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Ultracold molecules trapped in optical tweezers show great promise for the implementation of quantum technologies and precision measurements. We study a prototypical scenario where two interacting polar molecules placed in separate traps…

We theoretically investigate the collisions between ultracold polar molecules in the presence of two lasers ensuring a Raman resonant transition on individual molecules to suppress photon scattering, taking the example of bosonic…

Spectroscopic measurements of the rotational distribution of $^{84}$Sr and $^{86}$Sr 5sns $^1S_0$ ultralong-range Rydberg molecular dimers created via photoassociation in a cold gas are reported. The dimers are produced by two-photon…

原子物理 · 物理学 2024-06-14 C. Wang , Y. Lu , S. K. Kanungo , F. B. Dunning , T. C. Killian , S. Yoshida

Two-photon intensity interferometry is shown to provide an accurate measurement of lifetime of quark-gluon plasma created in ultra-relativistic heavy ion collisions via the difference of outward and sidewardcorrelation radii. Under the…

高能物理 - 唯象学 · 物理学 2009-10-22 Dinesh K. Srivastava , Charles Gale

The main limitation of most ultracold chemistry studies to date is the lack of an analysis of reaction products. Here, we discuss the first generally tractable, rigorous theoretical framework for computing statistical product-state…

A recent experiment reported for the first time the preparation of a Fermi degenerate gas of polar molecules and observed a suppression of their chemical reaction rate compared to the one expected from a purely classical treatment. While it…

量子气体 · 物理学 2021-01-04 Peiru He , Thomas Bilitewski , Chris H. Greene , Ana Maria Rey

The K + KRb $\longrightarrow$ Rb + K$_{2}$ chemical reaction is the first ultracold atom-diatom chemical reaction for which experimental results have been reported for temperatures below 1 $\mu$K more than a decade ago. The reaction occurs…

化学物理 · 物理学 2025-06-03 H. da Silva , B. K. Kendrick , H. Li , S. Kotochigova , N. Balakrishnan

Chemical reaction networks in living cells maintain precise control over thousands of metabolites despite operating far from equilibrium under constant perturbations. While mass action kinetics accurately describe the underlying dynamics,…

最优化与控制 · 数学 2025-08-27 Steven Diamond

Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…

量子物理 · 物理学 2017-11-15 S. Kallush , J. L. Carini , P. L. Gould , R. Kosloff

Quantum coherent control of ultrafast bond making and the subsequent molecular dynamics is crucial for the realization of a new photochemistry, where a shaped laser field is actively driving the chemical system in a coherent way from the…

原子物理 · 物理学 2021-09-03 Liat Levin , Daniel M. Reich , Moran Geva , Ronnie Kosloff , Christiane P. Koch , Zohar Amitay

We study the formation of the RbCs molecule by an intense laser pulse using nonlinear dynamics. Under the Born-Oppenheimer approximation, the system is modeled by a two degree of freedom rovibrational Hamiltonian, which includes the ground…

混沌动力学 · 物理学 2017-04-05 Cristel Chandre , J Mahecha , J Salas

Ultracold polar molecules (UPMs) are emerging as a novel and powerful platform for fundamental applications in quantum science. Here, we report characterization of the coherence between nuclear spin levels of ultracold ground-state…

原子物理 · 物理学 2022-06-15 Junyu Lin , Junyu He , Mucan Jin , Guanghua Chen , Dajun Wang

Circular Rydberg states are ideal tools for quantum technologies, with huge mutual interactions and extremely long lifetimes in the tens of milliseconds range, two orders of magnitude larger than those of laser-accessible Rydberg states.…

原子物理 · 物理学 2023-01-25 Haiteng Wu , Rémi Richaud , Jean-Michel Raimond , Michel Brune , Sébastien Gleyzes

Many-body correlations govern a variety of important quantum phenomena such as the emergence of superconductivity and magnetism. Understanding quantum many-body systems is thus one of the central goals of modern sciences. Here we…

We propose a platform for observing and controlling the interactions between atomic ions and a quantum gas of polar molecules in the ultracold regime. This approach is based on the combination of several recently developed methods in two…

原子物理 · 物理学 2025-06-26 Leon Karpa , Olivier Dulieu

In ultrafast experiments with gas phase molecules, the alignment of the molecular axis relative to the polarization of the interacting laser pulses plays a crucial role in determining the dynamics following this light-matter interaction.…

化学物理 · 物理学 2025-04-14 Shashank Kumar , Eric Liu , Liang Z. Tan , Varun Makhija , Niranjan Shivaram

The exquisite properties of Rydberg levels make them particularly appealing for emerging quantum technologies. The lifetime of low-angular-momentum laser-accessible levels is however limited to a few $100\,\mu\mathrm{s}$ by optical…

Experiments in dense, ultracold gases of rubidium Rydberg atoms show a considerable decrease of the radiative excited state lifetimes compared to dilute gases. This accelerated decay is explained by collective and cooperative effects,…

量子物理 · 物理学 2007-05-23 Tun Wang , S. F. Yelin , R. Cote , E. E. Eyler , S. M. Farooqi , P. L. Gould , M. Kostrun , D. Tong , D. Vrinceanu

Coherent control of ultrafast molecule making from colliding reactants is crucial for realizing coherent control of binary photoreactions (CCBP). To handle diverse excitation scenarios, feasibility with both weak and strong fields is…

化学物理 · 物理学 2024-11-08 Moran Geva , Yonathan Langbeheim , Arie Landau , Zohar Amitay

A mechanism is considered for generating doorway states and intermediate structure in low-energy nuclear reactions as a result of collectivization of widths of unstable intrinsic states coupled to common decay channels. At the limit of…

核理论 · 物理学 2008-11-26 N. Auerbach , V. Zelevinsky