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We apply the density-functional theory to study various phases (including non-magnetic (NM), anti-ferromagnetic (AFM), and ferromagnetic (FM)) in monolayer magnetic chromium triiodide (CrI$_3$), a recently fabricated 2D magnetic material.…

介观与纳米尺度物理 · 物理学 2018-10-17 Lucas Webster , Liangbo Liang , Jia-An Yan

Chromium triiodide, CrI$_3$, is emerging as a promising magnetic two-dimensional semiconductor where spins are ferromagnetically aligned within a single layer. Potential applications in spintronics arise from an antiferromagnetic ordering…

A monolayer of CrI$_3$ is a two-dimensional crystal that in its equilibrium configuration is a ferromagnetic semiconductor, however, two coupled layers can be ferromagnetic or antiferromagnetic depending on the stacking. We study the…

介观与纳米尺度物理 · 物理学 2020-04-07 Andrea Leon , J. W. González , J. Mejía-López , F. Crasto de Lima , E. Suárez Morell

In twisted two-dimensional (2D) magnets, the stacking dependence of the magnetic exchange interaction can lead to regions of ferromagnetic and antiferromagnetic interlayer order, separated by non-collinear, skyrmion-like spin textures.…

The marked interplay between the crystalline, electronic, and magnetic structure of atomically thin magnets has been regarded as the key feature for designing next-generation magneto-optoelectronic devices. In this respect, a detailed…

强关联电子 · 物理学 2020-05-25 Michele Pizzochero , Ravi Yadav , Oleg V. Yazyev

Few-layer CrI$_3$ is the most known example among two-dimensional (2D) ferromagnets, which have attracted growing interest in recent years. Despite considerable efforts and progress in understanding the properties of 2D magnets both from…

强关联电子 · 物理学 2021-01-14 I. V. Kashin , V. V. Mazurenko , M. I. Katsnelson , A. N. Rudenko

The recent discovery of ferromagnetic single-layer CrI3 creates ample opportunities for studying fundamental properties of atomically-thin magnets. By using first-principles calculations and model analysis, we show that a lateral strain…

介观与纳米尺度物理 · 物理学 2017-09-19 Fawei Zheng , Jize Zhao , Zheng Liu , Menglei Li , Mei Zhou , Shengbai Zhang , Ping Zhang

The discovery of 2-dimensional (2D) materials, such as CrI3, that retain magnetic ordering at monolayer thickness has resulted in a surge of research in 2D magnetism from both pure and applied perspectives. Here, we report a magneto-Raman…

Exploring new parameter regimes to realize and control novel phases of matter has been a main theme in modern condensed matter physics research. The recent discovery of 2D magnetism in nearly freestanding monolayer atomic crystals has…

The successful synthesis of few-layer CrI3 has opened new avenues for research in two-dimensional magnetic materials. Owing to its simple crystal structure and excellent physical properties, layered CrI3 has been extensively studied in…

材料科学 · 物理学 2026-01-09 Xianzhe Zhu , Pu Liu , Wence Ding , Benhu Zhou , Xiaoying Zhou , Guanghui Zhou

Since the celebrated discovery of graphene, the family of two-dimensional (2D) materials has grown to encompass a broad range of electronic properties. Recent additions include spin-valley coupled semiconductors, Ising superconductors that…

Changes in the spin configuration of atomically-thin, magnetic van-der-Waals multilayers can cause drastic modifications in their opto-electronic properties. Conversely, the opto-electronic response of these systems provides information…

介观与纳米尺度物理 · 物理学 2020-05-28 Zhe Wang , Marco Gibertini , Dumitru Dumcenco , Takashi Taniguchi , Kenji Watanabe , Enrico Giannini , Alberto F. Morpurgo

Intrinsic structural phase is a crucial foundation for the fundamental physical properties, and for creating innovative devices with unprecedented performances and unique functionalities. Long-range ferromagnetic orders of van der Waals…

The latest discovery of ferromagnetism in atomically thin films of semiconductors Cr$_2$Ge$_2$Te$_6$ and CrI$_3$ has unleashed numerous opportunities for fundamental physics of magnetism in two-dimensional (2D) limit and also for…

介观与纳米尺度物理 · 物理学 2019-05-09 Vijay Kumar Gudelli , Guang-Yu Guo

We conduct a comprehensive study of three different magnetic semiconductors, CrI$_3$, CrBr$_3$, and CrCl$_3$, by incorporating both few- and bi-layer samples in van der Waals tunnel junctions. We find that the interlayer magnetic ordering,…

We performed the detailed microscopic analysis of the inter-layer magnetic couplings for bilayer CrI$_3$. As the first step toward understanding the recent experimental observations and utilizing them for device applications, we estimated…

材料科学 · 物理学 2019-04-10 Seung Woo Jang , Min Yong Jeong , Hongkee Yoon , Siheon Ryee , Myung Joon Han

The exploration of magnetism in two-dimensional layered materials has attracted extensive research interest. For the monoclinic phase CrI3 with interlayer antiferromagnetism, finding a static and robust way of realizing the intrinsic…

材料科学 · 物理学 2022-11-30 Shiyang Sun , Xuyan Chen , Xuqi Li , Huihui Zhang , Haidan Sang , Shifei Qi , Zhenhua Qiao

Layered transition-metal compounds with controllable magnetic behaviors provide many fascinating opportunities for the fabrication of high-performance magneto-electric and spintronic devices. The tuning of their electronic and magnetic…

The first magnetic 2D material discovered, monolayer (ML) CrI$_3$, is particularly fascinating due to its ground state ferromagnetism. Yet, because monolayer materials are difficult to probe experimentally, much remains unresolved about ML…

We investigate the impact of mechanical strains and a perpendicular electric field on the electronic and magnetic ground-state properties of two-dimensional monolayer CrI$_3$ using density functional theory. We propose a minimal spin model…

材料科学 · 物理学 2020-09-23 Sahar Izadi Vishkayi , Zahra Torbatian , Alireza Qaiumzadeh , Reza Asgari
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