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The slow decay of charge carriers in polymer-fullerene blends measured in transient studies has raised a number of questions about the mechanisms of nongeminate recombination in these systems. In an attempt to understand this behavior, we…

Transient photovoltage (TPV) is a technique frequently used to determine charge carrier lifetimes in thin-film solar cells such as organic, dye sensitized and perovskite solar cells. As this lifetime is often incident light intensity…

应用物理 · 物理学 2019-08-06 Oskar J. Sandberg , Kristofer Tvingstedt , Paul Meredith , Ardalan Armin

Transient reflectivity (TR) from thin films (6 - 40 nm thick) of the topological insulator Bi2Se3 reveal ultrafast carrier dynamics, which suggest the existence of both radiative and non-radiative recombination between electrons residing in…

介观与纳米尺度物理 · 物理学 2015-06-23 Yuri D. Glinka , Sercan Babakiray , Trent A. Johnson , Mikel B. Holcomb , David Lederman

Integration of organic semiconductors into flexible electronics requires that their optoelectronic properties remain stable under mechanical deformation. Among these, the optical band gap governs exciton generation and limits photovoltaic…

材料科学 · 物理学 2025-11-13 Mahya Ghorab , Ayush K. Ranga , Arnulf Materny , Veit Wagner , Mojtaba Joodaki

Materials research with a focus on enhancing the minority-carrier lifetime of the light-absorbing semiconductor is key to advancing solar energy technology for both early-stage and mature material platforms alike. Tin sulfide (SnS) is an…

The ultrafast relaxation and recombination dynamics of photogenerated electrons and holes in epitaxial graphene are studied using optical-pump Terahertz-probe spectroscopy. The conductivity in graphene at Terahertz frequencies depends on…

介观与纳米尺度物理 · 物理学 2015-05-13 Paul A. George , Jared Strait , Jahan Dawlaty , Shriram Shivaraman , Mvs Chandrashekhar , Farhan Rana , Michael G. Spencer

Microscale energy transport processes are crucial in microelectronics, energy harvesting devices, and emerging quantum materials. To study these processes, methods that can probe transport with conveniently tunable length scales are highly…

材料科学 · 物理学 2022-01-05 Usama Choudhry , Taeyong Kim , Melanie Adams , Jeewan Ranasinghe , Runqing Yang , Bolin Liao

We performed temperature dependent transient photovoltage and photocurrent measurements on poly(3-hexylthiophene):[6,6]-phenyl-C61 butyric acid methylester bulk heterojuction solar cells. We found a strongly charge carrier concentration and…

材料科学 · 物理学 2009-08-07 A. Foertig , A. Baumann , D. Rauh , V. Dyakonov , C. Deibel

The methodology for a heterodyned laser-induced transient thermal grating technique for non-contact, non-destructive measurements of thermal transport in opaque material is presented. Phase-controlled heterodyne detection allows us to…

We probe charge photogeneration and subsequent recombination dynamics in neat regioregular poly(3-hexylthiophene) films over six decades in time by means of time-resolved photoluminescence spectroscopy. Exciton dissociation at 10K occurs…

We have developed a transient thermoreflectance technique using picosecond pulsed and cw laser to study thermal conductivity and interface conductance in both thin-films and bulk materials. A real time-resolved system observes a thermal…

Black phosphorus is emerging as a promising semiconductor for electronic and optoelectronic applications. To study fundamental carrier properties, we performed ultrafast femtosecond pump-probe spectroscopy on thin film black phosphorus…

介观与纳米尺度物理 · 物理学 2017-03-13 Vasudevan Iyer , Peide Ye , Xianfan Xu

The dynamics of photocarriers in reduced graphene oxide thin films is studied by using ultrafast pump-probe spectroscopy. Time dependent differential transmissions are measured with sample temperatures ranging from 9 to 300 K. At each…

介观与纳米尺度物理 · 物理学 2015-05-18 Brian A. Ruzicka , Lalani K. Werake , Hui Zhao , Shuai Wang , Kian Ping Loh

We studied the recombination dynamics of charge carriers in organic bulk heterojunction solar cells made of the blend system poly(2,5-bis(3-dodecyl thiophen-2-yl) thieno[2,3-b]thiophene) (pBTCT-C12):[6,6]-phenyl-C61-butyric acid methyl…

Understanding the opto-electronic properties of semiconducting polymers under external strain is essential for their applications in flexible opto-electronic, light-emitting and photovoltaic devices. While prior studies have highlighted the…

应用物理 · 物理学 2021-11-24 Taeyong Kim , Saejin Oh , Usama Choudhry , Carl Meinhart , Michael L. Chabinyc , Bolin Liao

Optical grating technique, where optical gratings are generated via light inference, has been widely used to measure charge carrier and phonon transport in semiconductors. In this paper, compared are three types of transient optical grating…

材料科学 · 物理学 2018-05-07 Ke Chen , Xianghai Meng , Feng He , Yongjian Zhou , Jihoon Jeong , Nathanial Sheehan , Seth R Bank , Yaguo Wang

Using synchronized near-infrared (NIR) and terahertz (THz) lasers, we have performed picosecond time-resolved THz spectroscopy of transient carriers in semiconductors. Specifically, we measured the temporal evolution of THz transmission and…

凝聚态物理 · 物理学 2009-11-07 M. A. Zudov , A. P. Mitchell , A. H. Chin , J. Kono

We use optical pump--THz probe spectroscopy at low temperatures to study the hot carrier response in thin Bi$_2$Se$_3$ films of several thicknesses, allowing us to separate the bulk from the surface transient response. We find that for…

介观与纳米尺度物理 · 物理学 2015-06-23 R. Valdés Aguilar , J. Qi , M. Brahlek , N. Bansal , A. Azad , J. Bowlan , S. Oh , A. J. Taylor , R. P. Prasankumar , D. A. Yarotski

Graphene is a promising material for nonlinear THz applications owing to its high third-order susceptibility and tunable optical properties. Its strong nonlinear response, driven by free-carrier thermodynamics, facilitates efficient…

Atomically thin materials such as graphene are uniquely responsive to charge transfer from adjacent materials, making them ideal charge transport layers in phototransistor devices. Effective implementation of organic semiconductors as a…

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