相关论文: Raman Shifting induced by Cascaded Quadratic Nonli…
Terahertz nonlinear optics is a viable method to interrogate collective phenomena in quantum materials spanning ferroelectrics, charge-density waves, and superconductivity. In superconductors this includes the Higgs amplitude and Josephson…
Practical implementations of quantum information networks require frequency conversion of individual photons. Approaches based on a molecular gas as the nonlinear medium cover a wide range of the optical spectrum and promise high efficiency…
We report coherent association of atoms into a single weakly bound NaCs molecule in an optical tweezer through an optical Raman transition. The Raman technique uses a deeply bound electronic excited intermediate state to achieve a large…
High-quality micro-lasers are key ingredients in non-linear optics, communication, sensing and low-threshold solar-pumped lasers. However, such micro-lasers exhibit negligible absorption of free-space broadband pump light. Recently, this…
We present a temporally-multiplexed dual-colour terahertz (THz) imaging technique using THz-to-optical conversion in atomic vapour. By rapidly alternating the pump laser frequency, we sequentially excite two atomic states, each absorbing a…
A laser pulse composed of a fundamental and an appropriately phased second harmonic can drive a time-dependent current of photoionized electrons that generates broadband THz radiation. Over the propagation distances relevant to many…
We observe a terahertz radiation from a hydrogen-bonded organic molecular ferroelectric 5,6-dichloro-2-methylbenzimidazole excited by a femtosecond laser pulse at room temperature. The emitted terahertz wave consists of three oscillatory…
The Raman effect -- inelastic scattering of light by lattice vibrations (phonons) -- produces an optical response closely tied to a material's crystal structure. Here we show that resonant optical excitation of IR and Raman phonons gives…
Room temperature Terahertz stimulated emission and population inversion in optically pumped graphene is reported. We experimentally observe fast relaxation and relatively slow recombination dynamics of photogenerated electrons/holes in an…
We report the first coherent excitation of intramolecular vibrational modes via the nonlinear interaction of a TeraHertz (THz) light field with molecular liquids. A terahertz-terahertz-Raman pulse sequence prepares the coherences with a…
Plasma is capable of mediating the conversion of two pump photons into two different photons through a relativistic four-wave mixing nonlinearity. Spontaneously created photon pairs are emitted at symmetric angles with respect to the…
An optical transistor capable of simultaneous amplification and switching is theoretically proposed via cascaded second-order nonlinear interactions in a resonant structure. Two distinct operational schemes are analyzed. A single frequency…
We demonstrate the dynamics of stimulated Raman scattering in designed high-Q/Vm silicon photonic band gap nanocavities through the coupled-mode theory framework towards optically-pumped silicon lasing. The interplay of other chi(3) effects…
Using an example of a Raman active medium we describe how a common nonlinear process of four-wave mixing can be used to induce strong coupling between the spatial and temporal degrees of freedom in optical waves. This coupling produces…
We characterize the optical response of a three-level atom subjected to an incoherent pump and continuously illuminated with a weak, quasi-resonant probe field. To this end, we apply a wavefunction approach based on QED Hamiltonian…
High-energy terahertz pulses are challenging to produce due to the low conversion efficiency and limited optical damage threshold of nonlinear crystals. Here, we describe the high-efficiency generation of terahertz radiation pulses with…
Plasmonic metamaterials and metasurfaces offer new opportunities in developing high performance terahertz emitters and detectors beyond the limitations of conventional nonlinear materials. However, simple meta-atoms for second-order…
We report on terahertz (THz) radiation under electrical pumping from a degenerate semiconductor possessing an electron accumulation layer. In InN, the random grating formed by topographical defects provides high-efficiency coupling of…
Transduction of quantum signals between the microwave and the optical ranges will unlock powerful hybrid quantum systems enabling information processing with superconducting qubits and low-noise quantum networking through optical photons.…
Using optical technology for current injection and electromagnetic emission simplifies the comparison between materials. Here, we inject current into monolayer graphene and bulk gallium arsenide (GaAs) using two-color quantum interference…