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The role of dipolar interactions and anisotropy are important to obtain, otherwise forbidden, ferromagnetic ordering at finite temperature for ions arranged in two-dimensional (2D) arrays (monolayers). Here we demonstrate that conventional…

介观与纳米尺度物理 · 物理学 2007-05-23 M. K. Mukhopadhyay , M. K. Sanyal , T. Sakakibara , V. Leiner , R. M. Dalgliesh , S. Langridge

Hole doping in Nd${}_{2}$NiO${}_{4.00}$ can be either achieved by substituting the trivalent Nd atoms by bivalent alkaline earth metals or by oxygen doping, yielding Nd${}_{2}$NiO${}_{4+\delta}$. In this study, we investigated the interplay…

The commensurate and incommensurate magnetic structures of the magnetoelectric system YMn$_{2}$O$_{5}$, as determined from neutron diffraction, were found to be spin-density waves lacking a global center of symmetry. We propose a model,…

材料科学 · 物理学 2009-11-11 L. C. Chapon , P. G. Radaelli , G. R. Blake , S. Park , S-W. Cheong

Magnetism in 2D networks of the acetylene-bridged transition metal porphyrins M(P)-2(C-C)-2 (denoted P-TM), and oxo-TM-porphyrins OM(P)-2(C-C)-2 (denoted P-TMO), is studied with the density functional theory (DFT) and the self-interaction…

材料科学 · 物理学 2015-10-26 Malgorzata Wierzbowska , Andrzej L. Sobolewski

Multi-orbital physics in quasi-two-dimensional electron gases (q2DEGs) triggers unique phenomena not observed in bulk materials, such as unconventional superconductivity and magnetism. Here, we investigate the mechanism of orbital selective…

The low-temperature electronic and magnetic properties of NH$_4$V$_2$O$_5$, an isoelectronic analog of the spin-ladder compound $\alpha'$-NaV$_2$O$_5$, are investigated using DFT+$U$ calculations. Two charge-ordering patterns - zigzag and…

强关联电子 · 物理学 2025-08-20 Dm. M. Korotin

Magnetization, magnetocaloric, calorimetric, neutron and X-ray diffraction and inelastic neutron scattering measurements are performed on single crystals of BaCdVO(PO$_4$)$_2$. The low-temperature crystal structure is found to be of a lower…

Neutron diffraction, magnetization and muon spin relaxation measurements, supplemented by density functional theory (DFT) calculations are employed to unravel temperature-driven magnetization reversal (MR) in inverse spinel Co$_2$VO$_4$.…

Magnetic order typically emerges due to the short-range exchange interaction between the constituent electronic spins. Recent discoveries have found a crucial role for spin-phonon coupling in various phenomena from optical ultrafast…

介观与纳米尺度物理 · 物理学 2024-05-16 Petros Andreas Pantazopoulos , Johannes Feist , Francisco J. García-Vidal , Akashdeep Kamra

In order to establish the correlation between the magnetoelectric coupling and magnetic instability, we have studied the structural, magnetic, and ferroelectric properties of \textit{x}BaTiO${_3}$-(1-\textit{x})BiCoO${_3}$ as a function of…

材料科学 · 物理学 2019-02-14 Lokanath Patra , Zhao Pan , Jun Chen , Masaki Azuma , P. Ravindran

Recent works suggest that the surface chemistry, in particular, the presence of oxygen vacancies can affect the polarization in a ferroelectric material. This should, in turn, influence the domain ordering driven by the need to screen the…

Novel magnetic phases are expected to occur in highly frustrated spin systems. Here we study the structurally perfect kagom\'e antiferromagnet CdCu$_3$(OH)$_6$(NO$_3$)$_2\cdot$H$_2$O by magnetization, magnetic torque, and heat capacity…

强关联电子 · 物理学 2017-03-29 Ryutaro Okuma , Takeshi Yajima , Daisuke Nishio-Hamane , Tsuyoshi Okubo , Zenji Hiroi

Organometallic clusters based on transition metal atoms are interesting because possible applications in spintronics and quantum information. In addition to the enhanced magnetism at the nanoscale, the organic ligands may provide a natural…

化学物理 · 物理学 2017-06-12 J. W. González , T. Alonso-Lanza , F. Delgado , F. Aguilera-Granja , A. Ayuela

In this letter, we report the structural, electronic and ferroelectric properties of the layered mixed-valent transition-metal compound, Sr$_{4}$Fe$_{6}$O$_{12}$ (SFO). We demonstrate how SFO undergoes a phase transition from a…

强关联电子 · 物理学 2025-02-05 Arindam Sarkar , Hena Das , Prashant Singh , Aftab Alam

The development of short- and long-range magnetic order induced in a frustrated zig-zag ladder compound SrDy2O4 by an applied field is studied using neutron diffraction techniques. In zero field, SrDy2O4 lacks long-range magnetic order down…

强关联电子 · 物理学 2017-04-25 O. A. Petrenko , O. Young , D. Brunt , G. Balakrishnan , P. Manuel , D. D. Khalyavin , C. Ritter

Different types of order are discussed in the context of strongly correlated transition metal oxides, involving pure compounds and $3d^{3}-4d^{4}$ and $3d^{2}-4d^{4}$ hybrids. Apart from standard, long-range spin and orbital orders we…

强关联电子 · 物理学 2019-10-24 Wojciech Brzezicki

Given the paucity of single phase multiferroic materials (with large ferromagnetic moment), composite systems seem an attractive solution in the quest to realize magnetoelectric cou-pling between ferromagnetic and ferroelectric order…

介观与纳米尺度物理 · 物理学 2014-09-15 P. Jain , Q. Wang , M. Roldan , A. Glavic , V. Lauter , C. Urban , Z. Bi , T. Ahmed , J. Zhu , M. Varela , Q. Jia , M. R. Fitzsimmons

This article presents the results of several magnetic phases of doped La$_{2-x}$Sr$_x$CuO$_4$ using density-functional theory with an added Hubbard term (DFT+U). Doping factors from $x=0$ to 0.25 were examined. We found that a bond centered…

超导电性 · 物理学 2015-05-28 Simon Pesant , Michel Côté

CoSeO$_4$ has a structure consisting of edge-sharing chains of Co$^{2+}$ octahedra which are held together by SeO$_4^{2-}$ tetrahedra via shared oxygen atoms at the edges of the octahedra. DC magnetization measurements indicate a transition…

Mott insulators based on $4d$ and $5d$ transition-metal ions, where spin-orbit interaction plays a key role, can exhibit various forms of unusual magnetism. A particular example is the antiferromagnet Ca$_2$RuO$_4$ containing $d^4$…

强关联电子 · 物理学 2025-05-16 Jan Revenda , Krzysztof Wohlfeld , Jiří Chaloupka