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The double-slit interference in single-photon ionization of the diatomic molecular ion $\mathrm{H}_2^+$ is theoretically studied beyond the dipole approximation. Via simulating and comparing the interactions of the prealigned…

原子物理 · 物理学 2021-11-24 Kunlong Liu , Yibo Hu , Qingbin Zhang , Peixiang Lu

Triple photoionization of Xe3+, Xe4+ and Xe5+ ions has been studied in the energy range 670-750 eV, including the 3d ionization threshold. The photon-ion merged-beam technique was used at a synchrotron light source to measure the absolute…

The creation of superpositions of hole states via single-photon ionization using attosecond extreme-ultraviolet pulses is studied with the time-dependent configuration interaction singles (TDCIS) method. Specifically, the degree of…

原子物理 · 物理学 2011-02-04 Stefan Pabst , Loren Greenman , Phay J. Ho , David A. Mazziotti , Robin Santra

We present an experimental and theoretical energy- and angle-resolved study on the photoionization dynamics of non-resonant one-color two-photon single valence ionization of neutral N$_2$ molecules. Using 9.3 eV photons produced via high…

Using the photon-ion merged-beams technique at a synchrotron light source, we have measured relative cross sections for single and up to five-fold photoionization of Fe$^{2+}$ ions in the energy range 690--920 eV. This range contains…

We formulate a general hybrid quantum-classical technique to describe the interaction of diatomic molecules with XUV pulses. We demonstrate the accuracy of our model in the context of the interaction of the O$_2$ molecule with an XUV pulse…

We report on a precision measurement of the $(5\mathrm{p})^{5}6\mathrm{p} \, [1/2]_{0}\leftarrow (5\mathrm{p})^{6} \, ^{1}\mathrm{S}_{0}$ transition wavenumber of Xe by Doppler-free two-photon spectroscopy using…

原子物理 · 物理学 2025-09-11 M. H. Rayment , R. Stech , F. Merkt

We provide the experimental evidence that the single electron capture process in slow collisions between O$^{3+}$ ions and neon dimer targets leads to an unexpected production of low-energy electrons. This production results from the…

We review the main aspects of multiple photoionization processes in atoms exposed to intense, short wavelength radiation. The main focus is the theoretical framework for the description of such processes as well as the conditions under…

原子物理 · 物理学 2014-01-21 P. Lambropoulos , G. M. Nikolopoulos

function of the CEP, we observe a transition from a modulated to a continuous SHHG spectrum, indicating the transition from double to high-contrast isolated attosecond pulse emission. Single shot-acquisitions of XUV spectral continua…

Double ionization of an atom by single-photon absorption in the presence of a neighbouring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly to the other atom,…

原子物理 · 物理学 2020-02-19 A. Eckey , A. B. Voitkiv , C. Müller

The strong coupling between two autoionizing states in helium is studied theoretically with the pump-probe scheme. An isolated 100-as XUV pulse is used to excite helium near the 2s2p(1P) resonance state in the presence of an intense…

原子物理 · 物理学 2012-05-23 Wei-Chun Chu , Song-Feng Zhao , C. D. Lin

Above 54.4 eV, two-photon double ionization of helium is dominated by a sequential absorption process, producing characteristic behavior in the single and triple differential cross sections. We show that the signature of this process is…

原子物理 · 物理学 2009-11-13 D. A. Horner , T. N. Rescigno , C. W. McCurdy

Absolute Ar XK (3 keV) and Xe XL (4 keV) photon yields are measured as a function of laser peak intensity, for large (104 - 105 atoms) argon and xenon clusters submitted to intense laser pulses. A clear threshold behavior is observed. The…

原子与分子团簇 · 物理学 2007-05-23 C. Prigent , L. Adoui , E. Lamour , J. -P. Rozet , D. Vernhet , O. Gobert , P. Meynadier , D. Normand , M. Perdrix

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…

Photo-stimulated desorption (PSD) of Xe atoms from the Au(001) surface in thermal and nonthermal regimes was investigated by the time-of-flight measurement at photon energies of 6.4 and 2.3 eV. Xe was desorbed in a thermal way at high laser…

介观与纳米尺度物理 · 物理学 2016-06-14 Akihiko Ikeda , Masuaki Matsumoto , Shohei Ogura , Katsuyuki Fukutani , Tatsuo Okano

Attosecond noncollinear four wave mixing spectroscopy with one attosecond extreme ultraviolet (XUV) pulse and two few-cycle near-infrared (NIR) pulses was used to measure the autoionization decay lifetimes of inner valence electronic…

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

化学物理 · 物理学 2017-05-18 David Ayuso

We present a combined experimental and theoretical study on the photodissociation dynamics of ion-pair formation in O$_2$ following resonant two-photon absorption of a 9.3 eV femtosecond pulse, where the resulting O$^+$ ions are detected…

化学物理 · 物理学 2020-08-28 Kirk A. Larsen , Robert R. Lucchese , Daniel S. Slaughter , Thorsten Weber

Carrier and phonon dynamics in a multilayer WSe2 film are captured by extreme ultraviolet (XUV) transient absorption (TA) spectroscopy at the W N6,7, W O2,3, and Se M4,5 edges (30-60 eV). After the broadband optical pump pulse, the XUV…