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Lithium-ion batteries (LIBs) are becoming an important energy storage solution to achieve carbon neutrality, but it remains challenging to characterise their internal states for the assurance of performance, durability and safety. This work…

经典物理 · 物理学 2023-04-27 Ming Huang , Niall Kirkaldy , Yan Zhao , Yatish Patel , Frederic Cegla , Bo Lan

Next-generation lithium-ion batteries with silicon anodes have positive characteristics due to higher energy densities compared to state-of-the-art graphite anodes. However, the large volume expansion of silicon anodes can cause high…

数值分析 · 数学 2024-04-03 R. Schoof , G. F. Castelli , W. Dörfler

Optimization of the formation step in lithium-ion battery manufacturing is challenging due to limited physical understanding of solid electrolyte interphase formation and the long testing time (~100 days) for cells to reach the end of life.…

A data-driven solution is provided for the fast-charging problem of lithium-ion batteries with multiple safety and aging constraints. The proposed method optimizes the charging current based on the observed history of measurable battery…

系统与控制 · 电气工程与系统科学 2024-05-20 Hamed Taghavian , Malin Andersson , Mikael Johansson

Describing Li-ion battery positive electrodes in terms of distinct transition metal or oxygen redox regimes can lead to confusion in understanding metal-ligand hybridisation, oxygen dimerisation, and degradation. There is a pressing need to…

The use of solid-state electrolytes to provide safer, next-generation rechargeable batteries is becoming more feasible as new materials with greater stability and higher ionic diffusion coefficients are designed. However, accurate…

材料科学 · 物理学 2021-01-08 Ardeshir Baktash , James C. Reid , Tanglaw Roman , Debra J. Searles

This paper is the second part of a series of papers about empirical approaches to open circuit voltage (OCV) modeling and its performance comparison in lithium-ion batteries. The first part of the series introduced various sources of…

系统与控制 · 电气工程与系统科学 2023-06-30 Prarthana Pillai , James Nguyen , Balakumar Balasingam

Due to its exceptional lithium storage capacity silicon is considered as a promising candidate for anode material in lithium-ion batteries (LIBs). In the present work we demonstrate that methods of the soft X-ray emission spectroscopy…

The correct assessment of battery states is essential to maximize battery pack performances while ensuring reliable and safe operation. This work introduces EIS2MOD, a novel modelling framework for Li-ion cells based on Distribution of…

系统与控制 · 电气工程与系统科学 2022-03-17 Pietro Iurilli , Claudio Brivio , Rafael E. Carrillo , Vanessa Wood

Lithium-ion batteries (LIBs) are the leading technology used in consumer electronics, electric vehicles, and grid-level electrochemical energy storage applications. The ever-increasing use of LIBs has highlighted a gap in understanding of…

Li-ion battery (LIB) research has continuing importance for the entire range of applications from consumer products to vehicle electrification and grid stabilization. In many cases, standard electrochemical methods only provide an overall…

We introduce a simple and efficient model to describe the potential energy surface of lithium diffusing in a solid-state ionic conductor. First, we assume that the Li atoms are fully ionized and we neglect the weak dependence of the…

材料科学 · 物理学 2019-02-07 Leonid Kahle , Aris Marcolongo , Nicola Marzari

This paper investigates the state estimation of a high-fidelity spatially resolved thermal- electrochemical lithium-ion battery model commonly referred to as the pseudo two-dimensional model. The partial-differential algebraic equations…

系统与控制 · 计算机科学 2015-08-04 A. M. Bizeray , S. Zhao , S. R. Duncan , D. A. Howey

Lithium-ion batteries are playing a key role in the sustainable energy transition. To fully exploit the potential of this technology, a variety of modeling, estimation, and prediction problems need to be addressed to enhance its design and…

系统与控制 · 电气工程与系统科学 2023-05-09 Gabriele Pozzato , Simona Onori

We present a structural and magnetic study on two batches of polycrystalline LiNi$_{0.8}$Mn$_{0.1}$Co$_{0.1}$O$_2$ (commonly known as Li NMC 811), a Ni-rich Li ion battery cathode material, using elemental analysis, X-ray and neutron…

Lithium-ion batteries dominate battery research and industry due to their long research history and high energy density. However, increasing demand and limited lithium resources have raised lithium prices and battery costs, motivating…

材料科学 · 物理学 2025-12-17 Caolin Ua Tuiscint , Jonathan N Coleman

A new era for energy storage devices, such as rechargeable batteries, has been opened in the last decades. However, commercially available energy storage devices are based mainly on critical elements such as Li, Co, Mn, P, Ni, and graphite…

材料科学 · 物理学 2024-11-18 Siripak Sangsinsorn , Sonia Dsoke , Oana Cojocaru-Mirédin

All-solid-state batteries are currently developed at high pace and show a strong potential for market introduction within the next years. Though their performance has improved considerably over the last years, investigation of their…

Robust and Real-time State of Charge (SOC) estimation is essential for Lithium Iron Phosphate (LFP) batteries, which are widely used in electric vehicles (EVs) and energy storage systems due to safety and longevity. However, the flat Open…

系统与控制 · 电气工程与系统科学 2025-07-03 Junzhe Shi , Shida Jiang , Shengyu Tao , Jaewong Lee , Manashita Borah , Scott Moura

Two-dimensional (2D) materials have received considerable attention as possible electrodes in Li-ion batteries (LIBs), although a deeper understanding of the Li adsorption behavior as well as broad screening of the materials space is still…

材料科学 · 物理学 2022-03-22 Sheng Gong , Shuo Wang , Taishan Zhu , Xi Chen , Jeffrey C. Grossman