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相关论文: Polaritonic Chemistry: Collective Strong Coupling …

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Exciton polaritons are hybrid particles of excitons (bound electron-hole pairs) and cavity photons, which are renowned for displaying Bose Einstein condensation and other coherent phenomena at elevated temperatures. However, their formation…

介观与纳米尺度物理 · 物理学 2024-08-29 Kenneth Choo , Olivier Bleu , Jesper Levinsen , Meera M. Parish

Collective strong coupling of molecular ensembles to optical cavities opens a route to modifying matter through genuinely collective electronic correlations. Yet even in the absence of a cavity, Coulomb correlations are notoriously…

量子物理 · 物理学 2026-05-05 Dominik Sidler , Michael Ruggenthaler , Angel Rubio

Polaritonic modes in low-dimensional materials enable strong light-matter interactions and provide a platform for light manipulation at nanoscale. Very recently, a new class of polaritons has attracted considerable interest in…

Strong coupling between light and matter generates hybrid polariton modes. We present a continuum formalism that expresses the polariton modes in terms of light and matter densities of states (DOS). We derive exact expressions for the light…

材料科学 · 物理学 2024-12-03 Suman Gunasekaran , Ryan F. Pinard , Andrew J. Musser

We describe a new type of spatially periodic structure (lattice models): a polaritonic crystal (PolC) formed by a two-dimensional lattice of trapped two-level atoms interacting with quantised electromagnetic field in a cavity (or in a…

量子物理 · 物理学 2009-10-12 I. O. Barinov , A. P. Alodjants , S. M. Arakelian

Recent experiments have revealed the profound effect of strong light-matter interactions in optical cavities on the electronic ground state of molecular systems. This phenomenon, known as vibrational strong coupling (VSC), can modify…

量子物理 · 物理学 2023-12-19 Thomas Schnappinger , Markus Kowalewski

In the Reststrahlen region, between the transverse and longitudinal phonon frequencies, polar dielectric materials respond metallically to light and the resulting strong light-matter interactions can lead to the formation of hybrid…

介观与纳米尺度物理 · 物理学 2022-01-27 Christopher R. Gubbin , Simone De Liberato

We developed a new physical model to predict macroscopic properties of inorganic molten systems using a realistic description of inter-atomic interactions. Unlike the conventional approach, which tends to overestimate viscosity by several…

材料科学 · 物理学 2015-06-04 Vitaly V. Chaban , Yuriy V. Pereverzev , Oleg V. Prezhdo

Cavity-polaritons in semiconductor microstructures have emerged as a promising system for exploring nonequilibrium dynamics of many-body systems. Key advances in this field, including the observation of polariton condensation,…

介观与纳米尺度物理 · 物理学 2019-04-05 Aymeric Delteil , Thomas Fink , Anne Schade , Sven Höfling , Christian Schneider , Ataç Imamoğlu

In non-Hermitian open quantum systems, such as polariton condensates, local tailoring of gains and losses opens up an interesting possibility to realize functional optical elements. Here, we demonstrate that deliberately introducing losses…

Strong coupling between molecules and quantized fields has emerged as an effective methodology to engineer molecular properties. New hybrid states are formed when molecules interact with quantized fields. Since the properties of these…

化学物理 · 物理学 2023-06-28 Marco Romanelli , Rosario R. Riso , Tor S. Haugland , Enrico Ronca , Stefano Corni , Henrik Koch

Quantum-matter theory (QMT), based on the Schr\"odinger or Dirac equations, is firmly established for both intra- and intermolecular interactions. However, there are two key issues with QMT. First, its applicability to large molecular…

化学物理 · 物理学 2026-03-19 Reza Karimpour , Matteo Gori , Alexandre Tkatchenko

We theoretically and experimentally investigate quantum features of an interacting light-matter system from a multidisciplinary perspective, unifying approaches from semiconductor physics, quantum optics, and quantum information science. To…

Experiments have demonstrated that the strong light-matter coupling in polaritonic microcavities significantly enhances transport. Motivated by these experiments, we have solved the disordered multimode Tavis-Cummings model in the…

光学 · 物理学 2023-06-01 Georg Engelhardt , Jianshu Cao

We present an ab initio correlated approach to study molecules that interact strongly with quantum fields in an optical cavity. Quantum electrodynamics coupled cluster theory provides a non-perturbative description of cavity-induced effects…

化学物理 · 物理学 2020-12-07 Tor S. Haugland , Enrico Ronca , Eirik F. Kjønstad , Angel Rubio , Henrik Koch

Strong light-matter coupling between molecules and plasmonic nanoparticles give rise to new hybrid eigenstates of the coupled system, commonly referred to as polaritons, or more precisely, plexcitons. Over the last decade it has been amply…

化学物理 · 物理学 2024-02-06 Marco Romanelli , Stefano Corni

Lead halide perovskites have emerged as platforms for exciton-polaritonic studies at room temperature thanks to their excellent photoluminescence efficiency and synthetic versatility. In this work we find proof of strong exciton-photon…

The interaction Hamiltonian for a system of polarons a la Feynman in the presence of long range Coulomb interaction is derived and the dielectric function is computed in mean field. For large enough concentration a liquid of such particles…

强关联电子 · 物理学 2015-06-25 J. Lorenzana

The strong coupling of a dense layer of molecular excitons with surface-plasmon modes in a metal gives rise to polaritons (hybrid light-matter states) called plexcitons. Surface plasmons cannot directly emit into (or be excited by)…

介观与纳米尺度物理 · 物理学 2018-09-28 Joel Yuen-Zhou , Semion K. Saikin , Vinod M. Menon

The paradigm of $N$ quantum emitters coupled to a single cavity mode appears in many situations ranging from quantum technologies to polaritonic chemistry. The ideal case of identical emitters is elegantly modeled in terms of symmetric…

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