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In conventional superconductors, bulk physical properties typically degrade as the film thickness approaches the two-dimensional (2D) limit. Here in the (111) oriented LaAlO3/KTaO3 (LAO/KTO) heterostructure, we demonstrate experimental…

We address the fundamental issue of growth of perovskite ultra-thin films under the condition of a strong polar mismatch at the heterointerface exemplified by the growth of a correlated metal LaNiO$_3$ on the band insulator SrTiO$_3$ along…

强关联电子 · 物理学 2014-12-23 S. Middey , P. Rivero , D. Meyers , M. Kareev , X. Liu , Y. Cao , J. W. Freeland , S. Barraza-Lopez , J. Chakhalian

The relative importance of atomic defects and electron transfer in explaining conductivity at the crystalline LaAlO3/SrTiO3 interface has been a topic of debate. Metallic interfaces with similar electronic properties produced by amorphous…

We present a multi-band model for superconductivity at the metallic interface between insulating oxides LaAlO$_3$ and SrTiO$_3$ (001). Using a self-consistent Bogoliubov-de Gennes theory, formulated with the realistic bands at the…

超导电性 · 物理学 2015-12-09 N. Mohanta , A. Taraphder

We report on a metal-insulator transition in the LaAlO3-SrTiO3 interface electron system, of which the carrier density is tuned by an electric gate field. Below a critical carrier density n_c ranging from 0.5-1.5 * 10^13/cm^2, LaAlO3-SrTiO3…

材料科学 · 物理学 2013-05-29 Y. C. Liao , T. Kopp , C. Richter , A. Rosch , J. Mannhart

Heteroepitaxial growth of transition-metal oxide films on the open (111) surface of SrTiO3 results in significant restructuring due to the polar mismatch. Monitoring the structural and composition on an atomic scale of LaNiO3/SrTiO3 (111)…

材料科学 · 物理学 2017-04-26 Mohammad Saghayezhian , Zhen Wang , Hangwen Guo , Yimei Zhu , E. W. Plummer , Jiandi Zhang

The electronic structure of interfaces between LaAlO$_3$ and SrTiO$_3$ is studied using local spin density approximation (LSDA) with intra-atomic Coulomb repulsion (LSDA+U). We find that the nature of the interface metallic states is…

强关联电子 · 物理学 2011-05-03 Natalia Pavlenko , Thilo Kopp

SrTiO$_3$ is a superconducting semiconductor with a pairing mechanism that is not well understood. SrTiO$_3$ undergoes a ferroelastic transition at $T=$ 105 K, leading to the formation of domains with boundaries that can couple to…

超导电性 · 物理学 2020-02-28 David Pekker , C. Stephen Hellberg , Jeremy Levy

We investigate the effect of oxygen vacancies and hydrogen dopants at the surface and inside slabs of LaAlO3, SrTiO3, and LaAlO3/SrTiO3 heterostructures on the electronic properties by means of electronic structure calculations as based on…

强关联电子 · 物理学 2019-05-03 I. I. Piyanzina , V. Eyert , Yu. V. Lysogorskiy , D. A. Tayurskii , T. Kopp

At the interface between complex insulating oxides, novel phases with interesting properties may occur, such as the metallic state reported in the LaAlO3/SrTiO3 system. While this state has been predicted and reported to be confined at the…

Ferroelectric and ferromagnetic orders rarely coexist, and magnetoelectric coupling is even more scarce. A possible avenue for combining these orders is by interface design, where orders formed at the constituent materials can overlap and…

强关联电子 · 物理学 2022-04-12 Gal Tuvia , Sapir Weitz Sobelman , Shay Sandik , Beena Kalisky , Yoram Dagan

The interface electronic structure of correlated LaTiO$_3$/SrTiO$_3$ superlattices is investigated by means of the charge self-consistent combination of the local density approximation (LDA) to density functional theory (DFT) with dynamical…

强关联电子 · 物理学 2013-06-07 Frank Lechermann , Lewin Boehnke , Daniel Grieger

Superlattices of correlated oxides have been used to explore interfacial effects and to achieve additional control over the physical properties of individual constituents. In this work, we present a first-principles perspective of the…

强关联电子 · 物理学 2024-02-02 V. A. M. Lima , M. C. O. Aguiar , N. C. Plumb , M. Radovic , W. H. Brito

LaCrO$_3$ (LCO) / SrTiO$_3$ (STO) heterojunctions are intriguing due to a polar discontinuity along (001), two distinct and controllable interface structures [(LaO)$^+$/(TiO$_2$)$^0$ and (SrO)$^0$/(CrO$_2$)$^-$], and interface-induced…

Emergent magnetic states at oxide interfaces arise from the interplay of charge transfer, orbital reconstruction, and dimensional confinement, offering a route to engineered correlated-electron behavior in nanoscale spintronic materials.…

We show that the growth of the heterostructure LaGaO3/SrTiO3 yields the formation of a highly conductive interface. Our samples were carefully analyzed by high resolution electron microscopy, in order to assess their crystal perfection and…

Ultrathin two-dimensional (2D) electronic systems at the interfaces of layered materials are highly desirable platforms for exploring of novel quantum phenomena and developing advanced device applications. Here, we investigate ultrathin…

介观与纳米尺度物理 · 物理学 2025-03-31 Zengxing Lu , Jiatai Feng , Xuan Zheng , You-guo Shi , Run-Wei Li , Carmine Autieri , Mario Cuoco , Milan Radovic , Zhiming Wang

We have measured photoemission spectra of two kinds of TiO$_2$-capped VO$_2$ thin films, namely, that with rutile-type TiO$_2$ (r-TiO$_2$/VO$_2$) and that with amorphous TiO$_2$ (a-TiO$_2$/VO$_2$) capping layers. Below the Metal-insulator…

强关联电子 · 物理学 2009-11-11 K. Maekawa , M. Takizawa , H. Wadati , T. Yoshida , A. Fujimori , H. Kumigashira , M. Oshima , Y. Muraoka , Y. Nagao , Z. Hiroi

We have made very thin films of LaAlO3 on TiO2 terminated SrTiO3 and have measured the properties of the resulting interface in various ways. Transport measurements show a maximum sheet carrier density of 1016 cm-2 and a mobility around 104…

Motivated by the puzzling report of the observation of a ferromagnetic insulating state in LaMnO$_3$/SrTiO$_3$ heterostructures, we calculate the electronic and magnetic state of LaMnO$_3$, coherently matched to a SrTiO$_3$ square substrate…

材料科学 · 物理学 2019-09-25 Hrishit Banerjee , Oleg Janson , Karsten Held , Tanusri Saha-Dasgupta