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In this paper we use layer potentials and asymptotic analysis techniques to analyze the heat generation due to nanoparticles when illuminated at their plasmonic resonance. We consider arbitrary-shaped particles and both single and multiple…

偏微分方程分析 · 数学 2017-03-02 Habib Ammari , Francisco Romero , Matias Ruiz

Ultrafast laser measurements probe the non-equilibrium dynamics of excited electrons in metals with increasing temporal resolution. Electronic structure calculations can provide a detailed microscopic understanding of hot electron dynamics,…

Localized plasmons formed in ultrathin metallic nanogaps can lead to robust absorption of incident light. Plasmonic metasurfaces based on this effect can efficiently generate energetic charge carriers, also known as hot electrons, owing to…

光学 · 物理学 2022-09-28 Larousse Khosravi Khorashad , Christos Argyropoulos

We study the thermal response of a single spherical metal nanoparticle to continuous wave illumination as a function of its size. We show that the particle temperature increases non-monotonically as the particle size increases, indicating…

光学 · 物理学 2020-01-08 Ieng-Wai Un , Yonatan Sivan

It is known that both linear and nonlinear optical phenomena can be produced when the plasmon in metallic nanostructures are excited by the external electromagnetic waves. In this work, a coupled system of Maxwell equations and a gas…

计算物理 · 物理学 2020-03-18 Maohui Lyu , Weng Cho Chew , Lijun Jiang , Maojun Li , Liwei Xu

Bulk gold is a good metal, i.e., conductor of electricity and heat, due to its delocalized electron density that can respond to extremely small external perturbations such as electric field or temperature gradient. In energy space, the…

原子与分子团簇 · 物理学 2018-09-13 Sami Malola , Sami Kaappa , Hannu Hakkinen

Atomistic simulations provide insights into structure-property relations on an atomic size and length scale, that are complementary to the macroscopic observables that can be obtained from experiments. Quantitative predictions, however, are…

材料科学 · 物理学 2021-04-14 Nataliya Lopanitsyna , Chiheb Ben Mahmoud , Michele Ceriotti

We investigate melting and undercooling in nanoscale (radius ~100 nm) gold particles that are levitated in a quadrupole ion (Paul) trap in a high vacuum environment. The particle is heated via laser illumination and probed using two main…

介观与纳米尺度物理 · 物理学 2022-01-27 Joyce Coppock , Quinn Waxter , Robert Wolle , B. E. Kane

Low-temperature scanning tunneling microscopy is used here to study dynamic bonding of gold atoms on surfaces under low coordination conditions. In the experiments, using an atomically-sharp gold tip, a gold adatom is deposited onto a gold…

材料科学 · 物理学 2022-10-05 W. Dednam , S. Tewari , E. B. Lombardi , J. J. Palacios , J. M. van Ruitenbeek , C. Sabater

We report on the application of a feedback-controlled electromigration technique for the formation of nanometer-sized gaps in mesoscopic gold wires and rings. The effect of current density and temperature, linked via Joule heating, on the…

介观与纳米尺度物理 · 物理学 2015-06-15 Birgit Kießig , Hilbert v. Löhneysen , Roland Schäfer

This paper describes an imaging microscopic technique based on heterodyne digital holography where subwavelength-sized gold colloids can be imaged in cell environment. Surface cellular receptors of 3T3 mouse fibroblasts are labeled with 40…

We introduce a many body theory for thermal far-field emission of dipolar dielectric and metallic nanoparticles in the vicinity of a substrate within the framework of fluctuational electrodynamics. Our theoretical model includes the…

光学 · 物理学 2022-05-23 Florian Herz , Svend-Age Biehs

Surface structure affects the growth, shape and properties of nanoparticles. In wet chemical syntheses, metal additives and surfactants are used to modify surfaces and guide nanocrystal growth. To understand this process, it is critical to…

Photoinduced hyperthermia is a cancer therapy technique that induces death to cancerous cells via heat generated by plasmonic nanoparticles. While previous studies have shown that some nanoparticles can be effective at killing cancer cells…

We propose a feedback strategy to track prescribed heat profiles using plasmonic nanoparticles as actuators. Starting from a thermo--plasmonic Maxwell--heat model, we use a time-domain discrete effective description in which the generated…

偏微分方程分析 · 数学 2026-02-17 Arpan Mukherjee , Sérgio S. Rodrigues , Mourad Sini

Multilayered metal-dielectric nanostructures display both strong plasmonic behavior and hyperbolic optical dispersion. The latter is responsible for the appearance of two separated radiative and non-radiative channels in the extinction…

We discuss finite-difference time-domain simulations of femtosecond pulses interacting with silver nanowires and nanoparticles. We show how localized hot spots near the metal surfaces can be generated and controlled in a spatiotemporal…

光学 · 物理学 2009-11-10 Tae-Woo Lee , Stephen K. Gray

The effect of the electron temperature on both the light absorption and the scattering by metal nanoparticles (MNs) with excitation of the surface plasmon electron vibrations is studied in the framework of the kinetic theory. The formulae…

介观与纳米尺度物理 · 物理学 2013-11-25 N. I. Grigorchuk

Electron emission spectra of gold nanoparticles (AuNPs) after photon interaction were measured over the energy range between 50 eV and 9500 eV to provide reference data for Monte Carlo radiation-transport simulations. Experiments were…

医学物理 · 物理学 2023-04-19 Hans Rabus , Philine Hepperle , Christoph Schlueter , Andrei Hloskovsky , Woon Yong Baek

The yield of electrons generated by gold nanoparticles due to irradiation by fast charged projectiles is estimated. The results of calculations are compared to those obtained for pure water medium. It is demonstrated that a significant…

原子与分子团簇 · 物理学 2016-10-07 Alexey V. Verkhovtsev , Andrei V. Korol , Andrey V. Solov'yov