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Solar water splitting provides a promising path for sustainable hydrogen production and solar energy storage. One of the greatest challenges towards large-scale utilization of this technology is reducing the hydrogen production cost. The…

The splitting of water with sunlight using photoelectrochemical cell (PEC) to produce hydrogen is a promising avenue for sustainable energy production. The greatest virtue of PEC is that it uses sunlight as the only source to split water,…

化学物理 · 物理学 2013-05-14 Qiang Yu , Chuanbao Cao

The current state of the art in direct water splitting in photo-electrochemical cells (PECs) is presented together with: (i) a case study of water splitting using a simple solar cell with the most efficient water splitting electrodes and…

The majority of photoelectrochemical (PEC) water splitting cells cannot drive the overall water splitting reactions without the assistance of an external power source. To provide added power, the cells are usually connected to photovoltaic…

应用物理 · 物理学 2018-10-31 Gideon Segev , Jeffery Beeman , Ian D. Sharp

Although photoelectrochemical water splitting is likely to be an important and powerful tool to provide environmentally friendly hydrogen, most developments in this field have been conducted on a laboratory scale so far. In order for the…

Photoelectrochemical (PEC) water splitting to generate hydrogen is one of the most studied methods for converting solar energy into clean fuel because of its simplicity and potentially low cost. Despite over 40 years of intensive research,…

材料科学 · 物理学 2019-01-02 Ling-Ju Guo , Jun-Wei Luo , Tao He , Su-Huai Wei , Shu-Shen Li

Photoelectrochemical (PEC) water splitting is a promising method for conversing solar energy into chemical energy stored in the form of hydrogen. Nanostructured hematite ($\alpha$-Fe$_2$O$_3$) is one of the most attractive materials for…

In this review, we discuss disruptive decoupled water splitting schemes, in which the concurrent production of hydrogen and oxygen in close proximity to each other in conventional electrolysis is replaced by time- or space-separated…

应用物理 · 物理学 2020-07-28 Avigail Landman , Gideon S. Grader , Avner Rothschild

Photoelectrochemical solar water splitting is a promising approach to convert solar energy into sustainable hydrogen fuel using semiconductor electrodes. Due to their visible light absorption properties, oxynitrides have shown to be…

Photocatalytic water splitting offers a viable and sustainable method for hydrogen production. MXenes, a class of 2D transition-metal carbides/nitrides, have emerged as potential photocatalysts and co-catalysts due to their tunable…

材料科学 · 物理学 2025-06-17 C. B. Subba , Prasad Mattipally , J. Sivakumar , A. Laref , A. Yvaz , D. P. Rai , Z. Pachuau

A well-established procedure for the photoelectrochemical (PEC) splitting of water relies on using porous electrodes of WO3 sensitized with BiVO4 as a visible scavenger photoanode semiconductor. In this work, we propose an evolved…

In this work we present a simulation of the semiconductor electrodes of photoelectrochemical (PEC) water splitting cells based on the nonequilibrium Green's function (NEGF) formalism. While the performance of simple PEC cells can be…

介观与纳米尺度物理 · 物理学 2023-11-06 Lassi Hällström , Ilkka Tittonen

Hydrogen is considered a promising environmentally friendly energy carrier for replacing traditional fossil fuels. In this context, photoelectrochemical (PEC) cells effectively convert solar energy directly to H2 fuel by water…

应用物理 · 物理学 2019-03-22 Sebastiano Bellani , Maria Rosa Antognazza , Francesco Bonaccorso

The low conversion rate and efficiency always weaken the performance of thermochemical water-splitting reaction. Herein, we, for the first time, conducted the thermodynamic study of a hydrogen permeable membrane (HPM) in an isothermal…

材料科学 · 物理学 2018-08-08 Chenxi Sui , Hongsheng Wang , Xiang Liu , Xuejiao Hu

Photocatalytic water splitting has greatly stimulated as an ideal technique for producing hydrogen (H$_{2}$) fuel by employing two renewable sources, i.e., water and solar energy. Here, we have adopted a facile hydrothermal approach for the…

化学物理 · 物理学 2022-01-04 Fahmida Sharmin , Dayal Chandra Roy , M. A. Basith

Due to the energy supply pressure caused by non-renewable fuels as well as the environment-related issues, the efficient conversion of solar-chemical energy via photo-induced water splitting is one of the promising strategies to address the…

化学物理 · 物理学 2021-03-23 Zhexu Xi

Recent rapid progress in efficiencies for solar water splitting by photoelectrochemical devices has enhanced its prospects to enable storable renewable energy. Efficient solar fuel generators all use tandem photoelectrode structures, and…

Efficient artificial photosynthesis systems are currently realized as catalyst- and surfacefunctionalized photovoltaic tandem- and triple-junction devices, enabling photoelectrochemical (PEC) water oxidation while simultaneously recycling…

The production of hydrogen from water using only a catalyst and solar energy is one of the most challenging and promising outlets for the generation of clean and renewable energy. Semiconductor photocatalysts for solar hydrogen production…

Gallium selenide (GaSe) is a layered compound, which has been exploited in nonlinear optical applications and photodetectors due to its anisotropic structure and pseudo-direct optical gap. Theoretical studies predicted that its…

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