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Quantum spin liquids are exotic quantum phases of matter that do not order even at zero temperature. While there are several toy models and simple Hamiltonians that could host a quantum spin liquid as their ground state, it is very rare to…

强关联电子 · 物理学 2020-09-02 A. Kshetrimayum , C. Balz , B. Lake , J. Eisert

The study of quantum spin-liquid states (QSL) with lattice dimension $>1$ has proven an enduring problem in solid state physics. Key candidate materials are the $S=\frac{1}{2}$ kagome magnets due to their ability to host quantum…

材料科学 · 物理学 2016-10-04 E Connolly , P Reeves , D Boldrin , A S Wills

The search for novel phases of matter is a central theme of modern physics, with some of the most intriguing examples provided by the spin liquids found in magnets with competing, or "frustrated" interactions. Ca$_{10}$Cr$_7$O$_{28}$, a…

强关联电子 · 物理学 2025-04-11 Rico Pohle , Han Yan , Nic Shannon

Kagome lattice decorated with S=1/2 spins is one of the most discussed ways to realize a quantum spin liquid. However, all previous material realizations of this model have suffered from additional complications, ranging from additional…

We report synthesis of polycrystalline samples of the recently discovered spin liquid material Ca$_{10}$Cr$_7$O$_{28}$ and present measurements of the ambient and high pressure magnetic susceptibility $\chi$ versus temperature $T$,…

强关联电子 · 物理学 2017-07-20 Ashiwini Balodhi , Yogesh Singh

Ca$_{10}$Cr$_7$O$_{28}$ is a novel spin-$1/2$ magnet exhibiting spin liquid behaviour which sets it apart from any previously studied model or material. However, understanding Ca$_{10}$Cr$_7$O$_{28}$ presents a significant challenge,…

强关联电子 · 物理学 2021-07-28 Rico Pohle , Han Yan , Nic Shannon

A spin liquid is a new state of matter with topological order where the spin moments continue to fluctuate coherently down to the lowest temperatures rather than develop static long-range magnetic order as found in conventional magnets. For…

The spin-$\frac{1}{2}$ kagome antiferromagnet is considered an ideal host for a quantum spin liquid ground state. We find that when the bonds of the kagome lattice are modulated with a periodic pattern, new quantum ground states emerge.…

The quantum spin liquid (QSL) is a highly entangled magnetic state characterized by the absence of static magnetism in its ground state. Instead, the spins fluctuate in a highly correlated way down to the lowest temperatures. The QSL is…

Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…

Quantum spin liquid (QSL) is a novel state of matter with exotic excitations and was theoretically predicted to be realized most possibly in an S=1/2 kagome antiferromagnet. Experimentally searching for the candidate materials is a big…

One of the key questions concerning frustrated lattices that has lately emerged is the role of disorder in inducing spin-liquid-like properties. In this context, the quantum kagome antiferromagnets YCu$_3$(OH)$_6$Cl$_3$, which has been…

Geometric frustration of magnetic ions can lead to a quantum spin liquid ground state where long range magnetic order is avoided despite strong exchange interactions. The physical realization of quantum spin liquids comprises a major…

强关联电子 · 物理学 2023-06-07 Alex Hallett , Catalina Avarvarei , John W. Harter

Recent experiments suggest a quantum spin liquid ground state in the material PbCuTe$_2$O$_6$, where $S=1/2$ moments are coupled by antiferromagnetic Heisenberg interactions into a three dimensional structure of corner sharing triangles…

强关联电子 · 物理学 2021-09-15 Li Ern Chern , Yong Baek Kim

A quantum spin liquid (QSL) is an exotic quantum state of matter characterized by fluctuating spins which may exhibit long-range entanglement. Among the possible host candidates for a QSL ground state, the $S$=1/2 kagome lattice…

Recently, a novel material with bilayer kagome lattice Ca$_{10}$Cr$_7$O$_{28}$ was proposed to be a gapless quantum spin liquid, due to the lack of long-range magnetic order and the observation of broad diffuse excitations. Here, we present…

强关联电子 · 物理学 2018-11-02 J. M. Ni , Q. Y. Liu , Y. J. Yu , E. J. Cheng , Y. Y. Huang , Z. Y. Liu , X. J. Wang , Y. Sui , S. Y. Li

We present an X-band and tunable high-frequency/high-field electron spin resonance (HF-ESR) study of single-crystalline Ca$_{10}$Cr$_{7}$O$_{28}$, which constitutes alternating antiferromagnetic and ferromagnetic kagome bilayers. At high…

Actively shought since the turn of the century, two-dimensional quantum spin liquids (QSLs) are exotic phases of matter where magnetic moments remain disordered even at extremely low temperatures. Despite ongoing searches, QSLs remain…

强关联电子 · 物理学 2015-07-22 Juan Carrasquilla , Zhihao Hao , Roger G. Melko

We present measurements on a series of materials, Li$_2$In$_{1-x}$Sc$_x$Mo$_3$O$_8$, that can be described as a 1/6th-filled breathing kagome lattice. Substituting Sc for In generates chemical pressure which alters the breathing parameter…

强关联电子 · 物理学 2018-06-06 A. Akbari-Sharbaf , R. Sinclair , A. Verrier , D. Ziat , H. D. Zhou , X. F. Sun , J. A. Quilliam

A quantum spin liquid (QSL) is a state of matter where unpaired electrons' spins in a solid are quantum entangled, but do not show magnetic order in the zero-temperature limit. Because such a state may be important to the microscopic origin…

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