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A layered rhombohedral polymorph of indium (III) triiodide is synthesized at high pressure and temperature. The unit cell symmetry and approximate dimensions are determined by single crystal X-ray diffraction. Its R-3 crystal structure,…

材料科学 · 物理学 2023-11-09 Danrui Ni , Haozhe Wang , Xianghan Xu , Weiwei Xie , Robert J. Cava

Polyoxometalates (POMs) are unconventional electro-active molecules with a great potential for applications in molecular memories, providing efficient processing steps onto electrodes are available. The synthesis of the organic-inorganic…

We analyze in detail the possibility to use charge-dipole interaction between a single polar molecule or a 1D molecular array and a single Rydberg atom to read out rotational populations. The change in the Rydberg electron energy is…

量子物理 · 物理学 2016-10-05 Elena Kuznetsova , Seth T. Rittenhouse , H. R. Sadeghpour , Susanne F. Yelin

A high-frequency (95 GHz) EPR study is reported on single crystals of the planar tetranuclear complex Fe4(OCH3)6(dpm)6 (where Hdpm = dipivaloylmethane), which has been previously shown to present typical single-molecule magnet behaviour.…

介观与纳米尺度物理 · 物理学 2013-09-13 August Bouwen , Andrea Caneschi , Dante Gatteschi , Etienne Goovaerts , Dirk Schoemaker , Lorenzo Sorace , Mariana Stefan

We theoretically investigate the properties of highly polar diatomic molecules containing $^2S$-state transition-metal atoms. We calculate potential energy curves, permanent electric dipole moments, spectroscopic constants, and leading…

原子物理 · 物理学 2021-02-16 Michał Śmiałkowski , Michał Tomza

We investigate the structure and features of an ultralong-range triatomic Rydberg molecule formed by a Rb Rydberg atom and a KRb diatomic molecule. In our numerical description, we perform a realistic treatment of the internal rotational…

We report on a novel method for photo-association of strongly polar trilobite Rydberg molecules. This exotic ultralong-range dimer, consisting of a ground-state atom bound to the Rydberg electron via electron-neutral scattering, inherits…

We study a molecular dimer model that takes higher order interaction term as well as antisymmetric term into account. We mainly focus on the theoretical quantum properties that are of interest. We numerically diagonalize the system and…

介观与纳米尺度物理 · 物理学 2015-10-13 S. A. Owerre

Metallization and dissociation are key transformations in diatomic molecules at high densities particularly significant for modeling giant planets. Using X-ray absorption spectroscopy and atomistic modeling, we demonstrate that in halogens,…

Thermodynamic and muon spin-relaxation measurements have recently highlighted BiYbGeO$_5$ as a new example of a rare-earth-based quantum dimer magnet with isolated Yb$^{3+}$ spin-$\frac{1}{2}$ dimers. However, direct spectroscopic evidence…

强关联电子 · 物理学 2025-12-10 Rachit Kapoor , J. Ramirez Diaz , D. Yahne , V. O. Garlea , G. Hester

We present a novel binding mechanism where a neutral Rydberg atom and an atomic ion form a molecular bound state at large internuclear distance. The binding mechanism is based on Stark shifts and level crossings which are induced in the…

原子物理 · 物理学 2021-12-28 Markus Deiß , Shinsuke Haze , Johannes Hecker Denschlag

We investigate properties of ultralong-range polyatomic molecules formed with a Rb Rydberg atom and several ground-state atoms whose distance from the Rydberg atom is of the order of n^2a_0, where n is the principle quantum number of the…

原子物理 · 物理学 2007-05-23 Ivan C. H. Liu , Jan M. Rost

In this work we concentrate on the {\it point symmetry} of triangular triple quantum dot and its interplay with the {\it spin rotation symmetry} in the context of Kondo tunneling through this kind of artificial molecule. A fully symmetric…

强关联电子 · 物理学 2016-08-31 Tetyana Kuzmenko , Konstantin Kikoin , Yshai Avishai

We implement the impedance measurement technique (IMT) for characterization of interferometer-type superconducting qubits. In the framework of this method, the interferometer loop is inductively coupled to a high-quality tank circuit. We…

The 160Dy nucleus is classified as deformed nucleus (\beta=0.23) and has quite a complicated scheme of excited states. By now it has been quite well studied experimentally in nuclear reactions, Coulomb excitation, and \beta decays of 160Tb…

核理论 · 物理学 2009-09-29 V. P. Garistov , A. A Solnyshkin , J. Adam , V. G. Kalinnikov

Synthetic dimension platforms offer unique pathways for engineering quantum matter. We compute the phase diagram of a many-body system of ultracold atoms (or polar molecules) with a set of Rydberg states (or rotational states) as a…

We study isolated core excitation of ultra cold ytterbium Rydberg atoms of high orbital quantum number. Measurements were performed on the $6s_{1/2} 40l \rightarrow 6p_{1/2} 40l $ transition with $l=5-9$. The extracted energy shifts and…

原子物理 · 物理学 2021-02-17 Henri Lehec , Xin Hua , Pierre Pillet , Patrick Cheinet

We investigate the impact of an electric field on the structure of ultralong-range polar diatomic Rydberg molecules. Both the s-wave and p-wave interactions of the Rydberg electron and the neutral ground state atom are taken into account.…

原子物理 · 物理学 2015-06-15 Markus Kurz , Peter Schmelcher

We show that the resonant dipole-dipole interaction can give rise to bound states between two and three Rydberg atoms with non-overlapping electron clouds. The dimer and trimer states arise from avoided level crossings between states…

原子物理 · 物理学 2015-06-19 Martin Kiffner , Mingxia Huo , Wenhui Li , Dieter Jaksch

The largest non-cyclic molecules detected in the interstellar medium (ISM) are organic with a straight-chain carbon backbone. We report an interstellar detection of a branched alkyl molecule, iso-propyl cyanide (i-C3H7CN), with an abundance…

星系天体物理 · 物理学 2014-10-13 Arnaud Belloche , Robin T. Garrod , Holger S. P. Müller , Karl M. Menten