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We study experimentally and theoretically the exciton-phonon interaction in MoSe2 monolayers encapsulated in hexagonal BN, which has an important impact on both optical absorption and emission processes. The exciton transition linewidth…

The optical properties of semiconducting transition metal dichalcogenides are dominated by both neutral excitons (electron-hole pairs) and charged excitons (trions) that are stable even at room temperature. While trions directly influence…

Exciton-phonon coupling limits the homogeneous emission linewidth of nanocrystals. Hence, a full understanding of it is crucial. In this work, we statistically investigate exciton-phonon coupling by performing single-particle spectroscopy…

We investigate the correction of interlayer exciton binding energy in transition metal dichalcogenides double layers arising from the exciton-optical phonon coupling using the method of Lee-Low-Pines unitary transformation. We find that the…

介观与纳米尺度物理 · 物理学 2018-11-14 Zi-Wu Wang , Xi-Ying Dong , Run-Ze Li , Yao Xiao , Zhi-Qing Li

Temperature influences the performance of two-dimensional materials in optoelectronic devices. Indeed, the optical characterization of these materials is usually realized at room temperature. Nevertheless most {\it ab-initio} studies are…

介观与纳米尺度物理 · 物理学 2016-06-06 Alejandro Molina-Sánchez , Maurizia Palummo , Andrea Marini , Ludger Wirtz

Two-dimensional semiconducting transition metal dichalcogenides embedded in optical microcavities in the strong exciton-photon coupling regime may lead to promising applications in spin and valley addressable polaritonic logic gates and…

Exciton-phonon interactions govern the optical response of semiconductors, yet disentangling multiple coupling channels in lead halide perovskites remains challenging. We investigate CsPbBr3 microcrystals using photoluminescence, Raman and…

Excitonic quasi-particles, excitons/trions/bi-excitons, and their coupling with phonons and charge carriers play a crucial role in controlling the optical properties of atomically thin semiconducting 2D materials. In this work, we…

材料科学 · 物理学 2021-10-01 Deepu Kumar , Rahul Kumar , Mahesh Kumar , Pradeep Kumar

Probing phonons, quasi-particle excitations and their coupling has enriched our understanding of these 2D materials and proved to be crucial for developing their potential applications. Here, we report comprehensive temperature, 4-330 K,…

材料科学 · 物理学 2022-03-14 Deepu Kumar , Vivek Kumar , Rahul Kumar , Mahesh Kumar , Pradeep Kumar

The strong coupling between lattice modes and charges which leads to the formation of charge density waves in materials such as the transition-metal dichalcogenides may also give rise to superconductivity in the same materials, mediated by…

超导电性 · 物理学 2015-06-29 Jasper van Wezel , Paul Nahai-Williamson , Siddarth S. Saxena

We examine a mechanism by which excitons undergo ultrafast relaxation in common monolayer transition metal dichalcogenides. It is shown that at densities $\approx$ 1$\times$ 10$^{11}$ cm$^{-2}$ and temperatures $ \le 60$ K, excitons in well…

介观与纳米尺度物理 · 物理学 2016-06-29 A. Thilagam

The interaction between excitons and phonons in semiconductor nanocrystals plays a crucial role in the exciton energy spectrum and dynamics, and thus in their optical properties. We investigate the exciton2 phonon coupling in giant-shell…

The strong excitonic effect in monolayer transition metal dichalcogenide (TMD) semiconductors has enabled many fascinating light-matter interaction phenomena. Examples include strongly coupled exciton-polaritons and nearly perfect atomic…

介观与纳米尺度物理 · 物理学 2021-04-13 Hongchao Xie , Shengwei Jiang , Daniel A. Rhodes , James C. Hone , Jie Shan , Kin Fai Mak

A direct band gap, remarkable light-matter coupling as well as strong spin-orbit and Coulomb interaction establish two-dimensional (2D) crystals of transition metal dichalcogenides (TMDs) as an emerging material class for fundamental…

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

Monolayer transition metal dichalcogenides feature Coulomb-bound electron-hole pairs (excitons) with exceptionally large binding energy and coupled spin and valley degrees of freedom. These unique attributes have been leveraged for…

Coulomb bound electron-hole pairs, excitons, govern the optical properties of semi-conducting transition metal dichalcogenides like MoS$_2$ and WSe$_2$. We study optical transitions at the K-point for 2H homobilayer MoS$_2$ in Density…

Monolayered MoSe2 is a promising new material to investigate advanced light-matter coupling as it hosts stable and robust excitons with comparably narrow optical resonances. In this work, we investigate the evolution of the lowest lying…

介观与纳米尺度物理 · 物理学 2017-03-28 N. Lundt , A. Maryński , E. Cherotchenko , A. Pant , X. Fan , G. Sęk , S. Tongay , A. V. Kavokin , S. Höfling , C. Schneider

The efficiency of two-dimensional Dion-Jacobson-type materials relies on the complex interplay between electronic and lattice dynamics; however, questions remain about the functional role of exciton-phonon interactions. This study…

Cavity-integrated transition metal dichalcogenide excitons have recently emerged as a promising platform to study strong light-matter interactions and related cavity quantum electrodynamics phenomena. While this exciton-cavity system is…

应用物理 · 物理学 2020-03-10 David Rosser , Taylor Fryett , Albert Ryou , Abhi Saxena , Arka Majumdar
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