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The nitrogen-vacancy (N-V) center in diamond is promising as an electron spin qubit due to its long-lived coherence and optical addressability. The ground state is a spin triplet with two levels ($m_s = \pm 1$) degenerate at zero magnetic…

其他凝聚态物理 · 物理学 2007-10-15 T. P. Mayer Alegre , C. Santori , G. Medeiros-Ribeiro , R. G. Beausoleil

Initializing a set of qubits to a given quantum state is a basic prerequisite for the physical implementation of quantum-information protocols. Here, we discuss the polarization of the electronic and nuclear spin in a single nitrogen…

量子物理 · 物理学 2017-07-26 Tanmoy Chakraborty , Jingfu Zhang , Dieter Suter

Pulsed laser excitation causes the luminescence of Nitrogen Vacancy centers in diamond to unexpectedly decrease with increasing pulse energy. This decrease is observed in both the negatively charged and neutral centers and is caused by…

介观与纳米尺度物理 · 物理学 2017-12-22 Robert Chapman , Taras Plakhotnik

Nuclear spins nearby nitrogen-vacancy (NV) centers in diamond are excellent quantum memory for quantum computing and quantum sensing, but are difficult to be initialized due to their weak interactions with the environment. Here we propose…

量子物理 · 物理学 2019-09-04 Nanyang Xu , Yu Tian , Bing Chen , Jianpei Geng , Xiaoxiong He , Ya Wang , Jiangfeng Du

Initializing quantum registers with high fidelity is a fundamental precondition for many applications like quantum information processing and sensing. The electronic and nuclear spins of a Nitrogen-Vacancy (NV) center in diamond form an…

量子物理 · 物理学 2020-04-06 K. Rama Koteswara Rao , Yihua Wang , Zingfu Zhang , Dieter Suter

The ability to optically initialize the electronic spin of the nitrogen-vacancy (NV) center in diamond has long been considered a valuable resource to enhance the polarization of neighboring nuclei, but efficient polarization transfer to…

介观与纳米尺度物理 · 物理学 2018-08-01 F. Shagieva , S. Zaiser , P. Neumann , D. B. R. Dasari , R. Stöhr , A. Denisenko , R. Reuter , C. A. Meriles , J. Wrachtrup

We introduce an alternate route to dynamically polarize the nuclear spin host of nitrogen-vacancy (NV) centers in diamond. Our approach articulates optical, microwave and radio-frequency pulses to recursively transfer spin polarization from…

量子物理 · 物理学 2014-12-18 Daniela Pagliero , Abdelghani Laraoui , Jacob D. Henshaw , Carlos A. Meriles

A high-nitrogen-concentration diamond sample was subject to 200-keV electron irradiation using a transmission electron microscope. The optical and spin-resonance properties of the nitrogen-vacancy (NV) color centers were investigated as a…

量子物理 · 物理学 2012-08-10 Edwin Kim , Victor M. Acosta , Erik Bauch , Dmitry Budker , Philip R. Hemmer

NV-diamonds have attracted keen interest for nanoscale sensing and spin manipulation. In particular, the non-equilibrium electron spin polarization after optical excitation of single NV centers has successfully been transferred to nuclear…

介观与纳米尺度物理 · 物理学 2021-11-24 R. Rizzato , F. Bruckmaier , K. S. Liu , S. J. Glaser , D. B. Bucher

The novel aspect of the centre (NV-) in diamond is the high degree of spin polarisation achieved through optical illumination. In this paper it is shown that the spin polarisation occurs as a consequence of an electron-vibration interaction…

材料科学 · 物理学 2010-11-15 Neil Manson , Lachlan Rogers , Marcus Doherty , Lloyd Hollenberg

Nitrogen-vacancy centers possessing nuclear spins are promising candidates for a novel nuclear spin gyroscope. Preparation of a nuclear spin state is a crucial step to implement a sensor that utilizes a nuclear spin. In a low magnetic…

We present systematic measurements of longitudinal relaxation rates ($1/T_1$) of spin polarization in the ground state of the nitrogen-vacancy (NV$^-$) color center in synthetic diamond as a function of NV$^-$ concentration and magnetic…

量子物理 · 物理学 2015-12-17 A. Jarmola , A. Berzins , J. Smits , K. Smits , J. Prikulis , F. Gahbauer , R. Ferber , D. Erts , M. Auzinsh , D. Budker

We demonstrate optical spin polarization of the neutrally-charged silicon-vacancy defect in diamond ($\mathrm{SiV^{0}}$), an $S=1$ defect which emits with a zero-phonon line at 946 nm. The spin polarization is found to be most efficient…

The current work proposes a method for pulsed-light polarization of nitrogen-vacancy (NV) center electron spin. To evaluate the influence of pulsed spin polarization, we establish a polarization evaluation index based on polarizability and…

应用物理 · 物理学 2020-10-05 Zhang Jixing , Liu Tianzheng , Xu Lixia , Bian Guodong , Fan Pengcheng , Li Mingxin , Zhang Ning , Yuan Heng

After initial proof-of-principle demonstrations, optically pumped nitrogen-vacancy (NV) centres in diamond have been proposed as a non-invasive platform to achieve hyperpolarisation of nuclear spins in molecular samples over macroscopic…

介观与纳米尺度物理 · 物理学 2021-01-27 J. -P. Tetienne , L. T. Hall , A. J. Healey , G. A. L. White , M. -A. Sani , F. Separovic , L. C. L. Hollenberg

The study establishes that the degree of optically induced spin polarization that can be achieved for NV$^- $in 1b diamond is limited by the concentration of single substitutional nitrogen, N$^0$ . The polarization of the individual NV…

Ensembles of nitrogen-vacancy (NV) centers in diamond are versatile quantum sensors with broad applications in the physical and life sciences. The concentration of neutral substitutional nitrogen ([N$_\text{s}^0$]) strongly influences…

We propose and experimentally demonstrate a method to strongly increase the sensitivity of spin measurements on nitrogen-vacancy (NV) centers in diamond, which can be readily implemented in existing quantum sensing experiments. While charge…

One of the most remarkable properties of the nitrogen-vacancy (NV) center in diamond is that optical illumination initializes its electronic spin almost completely, a feature that can be exploited to polarize other spin species in their…

We studied the dynamic nuclear spin polarization of nitrogen in negatively charged nitrogen-vacancy (NV) centers in diamond both experimentally and theoretically over a wide range of magnetic fields from 0 to 1100 G covering both the…

量子物理 · 物理学 2021-01-04 Laima Busaite , Reinis Lazda , Andris Berzins , Marcis Auzinsh , Ruvin Ferber , Florian Gahbauer
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