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Twisted transition metal dichalcogenides (TMDs) present an intriguing platform for exploring excitons and their transport properties. By introducing a twist angle, a moir\'e superlattice forms, providing a spatially dependent exciton energy…

介观与纳米尺度物理 · 物理学 2024-01-17 Willy Knorr , Samuel Brem , Giuseppe Meneghini , Ermin Malic

Monolayers of transition-metal dichalcogenides such as WSe2 have become increasingly attractive due to their potential in electrical and optical applications. Because the properties of these 2D systems are known to be affected by their…

A self-consistent scheme for the calculations of the interacting groundstate and the near bandgap optical spectra of mono- and multilayer transition-metal-dichalcogenide systems is presented. The approach combines a dielectric model for the…

介观与纳米尺度物理 · 物理学 2018-01-24 Lars Meckbach , Tineke Stroucken , Stephan W. Koch

Monolayers of transition metal dichalcogenides (TMDs) exhibit bright photoluminescence, a desirable property for light-emitting diodes and single-photon emitters. Because the emission intensity is heavily influenced by factors such as…

介观与纳米尺度物理 · 物理学 2026-01-06 Juri G. Crimmann , Sander J. W. Vonk , Yannik M. Glauser , Gabriel Nagamine , David J. Norris

Monolayer SnS2 has emerged as a promising visible-light photocatalyst for photoelectrochemical applications, owing to its strong optical absorption in the visible range and excellent chemical stability. Despite its reduced dimensionality -…

介观与纳米尺度物理 · 物理学 2026-04-29 Vinicius Alves Bastos , Fulvio Paleari , Eleonora Luppi , Marco Gibertini , Alice Ruini

Enhanced Coulomb interactions in monolayer transition metal dichalcogenides cause tightly bound electron-hole pairs (excitons) which dominate their linear and nonlinear optical response. The latter includes bleaching, energy…

介观与纳米尺度物理 · 物理学 2020-06-25 Florian Katsch , Malte Selig , Andreas Knorr

Atomically thin transition metal dichalcogenides (TMDs) are direct-gap semiconductors with strong light-matter and Coulomb interaction. The latter accounts for tightly bound excitons, which dominate the optical properties of these…

Interlayer excitons (IXs) in hetero-bilayers of transition metal dichalcogenides (TMDs) represent an exciting emergent class of long-lived dipolar composite bosons in an atomically thin, near-ideal two-dimensional (2D) system. The…

Recent results on the optical properties of mono- and few-layers of semiconducting transition metal dichalcogenides are reviewed. Experimental observations are presented and discussed in the frame of existing models, highlighting the limits…

介观与纳米尺度物理 · 物理学 2017-09-19 M. Koperski , M. R. Molas , A. Arora , K. Nogajewski , A. O. Slobodeniuk , C. Faugeras , M. Potemski

In bilayers of semiconducting transition metal dichalcogenides, the twist angle between layers can be used to introduce a highly regular periodic potential modulation on a length scale that is large compared to the unit cell. In such…

材料科学 · 物理学 2022-04-27 N. Götting , F. Lohof , C. Gies

We report the first direct spectroscopic evidence for coherent electronic coupling between excitons and trions in atomically thin transition metal dichalcogenides, specifically monolayer MoSe2. Signatures of coupling appear as isolated…

介观与纳米尺度物理 · 物理学 2014-09-30 Akshay Singh , Galan Moody , Sanfeng Wu , Yanwen Wu , Nirmal J. Ghimire , Jiaqiang Yan , David G. Mandrus , Xiaodong Xu , Xiaoqin Li

Excitons -- elementary excitations formed by bound electron-hole pairs -- govern the optical properties and excited-state dynamics of materials. In two-dimensions (2D), excitons are theoretically predicted to have a linear energy-momentum…

材料科学 · 物理学 2025-03-14 Luna Y. Liu , Steffi Y. Woo , Jinyuan Wu , Bowen Hou , Cong Su , Diana Y. Qiu

We study a 2D system of trion-polaritons at the quantum level and demonstrate that for monolayer semiconductors they can exhibit a strongly nonlinear optical response. The effect is due to the composite nature of trion-based excitations…

量子物理 · 物理学 2020-11-11 O. Kyriienko , D. N. Krizhanovskii , I. A. Shelykh

Monolayer transition-metal dichalcogenides (ML-TMDs) offer exciting opportunities to test the manifestations of many-body interactions through changes in the charge density. Tuning the charge density by a gate voltage leads to profound…

材料科学 · 物理学 2019-03-18 Benedikt Scharf , Dinh Van Tuan , Igor Žutić , Hanan Dery

In recent years, enhanced light-matter interactions through a plethora of dipole-type polaritonic excitations have been observed in two-dimensional (2D) layered materials. In graphene, electrically tunable and highly confined…

Coherent coupling between excitons is at the heart of many-body interactions with transition metal dichalcogenide (TMD) heterostructures as an emergent platform for the investigation of these interactions. We employ multi-dimensional…

介观与纳米尺度物理 · 物理学 2022-01-05 Torben L. Purz , Eric W. Martin , Pasqual Rivera , William G. Holtzmann , Xiaodong Xu , Steven T. Cundiff

The interaction between off-resonant laser pulses and excitons in monolayer transition metal dichalcogenides is attracting increasing interest as a route for the valley-selective coherent control of the exciton properties. Here, we extend…

Two-dimensional transition metal dichalcogenides (2D TMDCs) are promising candidates for ultra-thin active nanophotonic elements due to the strong tunable excitonic resonances that dominate their optical response. Here we demonstrate…

光学 · 物理学 2023-04-26 Melissa Li , Claudio U. Hail , Souvik Biswas , Harry A. Atwater

Fabricating van der Waals (vdW) bilayer heterostructures (BL-HS) by stacking the same or different two-dimensional (2D) layers, offers a unique physical system with rich electronic and optical properties. Twist-angle between component…

介观与纳米尺度物理 · 物理学 2020-12-17 Kha Tran , Junho Choi , Akshay Singh

Structural defects in 2D-transition metal dichalcogenides are critical in modulating their optical and electrical behavior. Nevertheless, precise defect control within the monolayer regime poses a significant challenge. Herein, a…

介观与纳米尺度物理 · 物理学 2025-09-30 Anagha Gopinath , Faiha Mujeeb , Subhabrata Dhar , Jyoti Mohanty