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Revealing the interactions binding electronic and lattice components of cooperative quantum order is central to sculpting new states of matter. This challenge is epitomized by the charge density wave material 1T-TiSe$_2$, where…

We present a constrained density functional perturbation theory scheme for the calculation of structural and harmonic vibrational properties of insulators in the presence of an excited and thermalized electron-hole plasma. The method is…

材料科学 · 物理学 2021-10-13 Giovanni Marini , Matteo Calandra

Ultrafast light pulses can modify the electronic properties of quantum materials by perturbing the underlying, intertwined degrees of freedom. In particular, iron-based superconductors exhibit a strong coupling among electronic nematic…

Ultrafast spectroscopy is an emerging technique with great promise in the study of quantum materials, as it makes it possible to track similarities and correlations that are not evident near equilibrium. Thus far, however, the way in which…

Exciting electrons in solids with intense light pulses offers the possibility of generating new states of matter through nonthermal means and controlling their macroscopic properties on femto- to picosecond timescales. One way to manipulate…

材料科学 · 物理学 2021-10-07 Alfred Zong , Anshul Kogar , Nuh Gedik

There is growing interest in using ultrafast light pulses to drive functional materials into nonequilibrium states with novel properties. The conventional wisdom is that above gap photoexcitation behaves similarly to raising the electronic…

The electronic and structural properties of a material are strongly determined by its symmetry. Changing the symmetry via a photoinduced phase transition offers new ways to manipulate material properties on ultrafast timescales. However, in…

强关联电子 · 物理学 2015-09-25 Simon Wall , Daniel Wegkamp , Laura Foglia , Joyeeta Nag , Richard F. Haglund , Julia Staehler , Martin Wolf

We investigate the optical response of an atomic Bose-Einstein condensate with a vortex lattice. We find that it is possible for the vortex lattice to act as a photonic crystal and create photonic band gaps, by enhancing the refractive…

其他凝聚态物理 · 物理学 2007-05-23 O. E. Mustecaplioglu , M. O. Oktel

We study the nonequilibrium dynamics of photoinduced phase transitions in charge ordered (CO) systems with a strong electron-lattice interaction and analyze the interplay between electrons, periodic lattice distortions, and a phonon thermal…

强关联电子 · 物理学 2018-03-22 Linghua Zhu , Tsezar F. Seman , Michel van Veenendaal , Keun Hyuk Ahn

The photoexcited state in superconducting metals and alloys was studied via pump-probe spectroscopy. A pulsed Ti:sapphire laser was used to create the non-equilibrium state and the far-infrared pulses of a synchrotron storage ring, to which…

The simultaneous condensation of electronic and structural degrees of freedom gives rise to new states of matter, including superconductivity and charge-density-wave formation. When exciting such a condensed system, it is commonly assumed…

Photoinduced non-thermal phase transitions are new paradigms of exotic non-equilibrium physics of strongly correlated materials. An ultrashort optical pulse can drive the system to a new order through complex microscopic interactions that…

The interplay among charge, spin and lattice degrees of freedom in solids gives rise to intriguing macroscopic quantum phenomena such as colossal magnetoresistance, multiferroicity and high-temperature superconductivity. Strong coupling or…

超导电性 · 物理学 2012-07-18 K. W. Kim , A. Pashkin , H. Schäfer , M. Beyer , M. Porer , T. Wolf , C. Bernhard , J. Demsar , R. Huber , A. Leitenstorfer

Complex materials encompassing different phases of matter can display new photoinduced metastable states differing from those attainable under equilibrium conditions. These states can be realized when energy is injected in the material…

We numerically investigate photo-responses of the charge ordered state upon stimuli of pulsed laser light, especially paying attention to the differences in the pulse width, whose shortness has been a key to experimentally realize large…

强关联电子 · 物理学 2023-03-31 Hitoshi Seo , Yasuhiro Tanaka

The ultrafast electronic structures of the charge density wave material 1T-TiSe$_2$ were investigated by high-resolution time- and angle-resolved photoemission spectroscopy. We found that the quasiparticle populations drove ultrafast…

We use a coherent Bragg diffraction method to impart an external momentum to ultracold bosonic atoms trapped in a one-dimensional optical lattice. This method is based on the application of a single light pulse, with conditions where…

量子气体 · 物理学 2015-05-27 Xinxing Liu , Xiaoji Zhou , Wei Zhang , Thibault Vogt , Bo Lu , Xuguang Yue , Xuzong Chen

In the prevalent picture of ultrafast structural phase transitions, the atomic motion occurs in a slowly varying potential energy surface determined adiabatically by the fast electrons. However, this ignores non-conservative forces caused…

We study the interaction of a Bose-Einstein condensate, which is confined in an optical lattice, with a largely detuned light field propagating through the condensate. If the condensate is in its ground state it acts as a periodic…

统计力学 · 物理学 2009-10-31 Karl-Peter Marzlin , Weiping Zhang

Non-equilibrium states generated by ultrafast laser pulses are characterized by specific phenomena that are not accessible in static measurements. Previous time- and angle-resolved photoemission spectroscopy (TARPES) studies on rare-earth…

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