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This study reports a general scenario for the out-of-equilibrium features of collapsing polymeric architectures. We use molecular dynamics simulations to characterize the coarsening kinetics, in bad solvent, for several macromolecular…

软凝聚态物质 · 物理学 2019-12-10 Mariarita Paciolla , Daniel J. Arismendi-Arrieta , Angel J. Moreno

We study conserved one-dimensional models of particle diffusion, attachment and detachment from clusters, where the detachment rates decrease with increasing cluster size as gamma(m) ~ m^{-k}, k>0. Heuristic scaling arguments based on…

统计力学 · 物理学 2009-11-13 F. D. A. Aarao Reis , R. B. Stinchcombe

A simple three-dimensional model of a fluid whose constituent particles interact via a short range attractive and long range repulsive potential is used to model the aggregation into large spherical-like clusters made up of hundreds of…

软凝聚态物质 · 物理学 2025-02-11 Antonio Díaz-Pozuelo , Diego González-Salgado , Enrique Lomba

The binodals and the non-ergodicity lines of a binary mixture of hard sphere-like particles with large size ratio are computed for studying the interplay between dynamic arrest and phase separation in depletion-driven colloidal mixtures.…

软凝聚态物质 · 物理学 2009-11-13 Ph. Germain , S. Amokrane

We solve the standard Lifshitz-Slyozov (LS) model with conservation of total particles in the limit of small super-saturation. The new element is an effective initial condition that follows from the initial exhaustion of nucleation as…

材料科学 · 物理学 2013-05-29 Yossi Farjoun , John C. Neu

In an expanding universe, velocity field and gravitational force field are proportional to each other in the linear regime. Neither of these quantities evolve in time and these can be scaled suitably so that the constant of proportionality…

天体物理学 · 物理学 2009-10-28 J. S. Bagla , T. Padmanabhan

We here discuss the results of 3d MonteCarlo simulations of a minimal lattice model for gelling systems. We focus on the dynamics, investigated by means of the time autocorrelation function of the density fluctuations and the particle mean…

软凝聚态物质 · 物理学 2007-05-23 E. Del Gado , A. Fierro , L. de Arcangelis , A. Coniglio

We present results from a detailed simulation of a quasi-2D dissipative granular gas, kept in a non-condensed steady state via vertical shaking over a rough substrate. This gas shows a weak power-law decay in the tails of its Pair…

软凝聚态物质 · 物理学 2015-05-19 J. A. Perera-Burgos , G. Perez-Angel , Y. Nahmad-Molinari

With numerical simulations of the mW model of water, we investigate the energetic stability of crystalline clusters for both Ice I (cubic and hexagonal ice) and for the metastable Ice 0 phase as a function of the cluster size. Under a large…

软凝聚态物质 · 物理学 2019-09-04 Fabio Leoni , Rui Shi , Hajime Tanaka , John Russo

We compare the slow dynamics of irreversible gels, colloidal gels, glasses and spin glasses by analyzing the behavior of the so called non-linear dynamical susceptibility, a quantity usually introduced to quantitatively characterize the…

软凝聚态物质 · 物理学 2015-06-25 A. Coniglio , T. Abete , A. de Candia , E. Del Gado , A. Fierro

Mode-coupling theory (MCT) predicts arrest of colloids in terms of their volume fraction, and the range and depth of the interparticle attraction. We discuss how effective values of these parameters evolve under cluster aggregation. We…

软凝聚态物质 · 物理学 2009-11-10 K. Kroy , M. E. Cates , W. C. K. Poon

We study a two-dimensional model for interacting colloidal particles which displays spontaneous clustering. Within this model we investigate the competition between the pinning to a periodic corrugation potential, and a sideways constant…

软凝聚态物质 · 物理学 2018-05-23 Mirko Rossini , Lorenzo Consonni , Andrea Stenco , Luciano Reatto , Nicola Manini

We study gelation in suspensions of model colloidal particles with short-ranged attractive and long-ranged repulsive interactions by means of three-dimensional fluorescence confocal microscopy. At low packing fractions, particles form…

软凝聚态物质 · 物理学 2009-11-10 Andrew I. Campbell , Valerie J. Anderson , Jeroen S. van Duijneveldt , Paul Bartlett

We present large-scale molecular dynamics simulations to study the free evolution of granular gases. Initially, the density of particles is homogeneous and the velocity follows a Maxwell-Boltzmann (MB) distribution. The system cools down…

统计力学 · 物理学 2016-09-21 Prasenjit Das , Sanjay Puri , Moshe Schwartz

The premelting plays an important role in ice growth, but there is a significant gap in our knowledge between the atomistic premelting surface structure and the macroscopic growth mechanism. In this work, using large-scale molecular…

化学物理 · 物理学 2022-11-04 Shifan Cui , Haoxiang Chen , Zhengpu Zhao

We present a model for sticky particles in which cluster sizes after a reaction have $\ell$ fewer total particles than the sum of their reactants. The finite particle system is modeled as a Markov process under a mean-field assumption for…

偏微分方程分析 · 数学 2026-04-16 Joseph Klobusicky , Matthew Rakauskas

The pair-correlation function $g(r,t)$ and its Fourier transform, the structure factor $S(q,t)$, are computed during the gelation process of identical spherical particles using the diffusion-limited cluster-cluster aggregation model in a…

凝聚态物理 · 物理学 2009-10-28 Anwar Hasmy , Rémi Jullien

The addition of enough non-adsorbing polymer to an otherwise stable colloidal suspension gives rise to a variety of phase behavior and kinetic arrest due to the depletion attraction induced between the colloids by the polymers. We report a…

软凝聚态物质 · 物理学 2024-06-19 Sam E Griffiths , Nick Koumakis , Aidan T Brown , Teun Vissers , Patrick B Warren , Wilson C K Poon

Colloidal model systems allow studying crystallization kinetics under fairly ideal conditions with rather well characterized pair interactions and minimized external influences. In complementary approaches therefore experiment, analytic…

软凝聚态物质 · 物理学 2015-06-19 Thomas Palberg

This paper analyzes the compaction behavior of assemblies composed of soft (elastic) spherical particles beyond the jammed state, using three-dimensional non-smooth contact dynamic simulations. The assemblies of particles are characterized…

软凝聚态物质 · 物理学 2021-09-09 Manuel Cárdenas-Barrantes , David Cantor , Jonathan Barés , Mathieu Renouf , Emilien Azéma