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Molecules have vibrational, rotational, spin-orbit and hyperfine degrees of freedom or quantum states, each of which responds in a unique fashion to external electromagnetic radiation. The control over superpositions of these quantum states…

量子物理 · 物理学 2024-04-29 Svetlana Kotochigova , Qingze Guan , Eite Tiesinga , Vito Scarola , Brian DeMarco , Bryce Gadway

We report measurements of the ac polarizabilities of ultracold ground-state $^{23}\rm{Na}^{87}\rm{Rb}$ molecules. While the polarizability of the ground rotational state $J = 0$ is isotropic, that of the first excited rotational state $J =…

原子物理 · 物理学 2021-03-17 Junyu Lin , Junyu He , Xin Ye , Dajun Wang

We investigate magic-wavelength trapping of ultracold bialkali molecules in the vicinity of weak optical transitions from the vibrational ground state of the X$^1\Sigma^+$ potential to low-lying rovibrational states of the b$^3\Pi_0$…

量子物理 · 物理学 2021-04-14 Q. Guan , S. L. Cornish , S. Kotochigova

We demonstrate coherent microwave control of rotational and hyperfine states of trapped, ultracold, and chemically stable $^{23}$Na$^{40}$K molecules. Starting with all molecules in the absolute rovibrational and hyperfine ground state, we…

量子气体 · 物理学 2016-06-08 Sebastian A. Will , Jee Woo Park , Zoe Z. Yan , Huanqian Loh , Martin W. Zwierlein

We report on the optical polarizability of microwave-shielded ultracold NaCs molecules in an optical dipole trap. While dressing a pair of rotational states with a microwave field, we observe a marked dependence of the optical…

量子气体 · 物理学 2025-01-16 Siwei Zhang , Weijun Yuan , Niccolò Bigagli , Claire Warner , Ian Stevenson , Sebastian Will

We propose and analyze an electrostatic-optical nano-scale trap for cold diatomic polar molecules. The main ingredient of our proposal is an square-array of ferroelectric nano-rods {with alternating polarization}. We show that, in contrast…

量子气体 · 物理学 2018-02-21 Omjyoti Dutta , Geza Giedke

Extending the search for the magic wavelengths using the circularly polarized light in rubidium [Phys. Rev. A 86, 033416 (2012)], we pursue here to look for the magic wavelengths in the $ns-np_{1/2,3/2}$ transitions of Li, Na and K alkali…

原子物理 · 物理学 2015-06-12 B. K. Sahoo , Bindiya Arora

Detecting the internal state of polar molecules is a substantial challenge when standard techniques such as resonance-enhanced multi photon ionization (REMPI) or laser-induced fluorescense (LIF) do not work. As this is the case for most…

原子物理 · 物理学 2014-12-01 Rosa Glöckner , Alexander Prehn , Gerhard Rempe , Martin Zeppenfeld

Selection of "magic" trapping conditions with ultracold atoms or molecules, where pairs of internal states experience identical trapping potentials, brings substantial benefits to precision measurements and quantum computing schemes.…

量子物理 · 物理学 2011-01-04 Svetlana Kotochigova , David DeMille

Diatomic polar molecules are one of the most promising platforms of quantum computing due to their rich internal states and large electric dipole moments. Here, we propose entangling rotational states of adjacent polar molecules via a…

原子物理 · 物理学 2021-05-07 Eunmi Chae

We report the measurement of the anisotropic AC polarizability of ultracold polar $^{40}$K$^{87}$Rb molecules in the ground and first rotationally excited states. Theoretical analysis of the polarizability agrees well with experimental…

原子物理 · 物理学 2012-12-11 B. Neyenhuis , B. Yan , S. A. Moses , J. P. Covey , A. Chotia , A. Petrov , S. Kotochigova , J. Ye , D. S. Jin

Superpositions of rotational states in polar molecules induce strong, long-range dipolar interactions. Here we extend the rotational coherence by nearly one order of magnitude to 8.7(6) ms in a dilute gas of polar $^{23}$Na$^{40}$K…

The frequency dependent polarizabilities of the francium atom are calculated from the available data of energy levels and transition rates. Magic wavelengths for the state insensitive optical dipole trapping are identified from the…

原子物理 · 物理学 2016-04-12 U. Dammalapati , K. Harada , Y. Sakemi

Precise state-dependent control of optical potentials is of great importance for various applications utilizing cold neutral atoms. In particular, tune-out wavelengths for the clock state pair in alkaline-earth(-like) atoms provide…

量子气体 · 物理学 2026-01-08 Tim O. Höhn , René A. Villela , Er Zu , Leonardo Bezzo , Ronen M. Kroeze , Monika Aidelsburger

We present measurements of three distinctive state-(in)dependent wavelengths for the $^1\text{S}_{0}-^3\text{P}_{0}$ clock transition in $^{174}\text{Yb}$ atoms. Specifically, we determine two magic wavelengths at $652.281(21)\,$THz and…

Trapping ultracold molecules in conservative traps is essential for applications -- such as quantum state-controlled chemistry, quantum simulations, and quantum information processing. These applications require high densities or…

原子物理 · 物理学 2022-11-29 Juliana J. Park , Yu-Kun Lu , Alan O. Jamison , Wolfgang Ketterle

We theoretically investigate trapping conditions for ultracold polar molecules in optical lattices, when external magnetic and electric fields are simultaneously applied. Our results are based on an accurate electronic-structure calculation…

Dynamic polarizabilities of cesium Rydberg states, explicitly $nS_{1/2}$, $nP_{1/2}$, $nP_{3/2}$, $nD_{3/2}$, and $nD_{5/2}$, where the principal quantum number $n$ is $40$ to $70$, are presented for linearly polarized light. The dynamic…

原子物理 · 物理学 2024-06-04 A. Bhowmik , M. Gaudesius , G. Biedermann , D. Blume

Using first-principles calculations, we identify magic wavelengths for the 2s-2p and 2s-3p transitions in lithium. The ns and np atomic levels have the same ac Stark shifts at the corresponding magic wavelength, which facilitates…

原子物理 · 物理学 2015-06-05 M. S. Safronova , U. I. Safronova , Charles W. Clark

We demonstrate long rotational coherence of individual polar molecules in the motional ground state of an optical trap. In the present, previously unexplored regime, the rotational eigenstates of molecules are dominantly quantized by…

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