interstellar clouds favour the formation of ice mantles on the surfaces of interstellar grains. It is predicted that most of the gaseous species heavier than H2 or He will adsorb onto the…
Currently ~36 different absorption bands have been detected in the infrared spectra of cold, dense interstellar and circumstellar environments. These are attributed to the vibrational transitions of ~17 different molecules frozen on dust…
Ice desorption affects the evolution of the gas-phase chemistry during the protostellar stage, and also determines the chemical composition of comets forming in circumstellar disks. From observations, most volatile species are found in…
In protoplanetary disks, CO$_2$ is solid ice beyond its snow line at $\sim 10 \rm AU$. Due to its high abundance, it contributes heavily to the collisional evolution in this region of the disk. For the first time, we carried out laboratory…
We develop a model of dust evolution in a multiphase, inhomogeneous ISM including dust growth and destruction processes. The physical conditions for grain evolution are taken from hydrodynamical simulations of giant molecular clouds in a…
In order to interpret observations influenced by dust and to perform detailed modeling of the observable characteristics of dust-producing or dust-containing objects, knowledge of the micro-physical properties of relevant dust species are…
Accurate modeling of physical and chemical processes in the interstellar medium requires detailed knowledge of how atoms and molecule adsorb on dust grains. However, the sticking coefficient, a number between 0 and 1 that measures the first…
We argue that impact velocities between dust grains with sizes less than $\sim 0.1$ $\mu m$ in molecular cloud cores are dominated by drift arising from ambipolar diffusion. This effect is due to the size dependence of the dust coupling to…
Processing by interstellar photons affects the composition of the icy mantles on interstellar grains. The rate of photodissociation in solids differs from that of molecules in the gas phase. The aim of this work was to determine an average,…
Transitional discs have central regions characterised by significant depletion of both dust and gas compared to younger, optically-thick discs. However, gas and dust are not depleted by equal amounts: gas surface densities are typically…
We present Temperature Programmed Desorption (TPD) experiments of CO and N2 ices in pure, layered and mixed morphologies at various ice "thicknesses" and abundance ratios as well as simultaneously taken Reflection Absorption Infrared…
Protoplanetary disks are the target of many chemical studies (both observational and theoretical) as they contain the building material for planets. Their large vertical and radial gradients in density and temperature make them challenging…
The formation of molecular hydrogen in the interstellar medium takes place on the surfaces of dust grains. Hydrogen molecules play a role in gas-phase reactions that produce other molecules, some of which serve as coolants during…
In this work we investigate the effects of ion accretion and size-dependent dust temperatures on the abundances of both gas-phase and grain-surface species. While past work has assumed a constant areal density for icy species, we show that…
It has been implicitly assumed that ices on grains in molecular clouds and proto planetary disks are formed by homogeneous layers regardless of their composition or crystallinity. To verify this assumption, we observed the H2O deposition…
Atoms and molecules, and in particular CO, are important coolants during the evolution of interstellar star-forming gas clouds. The presence of dust grains, which allow many chemical reactions to occur on their surfaces, strongly impacts…