相关论文: $T$-matrix method for calculation of second-harmon…
We present high resolution two-photon excitation microscopy studies combining two-photon fluorescence (TPF) and second harmonic generation (SHG) in order to probe orientational distributions of molecular ensembles at room temperature. A…
LMTO calculations are presented for the frequency dependent second harmonic generation (SHG) in the polytypes 2H, 4H, 6H, 15R and 3C of SiC. All independent tensor components are calculated. The spectral features and the ratios of the 333…
The polarization matrix ($2\times2$) obtained from two component eigen-spinors of spherical harmonics help us to evaluate the differential matrix $N$ of the anisotropic optical medium. The geometric phase is realized through {\it helicity}…
We theoretically predict efficient optical second-harmonic generation (SHG) from a few hundred nanometer thick slab consisting of a quadratic nonlinear anisotropic medium whose linear principal permittivities are, at the fundamental…
Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…
Using classical electrodynamics we determine the higher harmonic radiation by a nonspherical metal cluster in form of a matrix formalism. Extending the theory for the source of the higher harmonic radiation for spherical metal clusters as…
The second harmonic generation is one of the most important applications of nonlinear effect, which has attracted great interests in nonlinear optics and microwave in the past decades. To the best of our knowledge, however, generating the…
We demonstrate the interest of combining Finite Element calculations with the Vector Partial Wave formulation (used in T-matrix and Mie theory) in order to characterize the electromagnetic scattering properties of isolated individual…
We employ transformation optics to optimize the generic nonlinear wave interaction of second-harmonic generation from a pair of touching metallic wires. We demonstrate a 10 orders of magnitude increase in the second-harmonic scattering…
We introduce a new mechanism for second-harmonic generation through geometrically rectifying-funneling-ballistic electrons in THz optical resonators. Our resonant rectifiers inherently act as second-order harmonic generators, rectifying…
We present in this paper a spectrally accurate numerical method for computing the spherical/vector spherical harmonic expansion of a function/vector field with given (elemental) nodal values on a spherical surface. Built upon suitable…
We studied the high-order harmonic generation (HHG) from 2D solid materials in circularly and bichromatic circularly polarized laser fields numerically by simulating the dynamics of single-active-electron processes in 2D periodic…
We theoretically study high-order harmonic generation (HHG) from solid-phase systems in spatially inhomogeneous strong laser fields originated by resonant plasmons within a metallic nanostructure. The intensity of the second plateau in HHG…
We observe the generation of high harmonics in the plane perpendicular to the driving laser polarization and show that these are driven by the spin-orbit interaction. Using R-Matrix with time-dependence theory, we demonstrate that for…
Plasmonic nanostructures that support surface plasmon (SP) resonance potentially provide a route for the development of nanoengineered nonlinear optical devices. In this work, second-order nonlinear light scattering, specifically…
The multiple scattering method T-matrix (MSTMM) can be used to solve the electromagnetic response of systems consisting of many compact scatterers, retaining a good level of accuracy while using relatively few degrees of freedom, largely…
Spatial and spectral properties of the pulsed second harmonic generation in a periodically-poled KTP waveguide exploiting simultaneously the first, second, and third harmonics of periodic nonlinear modulation are analyzed. Experimental…
The $T$-matrix formally describes the solution of any electromagnetic scattering problem by a given particle in a given medium at a given wavelength. As such it is commonly used in a number of contexts, for example to predict the…
Second harmonic generation is enhanced at the surface lattice resonance in plasmonic nanoparticle arrays. We carried out a parametric investigation on two-dimensional lattices composed of gold nanobars where the centrosymmetry is broken at…
Highly nonlinear optical phenomena can provide access to properties of electronic systems which are otherwise difficult to access through conventional linear optical spectroscopies. In particular, high harmonic generation (HHG) in…