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Dielectrics' refractive index limits photonics miniaturization. By coupling light to metal's free electrons, plasmonic devices achieve deeper localization, which scales with the device geometric size. However, when localization approaches…

Polarization-dependent scattering anisotropy of cylindrical nanowires has numerous potential applications in, for example, nanoantennas, photothermal therapy, thermophotovoltaics, catalysis, sensing, optical filters and switches. In all…

介观与纳米尺度物理 · 物理学 2022-03-29 Vaibhav Thakore , Tapio Ala-Nissila , Mikko Karttunen

Composite and janus type metallo-dielectric nanoparticles are increasingly considered as a means to control the spatial and temporal behavior of electromagnetic fields in diverse applications such as coupling to quantum emitters, achieve…

We study the electron-energy loss spectra of strongly correlated electronic systems doped away from half-filling using dynamical mean-field theory ($d=\infty$). The formalism can be used to study the loss spectra in the optical (${\bf…

强关联电子 · 物理学 2009-10-31 Luis Craco , Mukul S. Laad

The effect of the electron temperature on both the light absorption and the scattering by metal nanoparticles (MNs) with excitation of the surface plasmon electron vibrations is studied in the framework of the kinetic theory. The formulae…

介观与纳米尺度物理 · 物理学 2013-11-25 N. I. Grigorchuk

Hot carrier spatial and momentum distributions in nanoplasmonic systems depend sensitively on the optical excitation parameters and nanoscale geometry, which therefore determine the efficiency and functionality of plasmon-enhanced…

介观与纳米尺度物理 · 物理学 2021-02-03 Jacob Pettine , Sean M. Meyer , Fabio Medeghini , Catherine J. Murphy , David J. Nesbitt

Noble metal nanoparticles exhibit localized plasmon resonance modes that span the visible and near-infrared spectral ranges and have many applications. Modifying the size, shape, and composition of the nanoparticles changes the number of…

Spatial confinement of matter in functional nanostructures has propelled these systems to the forefront of nanoscience, both as a playground for exotic physics and quantum phenomena and in multiple applications including plasmonics,…

Electron energy loss spectroscopy is consolidating as a powerful tool to explore electronic (as well as vibrational) excitations of matter, including molecules. Performed in a scanning transmission electron microscope, this technique is…

化学物理 · 物理学 2021-03-05 Ciro A. Guido , Enzo Rotunno , Matteo Zanfrognini , Stefano Corni , Vincenzo Grillo

This review discusses how low-energy, valence excitations created by swift electrons can render information on the optical response of structured materials with unmatched spatial resolution. Electron microscopes are capable of focusing…

材料科学 · 物理学 2012-11-13 F. J. Garcia de Abajo

In previous work a different and powerful, analytical, technique was used to get data, such as the absolute atom concentration (AAC), specimen thickness etc., from public domain boron nitride EELS spectrum collected under a collection…

材料科学 · 物理学 2020-09-24 Noureddine Hadji

Contemporary quantum plasmonics capture subtle corrections to the properties of plasmonic nano-objects in equilibrium. Here, we demonstrate nonequilibrium spill-out redistribution of the electronic density at the ultrafast time scale. As…

Inspired by recent measurements on individual metallic nanospheres that can not be explained with traditional classical electrodynamics, we theoretically investigate the effects of nonlocal response by metallic nanospheres in three distinct…

介观与纳米尺度物理 · 物理学 2014-03-07 Thomas Christensen , Wei Yan , Søren Raza , Antti-Pekka Jauho , N. Asger Mortensen , Martijn Wubs

We investigated the plasmonic modes in a two-dimensional quasicrystalline array of metal nanoparticles. The polarization of the modes is in the array plane. A simplified eigen-decomposition method is presented with the help of rotational…

光学 · 物理学 2012-12-11 Zi-Lan Deng , Jian-Wen Dong , He-Zhou Wang

Angular resolved electron energy-loss spectroscopy (EELS) gives access to the momentum and the energy dispersion of electronic excitations and allows to explore the transition from individual to collective excitations. Dimensionality and…

原子与分子团簇 · 物理学 2015-09-02 Michael Schüler , Jamal Berakdar , Yaroslav Pavlyukh

Plasmon resonance in metals represents the collective oscillation of the free electron gas density and enables enhanced light-matter interactions in nanoscale dimensions. Traditionally, the classical Drude model describes the plasmonic…

A new type of excitations by highly focused electron beams in scanning transmission electron microscopes is predicted for nanoparticles. The calculated electron energy loss spectra of metallic (silver) and insulating (SiO(sub2))…

材料科学 · 物理学 2011-11-09 M. A. Itskovsky , H. Cohen , T. Maniv

We analyze dispersion properties of metal-dielectric nanostructured metamaterials. We demonstrate that, in a sharp contrast to the results for the corresponding effective medium, the structure demonstrates strong optical nonlocality due to…

光学 · 物理学 2015-05-27 Alexey A. Orlov , Pavel M. Voroshilov , Pavel A. Belov , Yuri S. Kivshar

In this article, we explore the anisotropic electron energy loss spectrum (EELS) in monolayer phosphorene based on ab-initio time dependent density functional theory calculations. Similar to black phosphorous, the EELS of undoped monolayer…

介观与纳米尺度物理 · 物理学 2017-07-26 Barun Ghosh , Piyush Kumar , Anmol Thakur , Yogesh Singh Chauhan , Somnath Bhowmick , Amit Agarwal

Aluminum nanostructures have recently been at the focus of numerous studies due to their properties including oxidation stability and surface plasmon resonances covering the ultraviolet and visible spectral windows. In this article, we…