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Monolayer transition metal dichalcogenide (TMDC) crystals, as direct-gap materials with unusually strong light-matter interaction, have attracted much recent attention. In contrast to the initial understanding, the minima of the conduction…

Monolayer transition metal dichalcogenides host tightly-bound excitons, which dominate their optoelectronic response even at room temperatures. Light beams are often used to study these materials with the polarization - often termed as the…

介观与纳米尺度物理 · 物理学 2024-03-01 Omadillo Abdurazakov , Chunqiang Li , Yun-Pil Shim

The possibility of almost linear tuning of the band gap and of the electrical and optical properties in monolayers (MLs) of semiconducting transition metal dichalcogenide (S-TMD) alloys opens up the way to fabricate materials with on-demand…

Transition metal dichalcogenide (TMD) monolayers are direct bandgap semiconductors that feature tightly bound excitons, strong spin-orbit coupling, and spin-valley degrees of freedom. Depending on the spin configuration of the electron-hole…

With the both spin and valley degrees of freedom, the low-lying excitonic spectra of photo-excited transition-metal dichalcogenide monolayers (TMDC-MLs) are featured by rich fine structures, comprising the intra-valley bright exciton states…

介观与纳米尺度物理 · 物理学 2019-04-10 Guan-Hao Peng , Ping-Yuan Lo , Wei-Hua Li , Yan-Chen Huang , Yan-Hong Chen , Chi-Hsuan Lee , Chih-Kai Yang , Shun-Jen Cheng

Two-dimensional transition metal dichalcogenides (TMDCs) have recently become attractive semiconductor materials for several optoelectronic applications, such as photodetection, light harvesting, phototransistors, light-emitting diodes, and…

光学 · 物理学 2018-07-04 Alex Krasnok , Sergey Lepeshov , Andrea Alú

High degree of valley polarization of optically active excitons in transition-metal dichalcogenide monolayers (TMD-MLs) is vital in valley-based photonic applications but known to be likely spoiled by the intrinsic electron-hole exchange…

介观与纳米尺度物理 · 物理学 2021-06-15 Ping-Yuan Lo , Guan-Hao Peng , Wei-Hua Li , Yi Yang , Shun-Jen Cheng

TMDCs have attracted a lot of attention in recent years due to their unique indirect to direct band gap transition from bulk to monolayer thickness. Strong confinement in the out-of-plane direction enhances the Coulomb potential between the…

Monolayer transition metal dichalcogenides, known for exhibiting strong excitonic resonances, constitute a very interesting and versatile platform for investigation of light-matter interactions. In this work we report on a strong coupling…

介观与纳米尺度物理 · 物理学 2019-05-20 M. Król , K. Lekenta , R. Mirek , K. Łempicka , D. Stephan , K. Nogajewski , M. R. Molas , A. Babiński , M. Potemski , J. Szczytko , B. Piętka

The dependence of the excitonic photoluminescence (PL) spectrum of monolayer transition metal dichalcogenides (TMDs) on the tilt angle of an applied magnetic field is studied. Starting from a four-band Hamiltonian we construct a theory…

介观与纳米尺度物理 · 物理学 2018-02-23 M. Van der Donck , M. Zarenia , F. M. Peeters

The intricate interplay between optically dark and bright excitons governs the light-matter interaction in transition metal dichalcogenide monolayers. We have performed a detailed investigation of the "spin-forbidden" dark excitons in WSe2…

Monolayers of transition metal dichalcogenides (TMDCs) have emerged as new optoelectronic materials in the two dimensional (2D) limit, exhibiting rich spin-valley interplays, tunable excitonic effects, and strong light-matter interactions.…

The polarization analysis of optical transitions in monolayer and bilayer transition-metal dichalcogenides provides invaluable information on the spin and valley (pseudospin) degrees of freedom. To explain optical properties of a given…

材料科学 · 物理学 2015-10-06 Hanan Dery , Yang Song

We present a comprehensive theoretical investigation of the photo-generated excitons in transition-metal dichalcogenide monolayers (TMD-ML's) by Laguerre-Gaussian beams, a celebrated kind of twisted lights (TL's) carrying quantized orbital…

介观与纳米尺度物理 · 物理学 2022-03-07 Guan-Hao Peng , Oscar Javier Gomez Sanchez , Wei-Hua Li , Ping-Yuan Lo , Shun-Jen Cheng

A monolayer of transition metal dichalcogenide (TMDC) is shown to be capable of supporting a guided optical mode below the exciton resonance, a two-dimensional exciton polariton. This visible or near IR mode is confined roughly within a…

光学 · 物理学 2015-05-05 Jacob B. Khurgin

Monolayers of semiconducting transition metal dichalcogenides are two-dimensional direct-gap systems which host tightly-bound excitons with an internal degree of freedom corresponding to the valley of the constituting carriers. Strong…

Monolayer transition metal dichalcogenides (TMDs) are the first truly two-dimensional (2D) semiconductor, providing an excellent platform to investigate light-matter interaction in the 2D limit. Apart from fundamental scientific…

Transition metal dichalcogenide monolayers are promising candidates for exploring new electronic and optical phenomena and for realizing atomically thin optoelectronic devices. They host tightly bound electron-hole pairs (excitons) that can…

The plasmon-mediated manipulation of light-matter interaction in two-dimensional atomically transition-metal dichalcogenides (TMDs) critically depends on the design of plasmonic nanostructures to achieve the maximum optical field in TMDs.…

光学 · 物理学 2021-12-07 Wei Li , Ming Xin , Wenze Lan , Qinghu Bai , Shuo Du , Gang Wang , Baoli Liu , Changzhi Gu

Monolayer transition metal dichalcogenides (TMDs) are direct gap semiconductors emerging promising applications in diverse optoelectronic devices. To improve performance, recent investigations have been systematically focused on the tuning…

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