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We theoretically investigate electrostatic properties between two charged surfaces with a grafted polyelectrolyte layer in an aqueous electrolyte solution by using the Poisson-Boltzmann approach accounting for ion partitioning. In order to…

软凝聚态物质 · 物理学 2022-02-07 Jun-Sik Sin

We study the electrophoretic flow of suspensions of charged colloids with a mesoscopic method that allows to model generic experimental conditions. We show that for highly charged colloids their electrophoretic mobility increases…

软凝聚态物质 · 物理学 2015-05-28 Giovanni Giupponi , Ignacio Pagonabarraga

Water and water-mediated interactions determine thermodynamic and kinetics of protein folding, protein aggregation and self-assembly in confined spaces. To obtain insights into the role of water in the context of folding problems, we…

软凝聚态物质 · 物理学 2015-05-28 S. Vaitheeswaran , Jie Chen , D. Thirumalai

A small, bimetallic particle in a hydrogen peroxide solution can propel itself by means of an electrocatalytic reaction. The swimming is driven by a flux of ions around the particle. We model this process for the presence of a monovalent…

软凝聚态物质 · 物理学 2015-06-04 Benedikt Sabass , Udo Seifert

Capacity degradation and destructive hazards are two core challenges for lithium-ion batteries at high temperatures, which need to be solved urgently. Adding flame retardants or fire extinguishing agents can only achieve one-time…

高能物理 - 实验 · 物理学 2022-03-18 Yuewang Yang , Zhaowen Bai , Sijing Liu , Yinggang Zhu , Jiongzhi Zheng , Guohua Chen , Baoling Huang

We characterise the structural properties of the quasi-liquid layer (QLL) at two low-index ice surfaces in the presence of sodium chloride (Na$^+/$Cl$^-$) ions by molecular dynamics simulations. We find that the presence of a high surface…

化学物理 · 物理学 2022-09-28 Margaret L. Berrens , Fernanda C. Bononi , Davide Donadio

In this work, we present detailed measurements of the Casimir-Lifshitz force between two gold surfaces (a sphere and a plate) immersed in ethanol and study the effect of residual electrostatic forces, which are dominated by static fields…

量子物理 · 物理学 2009-11-13 J. N. Munday , Federico Capasso , V. Adrian Parsegian , Sergey M. Bezrukov

We experimentally observed the enhanced contact angle hysteresis (CAH) of dilute aqueous salt solution on graphite surface, i.e., 40.6$^\circ$, 34.6$^\circ$, and 27.8$^\circ$, for LiCl, NaCl, and KCl, indicating the effective tuning of the…

应用物理 · 物理学 2020-04-07 Haijun Yang , Yangjie Wang , Yingying Huang , Shuai Wang , Qiufeng Lü , Xiaoling Lei , Haiping Fang

Phase transitions in polar binary mixtures can be drastically altered even by a small amount of salt. This is because the preferential solvation strongly depends on the ambient composition. Together with a summary of our research in this…

软凝聚态物质 · 物理学 2015-05-20 Akira Onuki , Takeaki Araki , Ryuichi Okamoto

A theory is presented which allows us to accurately calculate the surface tensions and the surface potentials of electrolyte solutions. Both the ionic hydration and the polarizability are taken into account. We find a good correlation…

软凝聚态物质 · 物理学 2011-06-07 Alexandre P. dos Santos , Alexandre Diehl , Yan Levin

By reinforcing the interaction energy of the liquid with respect to the surface using total wetting boundary conditions, the response of liquids to mechanical shear stress is stronger and exhibits at sub-millimeter scale elastic properties.…

软凝聚态物质 · 物理学 2022-07-29 Eni Kume , Peter Dunne , Nicolas Martin , Patrick Baroni , Laurence Noirez

The effects of additions of low-molecular-mass salts on the properties of aqueous lysozyme solutions are examined by using the cloud-point temperature, $T_{cloud}$, measurements. Mixtures of protein, buffer, and simple salt in water are…

软凝聚态物质 · 物理学 2016-03-24 T. Janc , M. Kastelic , M. Boncina , V. Vlachy

By means of Monte Carlo computer simulations in the isothermal-isobaric ensemble, we investigated the interaction of a hydrophobic ligand with the hydrophobic surfaces of various curvatures (planar, convex and concave). A simple…

软凝聚态物质 · 物理学 2016-03-08 G. Mazovec , M. Lukšič , B. Hribar-Lee

We characterize the electrokinetic flow due to the transport of electrolytes embedded in nanochannels of varying cross-section with inhomogeneous slip on their walls, modeled as an effective slip length on the channel wall. We show that,…

流体动力学 · 物理学 2025-04-10 F. Carusela , J. Harting , P. Malgaretti

Capacitive deionization (CDI) is a technology in which water is desalinated by ion electrosorption into the electric double layers (EDLs) of charging porous electrodes. In recent years significant advances have been made in modeling the…

化学物理 · 物理学 2017-02-01 Amit N. Shocron , Matthew E. Suss

Surface effect of low-surface-tension contaminants accumulating at the evaporation surface can easily induce membrane wetting in the application of membrane distillation, especially in hypersaline scenarios. In this work, we propose a novel…

化学物理 · 物理学 2023-12-25 Yanni Ma , Zehua Yu , Xifan Fu , Zhi Huang , Tenghui Qiu , Na Zhao , Huidong Liu , Kang Liu

We discuss how the wettability of solid walls impacts electrokinetic properties, from large systems to a nanoscale. We show in particular how could the hydrophobic slippage, coupled to confinement effects, be exploited to induce novel…

软凝聚态物质 · 物理学 2023-10-19 Olga I. Vinogradova , Elena F. Silkina , Evgeny S. Asmolov

Polymer electrolytes are intensely investigated for use as solid electrolytes in next generation lithium-ion and lithium-metal batteries. However, little is known about the structural and dynamical properties of polymer electrolytes close…

软凝聚态物质 · 物理学 2021-12-02 Andreas Thum , Diddo Diddens , Andreas Heuer

Accurate tracking of the internal electrochemical states of lithium-ion battery during cycling enables advanced battery management systems to operate the battery safely and maintain high performance while minimizing battery degradation. To…

系统与控制 · 电气工程与系统科学 2020-10-01 Sravan Pannala , Puneet Valecha , Peyman Mohtat , Jason B. Siegel , Anna G. Stefanopoulou

The hydration of ions in nanoscale hydrated clusters is ubiquitous and essential in many physical and chemical processes. Here we show that the hydrolysis reaction is strongly affected by relative humidity. The hydrolysis of CO32- with n =…

原子与分子团簇 · 物理学 2017-02-13 Hang Xiao , Xiaoyang Shi , Yayun Zhang , Xiangbiao Liao , Feng Hao , Klaus S. Lackner , Xi Chen