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Rare-earth chalcogenide compounds $\mathrm{ARECh_2}$ (A = alkali or monovalent metal, RE = rare earth, Ch = O, S, Se, Te) are a large family of quantum spin liquid (QSL) candidate materials. $\mathrm{NaYbS_2}$ is a representative member of…

强关联电子 · 物理学 2024-09-25 Weizhen Zhuo , Zheng Zhang , Mingtai Xie , Anmin Zhang , Jianting Ji , Feng Jin , Qingming Zhang

Very recently we revealed a large family of triangular lattice quantum spin liquid candidates named rare-earth chalcogenides, which features a high-symmetry structure without structural/charge disorders and spin impurities, and may serve as…

The family of rare earth chalcogenides $ARECh_{2}$ (A = alkali or monovalent ions, RE = rare earth, and Ch = O, S, Se, and Te) appears as an inspiring playground for studying quantum spin liquids (QSL). The crucial low-energy spin dynamics…

Recently, the family of rare-earth chalcohalides were proposed as candidate compounds to realize the Kitaev spin liquid (KSL). In the present work, we firstly propose an effective spin Hamiltonian consistents with the symmetry group of the…

After the discovery of the ARECh2 (A=alkali or monovalent ions, RE=rare-earth, Ch= chalcogen) triangular lattice quantum spin liquid (QSL) family, a series of its oxide, sulfide, and selenide counterparts has been consistently reported and…

强关联电子 · 物理学 2024-08-20 Weiwei Liu , Zheng Zhang , Dayu Yan , Jianshu Li , Zhitao Zhang , Jianting Ji , Feng Jin , Youguo Shi , Qingming Zhang

Frustrated quantum magnets are expected to host many exotic quantum spin states like quantum spin liquid (QSL), and have attracted numerous interest in modern condensed matter physics. The discovery of the triangular lattice spin liquid…

强关联电子 · 物理学 2018-10-02 Weiwei Liu , Zheng Zhang , Jianting Ji , Yixuan Liu , Jianshu Li , Xiaoqun Wang , Hechang Lei , Gang Chen , Qingming Zhang

The rare-earth chalcogenide $ARECh_{2}$ family ($A =$ alkali metal or monovalent ions, $RE =$ rare earth, $Ch =$ chalcogen) has emerged as a paradigmatic platform for studying frustrated magnetism on a triangular lattice. The family members…

强关联电子 · 物理学 2024-12-04 Mingtai Xie , Wenzhen Zhuo , Yanzhen Cai , Zheng Zhang , Qingming Zhang

Spin-orbit coupling is an important ingredient to regulate the many-body physics, especially for many spin liquid candidate materials such as rare-earth magnets and Kitaev materials. The rare-earth chalcogenides NaYbCh$_2$ (Ch = O, S, Se)…

In this paper, we performed thermodynamic and electron spin resonance (ESR) measurements to study low-energy magnetic excitations, which were significantly affected by crystalline electric field (CEF) excitations due to relatively small…

强关联电子 · 物理学 2021-08-24 Weiwei Liu , Zheng Zhang , Dayu Yan , Jianshu Li , Zhitao Zhang , Jianting Ji , Feng Jin , Youguo Shi , Qingming Zhang

Recently reported van der Waals layered honeycomb rare-earth chalcohalides REChX (RE = rare earth, Ch = chalcogen, and X = halogen) are considered to be promising Kitaev spin liquid (KSL) candidates. The high-quality single crystals of…

The interplay of magnetic correlations, crystal electric field interactions, and spin-orbit coupling in low-dimensional frustrated magnets fosters novel ground states with unusual excitations. Here, we report the magnetic properties and…

材料科学 · 物理学 2024-09-02 S. Guchhait , A. Painganoor , S. S. Islam , J. Sichelschmidt , M. D. Le , N. B. Christensen , R. Nath

We study the ultralow-temperature thermodynamics and thermal conductivity ($\kappa$) of the single-crystal rare-earth chalcogenides NaYbS$_2$ and NaYbSe$_2$, which have an ideal triangular lattice of the Yb$^{3+}$ ions and have been…

Tb2Ti2O7 is a pyrochlore antiferromagnet that has dynamical spins and only short-range correlations even at 50 mK; the lowest temperature explored so far, which is much smaller than the scale set by the Curie-Weiss temperature T_{CW}~14 K.…

统计力学 · 物理学 2009-12-16 Hamid R. Molavian , Paul A. McClarty , Michel J. P. Gingras

The thermodynamic properties of the pyrochlore Yb2Ti2O7 material are calculated using the numericallinked-cluster (NLC) calculation method for an effective anisotropic-exchange spin-1/2 Hamiltonian with parameters recently determined by…

强关联电子 · 物理学 2014-04-11 N. R. Hayre , K. A. Ross , R. Applegate , T. Lin , R. R. P. Singh B. D. Gaulin , M. J. P. Gingras

We report measurements of 19F nuclear spin-lattice relaxation 1/T1 as a function of temperature and external magnetic field in LiY0.998Ho0.002F4 single crystal, a single-ion magnet exhibiting interesting quantum effects. The 19F 1/T1 is…

介观与纳米尺度物理 · 物理学 2009-11-11 M. J. Graf , A. Lascialfari , F. Borsa , A. M. Tkachuk , B. Barbara

An indispensable step toward understanding magnetic interactions in rare-earth magnets is to determine the spatially anisotropic single-ion properties set by crystal electric field (CEF) physics. The CEF Hamiltonian yields a discrete energy…

Systematically magnetic and magnetothermal measurements at temperatures down to 2 K and magnetic fields up to 13.5 Tesla for Gd(OH)3 Single Crystal Nanowires - Quasi-1D Large Spin (S = -7/2) Chain Antiferromagnet have been conducted. We…

材料科学 · 物理学 2012-07-16 R. Zeng , C. F. Zhang , J. C. Debnath , P. Shamba , J. L. Wang , Z. X. Chen , Z. P. Guo , S. X. Dou

Kitaev spin liquid (KSL) system has attracted tremendous attention in past years because of its fundamental significance in condensed matter physics and promising applications in fault-tolerant topological quantum computation. Material…

强关联电子 · 物理学 2021-04-05 Jianting Ji , Mengjie Sun , Yanzhen Cai , Yimeng Wang , Yingqi Sun , Wei Ren , Zheng Zhang , Feng Jin , Qingming Zhang

The recently discovered dipole-octupole pyrochlore magnet Ce$_2$Hf$_2$O$_7$ is a promising three-dimensional quantum spin liquid candidate which shows no signs of ordering at low temperature. The low energy effective pseudospin-1/2…

We report the properties of a triangular lattice iron-chalcogenide antiferromagnet FeAl$_{2}$Se$_{4}$. The spin susceptibility reveals a significant antiferromagnetic interaction with a Curie-Weiss temperature {\Theta}$_{CW}$ ~ -200K and a…

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