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相关论文: Broadband critical dynamics in disordered lead-bas…

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While methods based on density-functional perturbation theory have dramatically improved our understanding of electron-phonon contributions to transport in materials, methods for accurately capturing electron-electron scattering relevant to…

A$_{2}$BX$_{6}$ vacancy-ordered double perovskites (VODPs) have captured substantial research interest in the scientific community as they offer environmentally friendly and stable alternatives to lead halide perovskites. In this study, we…

材料科学 · 物理学 2024-11-11 Surajit Adhikari , Priya Johari

The magnetic structure and spin-wave excitations in the quasi-square-lattice layered perovskite compound La$_5$Mo$_4$O$_{16}$ were studied by a combination of neutron diffraction and inelastic neutron scattering techniques using…

Mixed-halide lead perovskites, with photoexcited charge-carrier properties suitable for high-efficiency photovoltaics, hold significant promise for high-efficiency tandem solar cells. However, phase segregation under illumination, where an…

Lead halide perovskite semiconductors are soft, polar, materials. The strong driving force for polaron formation (the dielectric electron-phonon coupling) is balanced by the light band effective-masses, leading to a strongly-interacting…

材料科学 · 物理学 2017-11-15 Jarvist Moore Frost

Low-dimensional organic-inorganic perovskites synergize the virtues of two unique classes of materials featuring intriguing possibilities for next-generation optoelectronics: they offer tailorable building blocks for atomically thin,…

Distinct shortcomings of individual halide perovskites for solar applications, such as restricted range of band gaps, propensity of ABX3 to decompose into AX+BX2, or oxidation of 2ABX3 into A2BX6 have led to the need to consider alloys of…

材料科学 · 物理学 2018-12-31 Gustavo M. Dalpian , Xingang Zhao , Lawrence Kazmerski , Alex Zunger

Lead-free vacancy-ordered perovskites (VOHPs) such as Cs2SnCl6 have emerged as promising materials for optoelectronic applications but typically suffer from wide band gaps and low photoluminescence quantum yields (PLQY). In this work, the…

材料科学 · 物理学 2025-12-19 Shruti Prasad , Pabitra Kumar Nayak , Dibyajyoti Ghosh

Active systems, from bacterial suspensions to cellular monolayers, are continuously driven out of equilibrium by local injection of energy from their constituent elements and exhibit turbulent-like and chaotic patterns. Here we demonstrate…

软凝聚态物质 · 物理学 2016-02-04 Amin Doostmohammadi , Michael F. Adamer , Sumesh P. Thampi , Julia M. Yeomans

The complex Fermi surfaces of transition-metal dichalcogenides (TMDCs) challenge the standard Peierls-instability-driven charge-density-wave (CDW) formation. Recently, evidence has been accumulating of a prominent role of ionic thermal…

强关联电子 · 物理学 2020-10-21 Daniel T. Payne , Paolo Barone , Lara Benfatto , Fulvio Parmigiani , Federico Cilento

We report on the exciton formation and relaxation dynamics following photocarrier injection in a single-layer two-dimensional lead-iodide perovskite. We probe the time evolution of four distinct exciton resonances by means of time-resolved…

Lead halide perovskites (LHPs) have emerged as an excellent class of semiconductors for next-generation solar cells and optoelectronic devices. Tailoring physical properties by fine-tuning the lattice structures has been explored in these…

We study the phase transition phenomena for long-range oriented percolation and contact process. We studied a contact process in which the range of each vertex are independent, updated dynamically and given by some distribution $N$. We also…

概率论 · 数学 2025-01-03 Pablo A. Gomes , Bernardo N. B. de Lima

We present the vibrational properties and phonon dispersion for quasi-2D hybrid organic-inorganic perovskites (BA)$_2$CsPb$_2$I$_7$, (HA)$_2$CsPb$_2$I$_7$, (BA)$_2$(MA)Pb$_2$I$_7$, and (HA)$_2$(MA)Pb$_2$I$_7$ calculated from first…

材料科学 · 物理学 2024-01-23 Emily Y. Chen , Bartomeu Monserrat

Coupled transitions between distinct ordered phases are important aspects behind the rich phase complexity of correlated oxides that hinders our understanding of the underlying phenomena. For this reason, fundamental control over complex…

强关联电子 · 物理学 2018-04-12 S. Middey , D. Meyers , M. Kareev , Y. Cao , X. Liu , P. Shafer , J. W. Freeland , J. W. Kim , P. J. Ryan , J. Chakhalian

Lead-halide perovskites exhibit remarkable efficiency in photovoltaics, driven by exceptionally long carrier diffusion lengths and recombination times. Paradoxically, this performance persists even in defect-rich, solution-grown samples.…

材料科学 · 物理学 2025-03-17 Dmytro Rak , Dusan Lorenc , Ayan A. Zhumekenov , Osman M. Bakr , Zhanybek Alpichshev

Optical nonlinearities are crucial for advanced photonic technologies since they allow photons to be managed by photons. Exciton-polaritons resulting from strong light-matter coupling are hybrid in nature: they combine small mass and high…

Hybrid organic-inorganic halide perovskites with the prototype material of CH$_{3}$NH$_{3}$PbI$_{3}$ have recently attracted intense interest as low-cost and high-performance photovoltaic absorbers. Despite the high power conversion…

材料科学 · 物理学 2017-05-30 Xin-Gang Zhao , Ji-Hui Yang , Yuhao Fu , Dongwen Yang , Qiaoling Xu , Liping Yu , Su-Huai Wei , Lijun Zhang

Femtosecond time-resolved x-ray diffraction is employed to study the dynamics of the periodic lattice distortion (PLD) associated with the charge-density-wave (CDW) in K0.3MoO3. Using a multi-pulse scheme we show the ability to extend the…

Halide perovskites, such as methylammonium lead bromide (MAPbBr$_3$), host tightly bound three-dimensional excitons which are robust at room temperature. Excellent optical properties of MAPbBr$_3$ allow for designing of optical single-mode…