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Porous electrodes{made of hierarchically nanostructured materials{are omnipresent in various electrochemical energy technologies from batteries and supercapacitors to sensors and electrocatalysis. Modeling the system-level macroscopic…

应用物理 · 物理学 2022-02-03 Anis Allagui , Hachemi Benaoum

Understanding ion relaxation dynamics in overlapping electric double layers (EDLs) is critical for the development of efficient nanotechnology based electrochemical energy storage, electrochemomechanical energy conversion and…

化学物理 · 物理学 2014-11-04 Vaibhav Thakore , James J. Hickman

We study the role of the electrical double layer (EDL) in the formation of the quasistatic electrical conductivity of suspensions of nanosized particles. A suspension is viewed as a system of hard-core--penetrable-shell particles. The…

软凝聚态物质 · 物理学 2024-01-15 M. Ya. Sushko , S. D. Balika

High-concentration aqueous electrolytes have shown promise as candidates for a safer, lower-cost battery system. Ionic conductivity is a key property required in high performing electrolytes; the Advanced Electrolyte Model (AEM) has…

Topological quantum materials (TQMs) have symmetry protected band structures with useful electronic properties that have applications in information, sensing, energy, and other technologies. In the past 10 years, the applications of TQMs in…

材料科学 · 物理学 2023-09-08 Huixia Luo , Peifeng Yu , Guowei Li , Kai Yan

MXene transition-metal carbides and nitrides are of growing interest for energy storage applications. These compounds are especially promising for use as pseudocapacitive electrodes due to their ability to convert energy electrochemically…

Electrochemical gating has been demonstrated as a powerful tool to tune the physical properties of two-dimensional (2D) materials, leading to lots of fascinating quantum phenomena. However, the reported liquid-nature electrolytes (e.g,…

应用物理 · 物理学 2022-04-27 Xin Hu , Shou-Xin Zhao , Yang Li , Zhao-Yuan Sun , Liang Zhen , Cheng-Yan Xu

The development of fast and strong microactuators that can be integrated in microdevices is an essential challenge due to a lack of appropriate driving principles. In this paper, a membrane actuator powered by internal combustion of…

应用物理 · 物理学 2024-08-07 Ilia Uvarov , Pavel Shlepakov , Vitaly Svetovoy

Polymer electrolytes present a promising solution to the challenges posed by aqueous electrolytes in energy storage systems, offering the flexibility needed for wearable electronics. Despite the increasing interest in polymer…

材料科学 · 物理学 2025-05-06 Roya Rajabi , Shichen Sun , Booker Wu , Jamil Khan , Kevin Huang

Several effective methods have been developed recently to demonstrate simultaneous high energy and high power density in Li - carbon fluoride (CF$_x$) batteries. These methods can achieve as high as 1000 Wh/kg energy density at 60-70 kW/kg…

材料科学 · 物理学 2023-03-28 Haobin Huo , Leon L. Shaw , Karoly Nemeth

Manipulating the electrostatic double layer and tuning the conductance in nanofluidic systems at salt concentrations of 100 mM or higher has been a persistent challenge. The primary reasons are (i) the short electrostatic proximity length,…

Nanoporous carbon materials containing small domains of sp2-carbon with highly disordered structures are promising for supercapacitor applications. Herein, we synthesize amorphous carbon nanofoam with 98% volumetric void fraction and low…

Electrical double layers play a key role in a variety of electrochemical systems. The mean free path of secondary electrons in aqueous solutions is on the order of a nanometer, making them suitable for probing of ultrathin electrical double…

Biophotovoltaics has emerged as a promising technology for generating renewable energy since it relies on living organisms as inexpensive, self-repairing and readily available catalysts to produce electricity from an abundant resource -…

Controlling the charge density in low-dimensional materials with an electrostatic potential is a powerful tool to explore and influence their electronic and optical properties. Conventional solid gates impose strict geometrical constraints…

We present the first application of phase field modeling to electrochemistry. A free energy functional that includes the electrostatic effect of charged particles leads to rich interactions between concentration, electrostatic potential,…

材料科学 · 物理学 2007-05-23 J. E. Guyer , W. J. Boettinger , J. A. Warren , G. B. McFadden

Multilayered graphene-based nanoporous membranes with electrolyte incorporated between individual sheets is a unique nano-heterostructure system in which nanoconfined electrons in graphene and ions confined in between sheets are intimately…

介观与纳米尺度物理 · 物理学 2020-06-30 Jing Xiao , Hualin Zhan , Zaiquan Xu , Xiao Wang , Ke Zhang , Zhiyuan Xiong , George P. Simon , Zhe Liu , Dan Li

Controlling electrochemical reactivity requires a detailed understanding of the charging behavior and thermodynamics of the electrochemical interface. Experiments can independently probe the overall charge response of the electrochemical…

化学物理 · 物理学 2022-03-10 Abhishek Shandilya , Kathleen Schwarz , Ravishankar Sundararaman

Superconducting radio-frequency cavities are commonly used in modern particle accelerators for applied and fundamental research. Such cavities are typically made of high-purity, bulk Nb and are cooled by a liquid helium bath at a…

仪器与探测器 · 物理学 2020-06-24 G. Ciovati , G. Cheng , U. Pudasaini , R. Rimmer

Protonic ceramic fuel cells can be operated at low temperatures, but their performances relying on bulk ion transfer in solid electrolytes are usually limited by much lower proton conductivity than 0.1 S/cm below 600 {\deg}C. Herein,…

化学物理 · 物理学 2021-10-29 Wei Zhang , Siyuan Fang , Hanrui Su , Wei Hao , Bohak Yoon , Gyeong S. Hwang , Kai Sun , Chung-Fu Chen , Yu Zhu , Yun Hang Hu
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