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Two distinct ferromagnetic phases of LaMn$_{0.5}$Co$_{0.5}$O$_{3}$ having monoclinic structure with distinct physical properties have been studied. The ferromagnetic ordering temperature $\textit{T}_{c}$ is found to be different for both…

Ultrasound velocity measurements of magnesium chromite spinel MgCr$_2$O$_4$ reveal elastic anomalies in the paramagnetic phase that are characterized as due to geometrical frustration. The temperature dependence of the tetragonal shear…

强关联电子 · 物理学 2012-10-24 Tadataka Watanabe , Shin-Ichi Ishikawa , Haruki Suzuki , Yusuke Kousaka , Keisuke Tomiyasu

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

强关联电子 · 物理学 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

The low temperature lattice structure and magnetic properties of Co$_{2.75}$Fe$_{0.25}$O$_4$ ferrite have been investigated using experimental results from synchrotron x-ray diffraction (SXRD), dc magnetization, ac susceptibility, neutron…

强关联电子 · 物理学 2020-07-09 R. N. Bhowmik , Amit Kumar , A. K. Sinha , S. M. Yusuf

The origin of the cooperative Jahn-Teller distortion and orbital-order in LaMnO3 is central to the physics of the manganites. The question is complicated by the simultaneous presence of tetragonal and GdFeO3-type distortions and the strong…

强关联电子 · 物理学 2013-05-29 Eva Pavarini , Erik Koch

Neutron diffraction measurements on single crystals of Cr1-xVx (x=0, 0.02, 0.037) show that the ordering moment and the Neel temperature are continuously suppressed as x approaches 0.037, a proposed Quantum Critical Point (QCP). The wave…

强关联电子 · 物理学 2009-11-13 D. A. Sokolov , M. C. Aronson , R. Erwin , J. W. Lynn , M. D. Lumsden , S. E. Nagler

We present the results of neutron diffraction studies on polycrystals of a metallic kagome lattice, Tb3Ru4Al12, reported recently to undergo reentrant magnetism, with the onset of long range antiferromagnetic order below (TN=) 22 K and…

强关联电子 · 物理学 2019-02-20 Sudhindra Rayaprol , Andreas Hoser , Kartik K Iyer , Sanjay K Upadhyay , E. V. Sampathkumaran

Synchrotron diffraction as a function of temperature and pressure, specific heat, magnetic susceptibility and small-angle neutron scattering experiments have revealed an anomalous response of MnGe. Similar but less pronounced behavior has…

The atomic pair distribution function (PDF) technique is employed to probe the atomic local structural responses in naturally double layered manganites \lsmo in the doping range $0.54 \leq x \leq 0.80$. Our low temperature neutron powder…

强关联电子 · 物理学 2009-11-10 Xiangyun Qiu , Simon J. L. Billinge , Carmen R. Kmety , John F. Mitchell

We present here a neutron diffraction study, both in zero field and as a function of magnetic field, of the magnetic structure of the tetragonal intermetallic \eun\ on a single crystalline sample. This material is known to undergo a cascade…

强关联电子 · 物理学 2016-06-29 X. Fabreges , A. Gukasov , P. Bonville , A. Maurya , A. Thamizhavel , S. K. Dhar

We present powder and single crystal X-ray diffraction data as evidence for a monoclinic distortion in the low spin (S=0) and intermediate spin state (S=1) of LaCoO3. The alternation of short and long bonds in the ab plane indicates the…

强关联电子 · 物理学 2009-11-10 G. Maris , Y. Ren , V. Volotchaev , C. Zobel , T. Lorenz , T. T. M. Palstra

A C$_3$-symmetric crystal-field potential in the Fe(II)Fe(III) bimetallic oxalates splits the L=2 Fe(II) multiplet into two doublets and a singlet. In compounds that exhibit magnetic compensation, one of the doublets was predicted to lie…

其他凝聚态物理 · 物理学 2009-11-13 Randy S. Fishman , Satoshi Okamoto , Fernando A. Reboredo

The existence of exchange-coupled Ni$^{2+}$ ions -- the so-called magnetic dimers -- in wolframite-type NiWO$_4$ and Zn$_c$Ni$_{1-c}$WO$_4$ solid solutions with high nickel content was discovered by X-ray absorption spectroscopy combined…

材料科学 · 物理学 2021-08-09 G. Bakradze , A. Kalinko , A. Kuzmin

We report the magnetic properties of $A$-site spinel compound MnSc$_2$Se$_4$. The macroscopic magnetic measurements uncovers successive magnetic transitions at $T_{\rm{N1}}$= 2.04 K, followed by two further transitions at $T_{\rm{N2}}$=1.8…

强关联电子 · 物理学 2022-06-01 K. Guratinder , V. Tsurkan , L. Prodan , L. Keller , J. P. Embs , F. Juranyi , M. Medarde , Ch. Rüegg , O. Zaharko

We present a neutron triple-axis and resonant spin-echo spectroscopy study of the spin correlations in untwinned YBCO crystals with x= 0.3, 0.35, and 0.45 as a function of temperature and magnetic field. As the temperature T approaches 0,…

强关联电子 · 物理学 2015-05-19 D. Haug , V. Hinkov , Y. Sidis , P. Bourges , N. B. Christensen , A. Ivanov , T. Keller , C. T. Lin , B. Keimer

NaNiO$_2$ is a Ni$^{3+}$-containing layered material consisting of alternating triangular networks of Ni and Na cations, separated by octahedrally-coordinated O anions. At ambient pressure, it features a collinear Jahn--Teller distortion…

Using elastic and inelastic neutron scattering, we investigated the evolution of the local atomic structure and lattice dynamics of La(1-x)Sr(x)CoO3 (x=0-0.5) as it crosses over with x from an insulator to a ferromagnetic metal (FMM). Our…

强关联电子 · 物理学 2007-05-23 Despina Louca , J. L. Sarrao

The Jahn-Teller effect is a fascinating and ubiquitous phenomenon in modern quantum physics and chemistry. We propose a class of oxides with melilite structure Ba$_2$TGe$_2$O$_7$ (T=V,Ni) where Jahn-Teller distortions are the main…

材料科学 · 物理学 2015-08-03 Paolo Barone , Kunihiko Yamauchi , Silvia Picozzi

The atomic pair distribution function (PDF) of stoichiometric LaMnO_3 has been measured. This has been fit with a structural model to extract the local Jahn-Teller distortion for an ideal Mn(3+)O_6 octahedron. These results are compared to…

材料科学 · 物理学 2009-10-31 Th. Proffen , R. G. DiFrancesco , S. J. L. Billinge , E. L. Brosha , G. H. Kwei

Noncollinear metallic antiferromagnets, with their rapid spin dynamics, efficient spin transport, and distinctive spin textures, play a pivotal role in advancing the field of spintronics. In this study, we report a comprehensive…