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Present study investigates the photoabsorption properties of single crystal rutile TiO2 (110) surfaces after they have been implanted with low fluence of Cobalt ions. The surfaces, after implantation, demonstrate fabrication of…

High throughput theoretical methods are increasingly used to identify promising photocatalytic materials for hydrogen generation from water as a clean source of energy. While most promising water splitting candidates require co-catalyst…

材料科学 · 物理学 2022-02-14 Huaiyu , Wang , Rebecca Katz , Julian Fanghanel , Raymond E. Schaak , Venkatraman Gopalan

The characterization of Pt/TiO2 (Degussa P25) catalyst system using atomic resolution Z-contrast images and electron energy loss spectroscopy in the scanning transmission electron microscope has recently revealed that Pt particles have a…

材料科学 · 物理学 2009-11-11 Hakim Iddir , Vladimir Skavysh , Serdar Ogut , Nigel D. Browning

The structural, electronic, and optical properties of metal (Si, Ge, Sn, and Pb) mono- and co-doped anatase TiO$_{2}$ nanotubes are investigated, in order to elucidate their potential for photocatalytic applications. It is found that Si…

介观与纳米尺度物理 · 物理学 2020-04-29 Mohamed M. Fadlallah , Ulrich Eckern

In this study, we investigate noble metal free photocatalytic water splitting on natural anatase single crystal facets and on wafer slices of the [001] plane before and after these surfaces have been modified by high pressure hydrogenation…

应用物理 · 物理学 2020-04-30 Ning Liu , Hans-Georg Steinrueck , Andres Osvet , Yuyun Yang , Patrik Schmuki

The presence of small hematite (Fe2O3) clusters at low coverage on titanium dioxide (TiO2) surface has been observed to enhance photocatalytic activity, while excess loading of hematite is detrimental. We conduct a comprehensive density…

材料科学 · 物理学 2024-04-09 Kati Asikainen , Matti Alatalo , Marko Huttula , Bernardo Barbiellini , S. Assa Aravindh

In the present work, a simple strategy is used to thermally oxidize TiN nanopowder (ca. 20 nm) to an anatase phase of a TiO2:Ti3+:N compound. In contrast to the rutile phase of such a compound this photocatalyst provides photocatalytic…

材料科学 · 物理学 2016-10-21 Xuemei Zhou , Eva M. Zolnhofer , Nhat Truong Nguyen , Ning Liu , Karsten Meyer , Patrik Schmuki

Supported carbon nanosheets and carbon nanotubes served as sacrificial templates for preparing spacious TiO2 photocatalytic thin films. Amorphous TiO2 was deposited conformally on the carbonaceous template material by atomic layer…

In the present work, extended Argon ion bombardment was used to modify anatase TiO2 nanotube (NTs) layers. In situ X-ray photoelectron spectroscopy revealed a high content of sub-oxide formed (Ti3+, Ti2+ states) in the nanotube layers.…

材料科学 · 物理学 2016-10-14 Xuemei Zhou , Ning Liu , Patrik Schmuki

Electronic structures and optical properties of C-N-codoped anatase TiO2 were calculated by using GGA+U method based on the density functional theory. The calculated results showed that the N-doped, C-doped, and C-N-codoped TiO2 produced 2p…

材料科学 · 物理学 2015-08-10 Meili Guo , Jiulin Du

Titanium-based oxides are abundant, chemically stable, non-toxic, and highly versatile materials, with applications ranging from photovoltaics to catalysis. For rutile and anatase phases of Titanium dioxide (TiO2), the bandgap ranges from…

材料科学 · 物理学 2022-01-04 Lynet Allan , George O Amolo , Julius Mwabora , Silas Mureramanzi

Generally adopted design strategies for enhancing the photocatalytic activity are aimed at tuning properties such as the visible light response, the exposed crystal facets, and the nanocrystal shape. Here, we present a different approach…

Reduced titanium dioxide has recently attracted large attention, particularly for its unique co-catalyst-free H$_2$ heterogeneous photocatalytic application. The enhanced photocatalytic activity of the reduced TiO$_2$ was previously…

Nb3O2(OH) has emerged as a highly attractive photocatalyst based on its chemical stability, energetic band positions, and large active lattice sites. Compared to other various photocatalytic semiconductors, it can be synthesized easily.…

材料科学 · 物理学 2025-02-17 Wilayat Khan , Alishba Tariq , Jan Minar , Sawera Durrani , Abdul Raziq , Sikander Azam , Khalid Saeed

A first-principles study has been carried out to evaluate the electronic and optical properties of rutile Ti1-xCdxO2 as a possible photocatalytic material. It was found that Cd incorporation lead to the enhancement of p states in the top of…

材料科学 · 物理学 2012-10-03 X. D. Zhang , M. L. Guo , C. L. Liu , W. X. Li , X. F. Hong

Doping is one of the most common strategies for improving the photocatalytic and solar energy conversion properties of TiO$_2$, hence an accurate theoretical description of the electronic and optical properties of doped TiO$_2$ is of both…

TiO$_2$ anatase has its significant importance in energy and environmental research. However, the major drawback of this immensely popular semi-conductor is its large bandgap of 3.2 eV. Several non-metals have been doped experimentally for…

材料科学 · 物理学 2020-02-25 Pooja Basera , Shikha Saini , Saswata Bhattacharya

Thin films of amorphous (a)-TiO2 are ubiquitous as photocatalysts, protective coatings, photoanodes and in memory application, where they are exposed to excess electrons and holes. We investigate trapping of excess electrons and holes in…

材料科学 · 物理学 2020-08-19 David Mora-Fonz , Moloud Kaviani , Alexander L. Shluger

Photocatalytic materials are pivotal for the implementation of disruptive clean energy applications such as conversion of H$_{2}$O and CO$_{2}$ into fuels and chemicals driven by solar energy. However, efficient and cost-effective materials…

材料科学 · 物理学 2019-09-04 Zhao Liu , Joel Shenoy , Cesar Menéndez , Judy N. Hart , Charles C. Sorrell , Claudio Cazorla

Knowledge of the molecular frontier levels' alignment in the ground state can be used to predict the photocatalytic activity of an interface. The position of the adsorbate's highest occupied molecular orbital (HOMO) levels relative to the…

材料科学 · 物理学 2015-06-16 Huijuan Sun , Duncan J. Mowbray , Annapaola Migani , Jin Zhao , Hrvoje Petek , Angel Rubio