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Mono-deuterated methanol is thought to form during the prestellar core stage of star formation. Observed variations in the CH2DOH/CH3OD ratio suggest that its formation is strongly dependent on the surrounding cloud conditions. Thus, it is…

Water and methanol are key components of interstellar ices and gas in star- and planet-forming regions, but direct observations of water in low-mass protostars are challenging due to atmospheric absorption. We present high-resolution (R =…

(Abridged) Gas-phase complex organic molecules are commonly detected in the warm inner regions of protostellar envelopes. Recent models show that photochemistry in ices followed by desorption may explain the observed abundances. This study…

星系天体物理 · 物理学 2015-05-13 K. I. Oberg , R. T. Garrod , E. F. van Dishoeck , H. Linnartz

Despite the organic molecule inventory detected in Orion KL, acetaldehyde (CH3CHO) -- one of the most ubiquitous interstellar aldehydes -- has not been firmly identified with mm-wave interferometry. We analyze extensive ALMA archival…

Ethanethiol (C$_2$H$_5$SH), a molecule detected in the interstellar medium (ISM), indicates the rich chemistry involving sulfur atoms. However, its behavior at low temperatures remains elusive, particularly the reported transition from an…

During the formation of stars, the accretion of the surrounding material toward the central object is thought to undergo strong luminosity outbursts, followed by long periods of relative quiescence, even at the early stages of star…

星系天体物理 · 物理学 2016-04-20 Vianney Taquet , Eva Wirström , Steven B. Charnley

In dense clouds of the interstellar medium, dust grains are covered by ice mantles, dominated by H$_2$O. CO and CO$_2$ are common ice components observed in infrared spectra, while infrared inactive N$_2$ is expected to be present in the…

地球与行星天体物理 · 物理学 2019-03-29 H. Carrascosa , L. -C. Hsiao , N. -E. Sie , G. M. Muñoz Caro , Y. -J. Chen

The standard model of cosmic ray heating-induced desorption of interstellar ices is based on a continuous representation of the sporadic desorption of ice mantle components from classical (0.1 micron) dust grains. This has been re-evaluated…

太阳与恒星天体物理 · 物理学 2022-08-17 Jonathan M. C. Rawlings

Recently, the extremely sensitive torsion-rotation transitions in methanol have been used to set a tight constraint on a possible variation of the proton-to-electron mass ratio over cosmological time scales. In order to improve this…

We carry out Monte-Carlo simulation to study deuterium enrichment of interstellar grain mantles under various physical conditions. Based on the physical properties, various types of clouds are considered. We find that in diffuse cloud…

星系天体物理 · 物理学 2015-10-06 Ankan Das , Dipen Sahu , Liton Majumdar , Sandip K. Chakrabarti

Aims. We aim to investigate whether a multilayer ice model can be as successful as a bulk ice model in reproducing the observed abundances of various deuterated gas-phase species toward starless cores. Methods. We calculate abundances for…

星系天体物理 · 物理学 2016-06-08 O. Sipilä , P. Caselli , V. Taquet

Aims. We aim to improve a previous model for the prediction of column densities and deuterium fractions of non- and singly deuterated methanol. Thereby, we try to identify crucial chemical and physical parameters, for which the study of…

星系天体物理 · 物理学 2023-12-20 W. Riedel , O. Sipilä , E. Redaelli , P. Caselli , A. I. Vasyunin , F. Dulieu , N. Watanabe

The interplay between radiation chemistry and sublimation dynamics of condensed organic compounds on cold grains is fundamental to describe observed gas-phase and ice-phase molecular abundances in the ISM. Infrared measurements are…

Up to 90% of the chemical reactions during star formation occurs on ice surfaces, probably including the formation of complex organics. Only the most abundant ice species are however observed directly by infrared spectroscopy. This study…

太阳与恒星天体物理 · 物理学 2015-05-13 Karin I. Oberg , Sandrine Bottinelli , Ewine F. van Dishoeck

A magnetohydrodynamic model of a steady, transverse C-type shock in a dense molecular cloud is presented. A complete gas-grain chemical network is taken into account: the gas-phase chemistry, the adsorption of gas species on dust grains,…

星系天体物理 · 物理学 2018-06-12 A. V. Nesterenok

The aim of this study is to understand the chemical conditions of ices around embedded young stellar objects (YSOs) in the metal-poor Large Magellanic Cloud (LMC). We performed near-infrared (2.5-5 micron) spectroscopic observations toward…

太阳与恒星天体物理 · 物理学 2015-05-18 Takashi Shimonishi , Takashi Onaka , Daisuke Kato , Itsuki Sakon , Yoshifusa Ita , Akiko Kawamura , Hidehiro Kaneda

Acetic acid (CH3COOH) was detected in the gas toward interstellar clouds, hot cores, protostars and comets. Its formation in ice mantles was proposed and acetic acid awaits detection in the infrared spectra of the ice as most other COMs…

天体物理仪器与方法 · 物理学 2023-12-05 C. del Burgo Olivares , H. Carrascosa , B. Escribano , G. M. Muñoz Caro , R. Martín-Doménech

Context. Methane is among the main components of the ice mantles of insterstellar dust grains, where it is at the start of a rich solid-phase chemical network. Quantification of the photon-induced desorption yield of these frozen molecules…

We present the results of astrochemical modeling of complex organic molecules (COMs) in the ice and gas of the prestellar core L1544 with the recently updated MONACO rate equations-based model. The model includes, in particular,…

Gas-phase methanol was recently detected in a protoplanetary disk for the first time with ALMA. The peak abundance and distribution of methanol observed in TW Hya differed from that predicted by chemical models. Here, the chemistry of…

地球与行星天体物理 · 物理学 2018-09-12 Catherine Walsh , Shreyas Vissapragada , Harry McGee