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We use ultrafast optical spectroscopy to investigate the electronic and lattice dynamics of the charge-density wave (CDW) material 1$T$-TiSe$_2$ across various temperatures and pump fluences. We reveal a close relationship between the…

We investigate the ultrafast lattice dynamics in ${1T-TiSe_2}$ using femtosecond reflection pump-probe and pump-pump-probe techniques at room temperature. The time-domain signals and Fourier-transformed spectra show the $A_{1g}$ phonon mode…

材料科学 · 物理学 2023-06-12 Yu Mizukoshi , Takumi Fukuda , Yuta Komori , Ryo Ishikawa , Keiji Ueno , Muneaki Hase

High-resolution angle-resolved photoemission spectroscopy and ultrafast optical pump-probe spectroscopy were used to study semimetallic 1T - TiTe2 quasiparticle dispersion and dynamics. A kink and a flat band, having the same energy scale…

Time-domain femtosecond laser spectroscopic measurements of the ultrafast lattice dynamics in 2H-MoTe2 bulk crystals were carried out to understand the carrier-phonon interactions that govern electronic transport properties. An unusually…

Dirac semimetal PdTe2 single-crystal temperature-dependent ultrafast carrier and phonon dynamics were studied using ultrafast optical pump-probe spectroscopy. Two distinct carrier and coherent phonons relaxation processes were identified in…

Coherent phonon control using ultrashort pulse trains is the key to realizing structural phase transitions in solids by non-thermal pathways. By combining double-pulse excitation and time-resolved second harmonic generation techniques under…

材料科学 · 物理学 2025-10-09 Mizuki Akei , Takumi Fukuda , Yu Mizukoshi , Kazuhiro Kikuchi , Muneaki Hase

Femtosecond dynamics of coherent optical phonons in GeTe/Sb$_{2}$Te$_{3}$ superlattices (SLs), a new class of semiconductor SLs with three different states, have been investigated by using a reflection-type pump-probe technique at various…

材料科学 · 物理学 2015-03-23 Muneaki Hase , Yoshinobu Miyamoto , Junji Tominaga

The femtosecond optical pump-probe technique was used to study dynamics of photoexcited electrons and coherent optical phonons in transition metals Zn and Cd as a function of temperature and excitation level. The optical response in time…

强关联电子 · 物理学 2009-11-11 Muneaki Hase , Kunie Ishioka , Jure Demsar , Kiminori Ushida , Masahiro Kitajima

Layered transition metal dichalcogenides have attracted substantial attention owing to their versatile functionalities and compatibility with current nanofabrication technologies. Thus, noninvasive means to determine the mechanical…

We investigate ultrafast phonon dynamics in the Bi$_{1-x}$Sb$_{x}$ alloy system for various compositions $x$ using a reflective femtosecond pump-probe technique. The coherent optical phonons corresponding to the A$_{1g}$ local vibrational…

材料科学 · 物理学 2021-02-05 Yuta Komori , Yuta Saito , Paul Fons , Muneaki Hase

A coherent THz optical lattice mode is triggered by femtosecond laser pulses in the antiferromagnetic van der Waals semiconductor FePS$_3$. The 380 nm thick exfoliated flake was placed on a substrate and laser-driven lattice and spin…

Using femtosecond time-resolved X-ray diffraction, we investigated optically excited coherent acoustic phonons in the Weyl semimetal TaAs. The low symmetry of the (112) surface probed in our experiment enables the simultaneous excitation of…

We report high-resolution inelastic x-ray measurements of the soft phonon mode in the charge-density-wave compound TiSe$_2$. We observe a complete softening of a transverse optic phonon at the L point, i.e. q = (0.5, 0, 0.5), at T ~…

强关联电子 · 物理学 2015-05-28 F. Weber , S. Rosenkranz , J. -P. Castellan , R. Osborn , G. Karapetrov , R. Hott , R. Heid , K. -P. Bohnen , A. Alatas

Phonon dispersion in a two-dimensional electron-lattice system described by a two-dimensional square-lattice version of Su-Schrieffer-Heeger's model and having the half-filled electronic band is studied theoretically at temperatures higher…

软凝聚态物质 · 物理学 2009-11-10 Shutaro Chiba , Yoshiyuki Ono

Anharmonic decay of coherent optical phonons in semimetal Sb has been investigated by using a femtosecond pump-probe technique. The coherent $A_{1g}$ mode is observed in time domain in a wide temperature range of 7 - 290 K. The decay rate…

材料科学 · 物理学 2015-01-12 Muneaki Hase , Kiminori Ushida , Masahiro Kitajima

The selective excitation of coherent phonons provides unique capabilities to control fundamental properties of quantum materials on ultrafast time scales. For instance, in the presence of strong electron-phonon coupling, the electronic band…

材料科学 · 物理学 2020-06-02 P. Hein , S. Jauernik , H. Erk , L. Yang , Y. Qi , Y. Sun , C. Felser , M. Bauer

The coupling of the electron system to lattice vibrations and their time-dependent control and detection provides unique insight into the non-equilibrium physics of semiconductors. Here, we investigate the ultrafast transient response of…

Here, we investigate phonon mode- and electron band-selective electron-phonon couplings in centrosymmetric 1T$'$-MoTe$_2$ using time- and angle-resolved photoemission spectroscopy combined with frequency-domain analysis. Femtosecond…

材料科学 · 物理学 2026-02-24 Carl E. Jensen , Christoph Emeis , Stephan Jauernik , Petra Hein , Fabio Caruso , Michael Bauer

Here we report an ultrafast optical spectroscopic study of the nodal-line semimetal ZrSiTe. Our measurements reveal that, converse to other compounds of the family, the sudden injection of electronic excitations results in a strongly…

Information technology demands high-speed optoelectronic devices, but going beyond the one terahertz (THz) barrier is challenging due to the difficulties associated with generating, detecting, and processing high-frequency signals. Here, we…

介观与纳米尺度物理 · 物理学 2021-11-29 Ziqi Li , Bo Peng , Miao-Ling Lin , Yu-Chen Leng , Bin Zhang , Chi Pang , Ping-Heng Tan , Bartomeu Monserrat , Feng Chen
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