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The discovery of 2-dimensional (2D) materials, such as CrI3, that retain magnetic ordering at monolayer thickness has resulted in a surge of research in 2D magnetism from both pure and applied perspectives. Here, we report a magneto-Raman…

The coupling between spin and charge degrees of freedom in a crystal imparts strong optical signatures on scattered electromagnetic waves. This has led to magneto-optical effects with a host of applications, from the sensitive detection of…

The challenge of controlling magnetism using electric fields raises fundamental questions and addresses technological needs such as low-dissipation magnetic memory. The recently reported two-dimensional (2D) magnets provide a new system for…

Since the celebrated discovery of graphene, the family of two-dimensional (2D) materials has grown to encompass a broad range of electronic properties. Recent additions include spin-valley coupled semiconductors, Ising superconductors that…

The recent discovery of 2D magnets has revealed various intriguing phenomena due to the coupling between spin and other degree of freedoms (such as helical photoluminescence, nonreciprocal SHG). Previous research on the spin-phonon coupling…

The recent discovery of ferromagnetism in 2D van der Waals (vdw) crystals has generated widespread interest, owing to their potential for fundamental and applied research. Advancing the understanding and applications of vdw magnets requires…

We apply the density-functional theory to study various phases (including non-magnetic (NM), anti-ferromagnetic (AFM), and ferromagnetic (FM)) in monolayer magnetic chromium triiodide (CrI$_3$), a recently fabricated 2D magnetic material.…

介观与纳米尺度物理 · 物理学 2018-10-17 Lucas Webster , Liangbo Liang , Jia-An Yan

The discovery of spontaneous magnetism in van der Waal (vdW) magnetic monolayers has opened up an unprecedented platform for investigating magnetism in purely two-dimensional systems. Recently, it has been shown that the magnetic properties…

介观与纳米尺度物理 · 物理学 2022-01-19 Eliot Heinrich , Xin Li , Benedetta Flebus

The first magnetic 2D material discovered, monolayer (ML) CrI$_3$, is particularly fascinating due to its ground state ferromagnetism. Yet, because monolayer materials are difficult to probe experimentally, much remains unresolved about ML…

We use a combination of polarized Raman spectroscopy experiment and model magnetism-phonon coupling calculations to study the rich magneto-Raman effect in the two-dimensional (2D) magnet $\mathrm{CrI_3}$. We reveal a novel…

Two-dimensional (2D) honeycomb ferromagnets, such as monolayer chromium-trihalides, are predicted to behave as topological magnon insulators - characterized by an insulating bulk and topologically protected edge states, giving rise to a…

介观与纳米尺度物理 · 物理学 2023-08-10 M. Soenen , M. V. Milosevic

The discovery of ferromagnetic order in monolayer 2D crystals has opened a new venue in the field of two dimensional (2D) materials. 2D magnets are not only interesting on their own, but their integration in van der Waals heterostructures…

介观与纳米尺度物理 · 物理学 2020-08-24 D. Soriano , M. I. Katsnelson , J. Fernández-Rossier

Magnon Chern insulators (MCIs) exhibit unique topological magnon band structures featuring chiral edge states. Direct observations of the topologically protected magnon edge states have long been pursued. Here, we report the spatially…

介观与纳米尺度物理 · 物理学 2024-10-25 Jihai Zhang , Meng-Han Zhang , Peigen Li , Zizhao Liu , Ye Tao , Hongkun Wang , Dao-Xin Yao , Donghui Guo , Dingyong Zhong

Magnons dominate the magnetic response of the recently discovered insulating ferromagnetic two dimensional crystals such as CrI$_3$. Because of the arrangement of the Cr spins in a honeycomb lattice, magnons in CrI$_3$ bear a strong…

介观与纳米尺度物理 · 物理学 2020-02-04 A. T. Costa , D. L. R. Santos , N. M. R. Peres , J. Fernández-Rossier

We conduct a comprehensive study of three different magnetic semiconductors, CrI$_3$, CrBr$_3$, and CrCl$_3$, by incorporating both few- and bi-layer samples in van der Waals tunnel junctions. We find that the interlayer magnetic ordering,…

The discovery of two-dimensional (2D) systems hosting intrinsic long-range magnetic order represents a seminal addition to the rich physical landscape of van der Waals (vdW) materials. CrI3 has emerged as perhaps the most salient example,…

Exploring new parameter regimes to realize and control novel phases of matter has been a main theme in modern condensed matter physics research. The recent discovery of 2D magnetism in nearly freestanding monolayer atomic crystals has…

Bulk chromium triiodide (CrI$_3$) has long been known as a layered van der Waals ferromagnet. However, its monolayer form was only recently isolated and confirmed to be a truly two-dimensional (2D) ferromagnet, providing a new platform for…

Monolayer chromium trihalides, the archetypal two dimensional (2D) magnetic materials, are readily suggested as a promising platform for high frequency magnonics. Here we detail the spin wave properties of monolayer CrBr$_3$ and CrI$_3$,…

The discovery of atomically thin two-dimensional (2D) magnetic semiconductors has triggered enormous research interest recently. In this work, we use first-principles many-body perturbation theory to study a prototypical 2D ferromagnetic…

材料科学 · 物理学 2022-02-01 Meng Wu , Zhenglu Li , Steven G. Louie
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