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The intricate interplay between colloidal particle shape and precisely engineered interaction potentials has paved the way for the discovery of unprecedented crystal structures in both two and three dimensions. Here, we make use of…

软凝聚态物质 · 物理学 2023-11-27 Fabrizio Camerin , Susana Marín-Aguilar , Marjolein Dijkstra

DNA-coated colloids can self-assemble into an incredible diversity of crystal structures, but applications of this technology are limited by poor understanding and control over the dynamical crystallization pathways. To address this…

软凝聚态物质 · 物理学 2021-06-01 Alexander Hensley , William M. Jacobs , W. Benjamin Rogers

Diblock copolymers by virtue of the chemical dissimilarity between the constituting blocks exhibit microphase separation in the melt state. The phase separated melt can successfully be exploited to control the morphology of the final semi…

软凝聚态物质 · 物理学 2018-02-19 Chitrita Kundu , Nikhil S. Joshi , Ashok Kumar Dasmahapatra

This paper aims to elucidate the role of interface energy anisotropy in orientation selection during nucleation of new grains in a polycrystalline film growth. An assessment of (heterogeneous) nucleation probability as function of…

材料科学 · 物理学 2023-10-11 Martin Minar , Nele Moelans

In this paper the state-of-the-art for exploiting the unique physical and chemical properties of crystalline materials and their possible applications for development of crystalline nanocomposites with the tailored anisotropy were…

材料科学 · 物理学 2019-02-26 Nazariy Andrushchak , Petra Goering , Anatoliy Andrushchak

A simple numerical model which calculates the kinetics of crystallization involving randomly distributed nucleation and isotropic growth is presented. The model can be applied to different thermal histories and no restrictions are imposed…

材料科学 · 物理学 2008-11-17 J. Farjas , P. Roura

The assembly of colloidal cubic diamond is a challenging process since the shape and interaction parameters and the thermodynamic conditions where this structure is stable are elusive. The simultaneous use of shape-anisotropic particles and…

软凝聚态物质 · 物理学 2024-06-12 Susana Marín-Aguilar , Fabrizio Camerin , Marjolein Dijkstra

Studying the crystallization process of silicon is a challenging task since empirical potentials are not able to reproduce well the properties of both semiconducting solid and metallic liquid. On the other hand, nucleation is a rare event…

计算物理 · 物理学 2019-01-10 Luigi Bonati , Michele Parrinello

The classical nucleation theory finds the rate of nucleation proportional to the monomer concentration raised to the power, which is the `critical nucleaus size', ${n_c}$. The implicit assumption, that amyloids nucleate in the same way, has…

软凝聚态物质 · 物理学 2020-05-19 Cheng-Tai Lee , Eugene M. Terentjev

Polymorphism, which describes the occurrence of different lattice structures in a crystalline material, is a critical phenomenon in material science and condensed matter physics. It has emerged as a major focus for industry and regulatory…

材料科学 · 物理学 2021-01-26 Kyoung Hwan Choi , Da Young Hwang , Dong Hack Suh

We study the conditions under which and how an imposed cluster of fixed colloidal particles at prescribed positions triggers crystal nucleation from a metastable colloidal fluid. Dynamical density functional theory of freezing and Brownian…

软凝聚态物质 · 物理学 2009-11-13 Sven van Teeffelen , Christos N. Likos , Hartmut Löwen

We study the freezing kinetics of colloidal polycrystals made of micelles of Pluronic F108, a thermosensitive copolymer, to which a small amount of silica nanoparticles of size comparable to that of the micelles are added. We use rheology…

软凝聚态物质 · 物理学 2013-03-18 A. Louhichi , E. Tamborini , N. Ghofraniha , F. Caton , D. Roux , J. Oberdisse , L. Cipelletti , L. Ramos

Non-aligning self-propelled particles with purely repulsive excluded volume interactions undergo athermal motility-induced phase separation into a dilute gas and a dense cluster phase. Here, we use enhanced sampling computational methods…

软凝聚态物质 · 物理学 2016-10-05 Gabriel S. Redner , Caleb G. Wagner , Aparna Baskaran , Michael F. Hagan

The self-assembly of proteins into $\beta$-sheet-rich amyloid fibrils has been observed to occur with sigmoidal kinetics, indicating that the system initially is trapped in a metastable state. Here, we use a minimal lattice-based model to…

生物物理 · 物理学 2016-01-05 Anders Irbäck , Jonas Wessén

Using quasi-simultaneous synchrotron X-ray diffraction and tomography techniques, we have studied in-situ and in real-time the nucleation and co-growth dynamics of the peritectic structures in an Al-Mn alloy during solidification. We…

New metal-organic frameworks (MOFs) are periodically synthesized all over the world due to the wide range of societally and environmentally relevant applications they possess. However, the mechanisms and thermodynamics associated to MOF…

化学物理 · 物理学 2024-11-08 Emilio Méndez , Rocio Semino

Experimental DSC and Avrami curves for the crystallization of metallic glasses demonstrate nucleation at grain boundaries and thus indicate their grain structure, which refutes the generally accepted idea of glass as a homogeneous frozen…

材料科学 · 物理学 2025-06-27 Nikolay V. Alekseechkin

Nanocrystalline materials have been proposed for use in future fusion reactors due to their high grain boundary density that may act as a sink for irradiation-induced defects. We use molecular dynamics to model collision cascades in…

We study a simple growth model for (d+1)-dimensional films of binary alloys in which atoms are allowed to interact and equilibrate at the surface, but are frozen in the bulk. The resulting crystal is highly anisotropic: Correlations…

统计力学 · 物理学 2009-10-28 Barbara Drossel , Mehran Kardar

Over the past decade, topology has garnered great attention in a wide area of physics. In particular, it has exerted influence on photonics because carefully engineered photonic crystals and metamaterials can help explore the non-trivial…

光学 · 物理学 2021-01-14 Kyoung Hwan Choi , Da Young Hwang , Dong Hack Suh
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