相关论文: Time-dependent coupled cluster theory for ultrafas…

We present an excited-state-specific coupled-cluster approach in which both the molecular orbitals and cluster amplitudes are optimized for an individual excited state. The theory is formulated via a pseudoprojection of the traditional…

We assess the performance of different protocols for simulating excited-state X-ray absorption spectra. We consider three different protocols based on equation-of-motion coupled-cluster singles and doubles, two of them combined with the…

We introduce a model description of femtosecond laser induced desorption at surfaces. The substrate part of the system is taken into account as a (possibly semi-infinite) linear chain. Here, being especially interested in the early stages…

We describe an approach based on compressive-sampling which allows for a considerable reduction in the acquisition time in Fourier-transform spectroscopy. In this approach, an N-point Fourier spectrum is resolved from much less than N…

The transient response of an intrinsic graphene, which is caused by the ultrafast interband transitions, is studied theoretically for the range of pumping correspondent to the saturated absorption regime. Spectral and temporal dependencies…

Efficient simulation of the timing jitter in passively mode-locking lasers is key to their numerical investigation and optimization. We introduce a method based on the pulse-period fluctuation auto-correlation function and compare it…

We show that two-photon coherent control in a $V$-shape three-level system projects one-photon coherent transient in a simple two-level system. Higher order chirps of a shaped laser pulse play the roles of time and linear chirp in…

For the energy absorption of atomic clusters as a function of the laser pulse duration we find a similar behavior as it has been observed for metallic clusters [K\"oller et al., Phys. Rev. Lett. {\bf 82}, 3783 (1999)]. In both situations…

We employ ultra-broadband terahertz-midinfrared probe pulses to characterize the optical response of photoinduced charge-carrier plasmas in high-resistivity silicon in a reflection geometry, over a wide range of excitation densities…

Laser control of ultrafast double proton transfer is investigated for a two-dimensional model system describing stepwise and concerted transfer pathways. The pulse design has been done by employing optimal control theory in combination with…

We investigate ionization of neon atoms by an isolated attosecond pump pulse in the presence of two coherent extreme ultraviolet or x-ray probe fields. The probe fields are tuned to a core-valence transition in the residual ion and induce…

A new upscaling procedure that provides 1D representations of 2D mixing-limited reactive transport systems is developed and applied. A key complication with upscaled models in this setting is that the procedure must differentiate between…

We derive a time-dependent density functional theory appropriate for calculating the near-edge X-ray absorption spectrum in molecules and condensed matter. The basic assumption is to increase the space of many-body wave functions from one…

We present transient absorption spectra of an extreme ultraviolet attosecond pulse train in helium dressed by an 800 nm laser field with intensity ranging from $2\times10^{12}$ W/cm$^2$ to $2\times10^{14}$ W/cm$^2$. The energy range probed…

We investigate, through simulation, the evolution of polarization states during atmospheric propagation of high power, ultrashort laser pulses. A delayed rotational response model handling arbitrary, transverse polarization couples both the…

We calculated third order non-linear polarization to estimate the two-photon absorption of non-interacting two-level molecules in the transmission-type degenerate pump-probe geometry. The spectral intensity and the phase changes of the…

We report on a general method for the calculation of the frequency-dependent optical response of clusters based upon time-dependent density functional theory (TDDFT). The implementation is done using explicit propagation in the time domain…

The sensitivity of the displacement transducer pumped with a train of high-intensity laser pulses is estimated. Due to the multicomponent character of the pump a consideration of transformations of the signal and the noises between optical…

We investigate changes in the optical conductivity of doped Mott insulators by tuning ultrashort pump pulses to target either the Drude or low-energy absorption regions. Using a hole-doped two-leg Hubbard ladder and a four-leg t-J ladders,…

The problem of the one-exciton absorption spectrum is considered for the lattice of two-level interacting atoms whose initial energy splitting depends on the coordinate. It is shown that for some types of interatomic interaction, this…