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Cu$_2$IrO$_3$ has attracted recent interest due to its proximity to the Kitaev quantum spin liquid state and the complex structural response observed at high pressures. We use x-ray spectroscopy and scattering as well as electrical…

Material realization of the non-Abelian Kitaev spin liquid phase - an example of Ising topological order (ITO) - has been the subject of intense research in recent years. The $4d$ honeycomb Mott insulator $\alpha$-RuCl$_3$ has emerged as a…

强关联电子 · 物理学 2021-02-26 Jacob S. Gordon , Hae-Young Kee

We present a temperature-dependent resonant elastic soft x-ray scattering (REXS) study of the metal-insulator transition in Sr3(Ru1-xMnx)2O7, performed at both Ru and Mn L-edges. Resonant magnetic superstructure reflections, which indicate…

A pseudo honeycomb system Li2RuO3 exhibits a second-order-like transition at temperature T=Tc=540 K to a low-T nonmagnetic phase with a significant lattice distortion forming Ru-Ru pairs. For this system, we have calculated the band…

强关联电子 · 物理学 2015-05-13 Yoko Miura , Masatoshi Sato , Youichi Yamakawa , Tatsuro Habaguchi , Yoshiaki Ono

We investigate the electronic structure of two Ir$^{5+}$ honeycomb iridates, Sr$_3$CaIr$_2$O$_9$ and NaIrO$_3$, by means of resonant x-ray techniques. We confirm that Sr$_3$CaIr$_2$O$_9$ realizes a large spin-orbit driven non-magnetic $J =…

强关联电子 · 物理学 2025-12-08 A. de la Torre , B. Zager , J. R. Chamorro , M. H. Upton , G. Fabbris , D. Haskel , D. Casa , T. M. McQueen , K. W. Plumb

The dynamical mean-field theory together with the non-crossing approximation is used to set up a novel scheme to study the electronic structure of strongly correlated electron systems. The non-interacting band structure is obtained from a…

强关联电子 · 物理学 2007-05-23 M. B. Zoelfl , Th. Pruschke , J. Keller , A. I. Poteryaev , I. A. Nekrasov , V. I. Anisimov

Young's archetypal double-slit experiment forms the basis for modern diffraction techniques: the elastic scattering of waves yields an interference pattern that captures the real-space structure. Here, we report on an inelastic incarnation…

The $t_{2g}$ orbitals of an edge-shared transition-metal oxide with a honeycomb lattice structure form dispersionless electronic bands when only hopping mediated by the edge-sharing oxygens is accessible. This is due to the formation of…

强关联电子 · 物理学 2016-10-27 Beom Hyun Kim , Tomonori Shirakawa , Seiji Yunoki

We develop a formalism for calculating resonant inelastic x-ray scattering (RIXS) spectra in systems of itinerant electrons with arbitrary band structures, accounting for the effect of the positively-charged core hole exactly. We apply this…

超导电性 · 物理学 2013-12-24 David Benjamin , Israel Klich , Eugene Demler

We investigate the role of electron correlation in the electronic structure of honeycomb lattice Li$_2$RuO$_3$ using photoemission spectroscopy and band structure calculations. Monoclinic Li$_2$RuO$_3$ having Ru network as honeycomb lattice…

强关联电子 · 物理学 2023-01-24 Sakshi Bansal , Asif Ali , B. H. Reddy , Ravi Shankar Singh

We use synchrotron x-ray diffraction and electrical transport under pressure to probe both the magnetism and the structure of single crystal NiS2 across its Mott-Hubbard transition. In the insulator, the low-temperature antiferromagnetic…

强关联电子 · 物理学 2011-09-02 Yejun Feng , R. Jaramillo , A. Banerjee , J. M. Honig , T. F. Rosenbaum

Motivated by the rich interplay among electronic correlation, spin-orbit coupling (SOC), crystal-field splitting, and geometric frustrations in the honeycomb-like lattice, we systematically investigated the electronic and magnetic…

We use Ru $L_3$-edge resonant inelastic x-ray scattering (RIXS) to study the full range of excitations in Ca$_3$Ru$_2$O$_7$ from meV-scale magnetic dynamics through to the eV-scale interband transitions. This bilayer $4d$-electron…

强关联电子 · 物理学 2021-02-10 J. Bertinshaw , M. Krautloher , H. Suzuki , H. Takahashi , A. Ivanov , B. J. Kim , H. Gretarsson , B. Keimer

We employ density functional theory plus dynamical mean field theory and identify the physical origin of why two layers of SrVO$_3$ on a SrTiO$_3$ substrate are insulating: the thin film geometry lifts the orbital degeneracy which in turn…

We study Na2IrO3 by ARPES, optics, and band structure calculations in the local-density approximation (LDA). The weak dispersion of the Ir 5d-t2g manifold highlights the importance of structural distortions and spin-orbit coupling (SO) in…

Resonant Inelastic X-ray Scattering (RIXS) was used to measure the local electronic structure in few-layer exfoliated flakes of the van der Waals antiferromagnet NiPS$_3$. The resulting spectra show a systematic softening and broadening of…

强关联电子 · 物理学 2024-02-09 M. F. DiScala , D. Staros , A. de la Torre , A. Lopez , D. Wong , C. Schulz , M. Bartkowiak , B. Rubenstein , K. W. Plumb

We determine how the elementary excitations of iridium-oxide materials, which are dominated by a strong relativistic spin-orbit coupling, appear in Resonant Inelastic X-ray Scattering (RIXS). Whereas the RIXS spectral weight at the L2 x-ray…

强关联电子 · 物理学 2012-12-03 Luuk J. P. Ament , Giniyat Khaliullin , Jeroen van den Brink

We report on the Cu 1s resonant inelastic X-ray scattering (RIXS) of Cu-O one-dimensional (1D) strongly correlated insulator systems with contrasting atomic arrangements, namely edge-sharing CuGeO3 and corner-sharing Sr2CuO3. Owing to good…

A new-type structural transition has been found in Li2RuO3 with honeycomb lattice of edge-sharing RuO6-octahedra. With decreasing temperature T, the electrical resistivity exhibits an anomalous increase at T=Tc~540 K, suggesting the (metal…

强关联电子 · 物理学 2015-06-25 Yoko Miura , Yukio Yasui , Masatoshi Sato , Naoki Igawa , Kazuhisa Kakurai

We use resonant inelastic x-ray scattering (RIXS) at the Ir L3 edge to study the effect of hole doping upon the Jeff=1/2 Mott-insulating state in Sr2IrO4, via Rh replacement of the Ir site. The spin-wave gap, associated with XY-type…

强关联电子 · 物理学 2020-03-24 J. Bertinshaw , J. K. Kim , J. Porras , K. Ueda , N. H. Sung , A. Efimenko , A. Bombardi , Jungho Kim , B. Keimer , B. J. Kim