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Medium and high entropy ceramics, with their distinctive disordered structures, exhibit ultra-low thermal conductivity and high temperature stability. These properties make them strong contenders for next generation thermal barrier coating…

材料科学 · 物理学 2024-05-27 Yuxuan Wang , Guoqiang Lan , Jun Song

Disorder enhances desired properties, as well as creating new avenues for synthesizing materials. For instance, hardness and yield stress are improved by solid-solution strengthening, a result of distortions and atomic size mismatches.…

Using fluorite oxides as an example, this study broadens high-entropy ceramics (HECs) to compositionally-complex ceramics (CCCs) or multi-principal cation ceramics (MPCCs) to include medium-entropy and/or non-equimolar compositions. Nine…

材料科学 · 物理学 2020-01-08 Andrew J. Wright , Qingyang Wang , Chuying Huang , Andy Nieto , Renkun Chen , Jian Luo

In this work, we show that above the glass transition there exists a strong unique interrelationship between the thermodynamic parameter of disorder of a metallic glass derived using its excess entropy, diffraction measure of disorder given…

无序系统与神经网络 · 物理学 2023-11-28 G. V. Afonin , A. S. Makarov , R. A. Konchakov , J. C. Qiao , A. N. Vasiliev , N. P. Kobelev , V. A. Khonik

The synthesis and characterization, along with the resulting properties, of fully dense \((\mathrm{Cr, Mo, Ta, V, W})\mathrm{C}\) high-entropy carbide ceramics were studied. The ceramics were synthesized from metal oxide and carbon powders…

High entropy carbides ceramics with randomly-distributed multiple principal cations have shown high temperature stability, low thermal conductivity, and possible radiation tolerance. While chemical disorder has been shown to suppress…

材料科学 · 物理学 2022-05-23 Cody A. Dennett , Zilong Hua , Eric Lang , Fei Wang , Bai Cui

Improved thermomechanical properties have been reported for various high-entropy oxides containing typically five metal cations. This study further investigates a series of duodenary (11 metals + oxygen) high-entropy oxides by mixing…

材料科学 · 物理学 2020-12-24 Andrew J. Wright , Qingyang Wang , Chongze Hu , Yi-Ting Yeh , Renkun Chen , Jian Luo

In the work, a modified effective medium theory is constructed for calculating the effective properties of thermoelectric composites with different values of percolation thresholds. It is shown that even at concentrations beyond the…

材料科学 · 物理学 2020-06-23 Snarskii Andrei , Yuskevich Pavel

Thermal behaviour of superconductors with complex order parameter symmetry is studied within a weak coupling theory. It is shown numerically, that the thermal nature of the different components of complex order parametrs are qualitatively…

超导电性 · 物理学 2016-08-31 Haranath Ghosh

The thermal conductivity of nanometric objects or nanostructured materials can be determined using non equilibrium molecular dynamics (NEMD) simulations. The technique is simple in its principle, and resembles a numerical guarded hot plate…

材料科学 · 物理学 2007-05-23 Patrice Chantrenne , Jean-Louis Barrat

The practically unlimited high-dimensional composition space of high-entropy materials (HEMs) has emerged as an exciting platform for functional materials design and discovery. However, the identification of stable and synthesizable HEMs…

材料科学 · 物理学 2024-03-01 Dibyendu Dey , Liangbo Liang , Liping Yu

Amorphous materials are also distinguished from crystals by their thermal properties. The structural disorder seems to be responsible both for a significant increase in heat capacity compared to crystals of the same composition, but also…

无序系统与神经网络 · 物理学 2023-07-28 Anne Tanguy

The thermal conductivity study on the pyrochlore structured ceramics is important for utilization of these materials as an inert matrix fuel, electrolytes for oxide fuel cell and thermal barrier coating. The impact of porosity, structural…

材料科学 · 物理学 2022-11-01 Yogendar Singh , Vivek Kumar , Saurabh Kumar Sharma , Pawan Kumar Kulriya

Thermal conductivity of a model glass-forming system in the liquid and glass states is studied using extensive numerical simulations. We show that near the glass transition temperture, where the structural relaxation time becomes very long,…

无序系统与神经网络 · 物理学 2020-02-26 Pranab Jyoti Bhuyan , Rituparno Mandal , Pinaki Chaudhuri , Abhishek Dhar , Chandan Dasgupta

High entropy oxides (HEOs) are a rapidly growing class of compositionally complex ceramics in which configurational disorder is engineered to unlock novel functionality. While average crystallographic symmetry is often retained, local…

Thermal expansion in materials can be accurately modeled with careful anharmonic phonon calculations within density functional theory. However, because of interest in controlling thermal expansion and the time consumed evaluating thermal…

材料科学 · 物理学 2017-11-03 Joseph T. Schick , Abhijith M. Gopakumar , Andrew M. Rappe

Silicon membranes patterned by nanometer-scale pillars standing on the surface provide a practical platform for thermal conductivity reduction by resonance hybridization. Using molecular simulations, we investigate the effect of nanopillar…

介观与纳米尺度物理 · 物理学 2021-09-01 Hossein Honarvar , Lina Yang , Mahmoud I. Hussein

Decreasing thermal conductivity is important for designing efficient thermoelectric devices. Traditional engineering strategies have focused on point defects and interface design. Recently, dislocations as line defects have emerged as a new…

The thermal conductivity of some orientational glasses of protonated C2H5OH and deuterated C2D5OD ethanol, cyclic substances (cyclohexanol C6H11OH, cyanocyclohexane C6H11CN, cyclohexene C6H10), and freon 112 (CFCl2)2 have been analyzed in…

无序系统与神经网络 · 物理学 2014-04-03 A. I. Krivchikov , G. A. Vdovychenko , O. A. Korolyuk , O. O. Romantsova

High entropy ceramics are highly promising as next generation thermal barrier coatings due to their unique disorder structure, which imparts ultra-low thermal conductivity and good high temperature stability. Unlike traditional ceramic…

材料科学 · 物理学 2023-11-15 Yuxuan Wang , Guoqiang Lan , Jun Song
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