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We study dynamical heterogeneity and glassy dynamics in a kinetically constrained lattice gas model which has both translational and rotational degrees of freedom. We find that the rotational diffusion constant tracks the structural…

软凝聚态物质 · 物理学 2015-06-25 Albert C. Pan

Little is known about the coupling of rotation and translation in dense systems. Here, we report results of confocal fluorescence microscopy where simultaneous recording of translational and rotational particle trajectories from a…

软凝聚态物质 · 物理学 2024-11-08 John Geiger , Niklas Grimm , Matthis Fuchs , Andreas Zumbusch

We explore the effect of directionality on rotational and translational relaxation in glassy systems of patchy particles. Using molecular dynamics simulations we analyze the impact of two distinct patch geometries, one that enhance local…

软凝聚态物质 · 物理学 2020-03-18 Susana Marín-Aguilar , Henricus H. Wensink , Giuseppe Foffi , Frank Smallenburg

Previous studies have suggested a conundrum in the relaxation dynamics of polydisperse supercooled liquids. It has been shown that in two dimensions, the relative relaxation times of particles of different sizes become more similar as the…

软凝聚态物质 · 物理学 2025-03-06 Ilian Pihlajamaa , Lotte van Gessel , Corentin Laudicina , Luc van Burik , Liesbeth Janssen

We use molecular dynamics computer simulations to investigate the coupling/decoupling between translational and rotational dynamics in a glass-forming liquid of dumbbells. This is done via a careful analysis of the $\alpha$-relaxation time…

软凝聚态物质 · 物理学 2009-11-13 Song-Ho Chong , Walter Kob

Translational dynamics of two-dimensional glass forming fluids is strongly influenced by soft, long-wavelength fluctuations first recognized by D. Mermin and H. Wagner. As a result of these fluctuations, characteristic features of glassy…

软凝聚态物质 · 物理学 2019-03-27 Elijah Flenner , Grzegorz Szamel

We perform molecular dynamics simulations using the extended simple point charge SPC/E water model in order to investigate the dynamical behavior of supercooled-stretched water. We focus on the behavior of the translational diffusion…

统计力学 · 物理学 2007-05-23 P. A. Netz , F. Starr , M. C. Barbosa , H. Eugene Stanley

We numerically study dynamical properties of the one-component Gaussian Core Model in the supercooled states. We find that nucleation is suppressed as density increases. Concomitantly the system exhibits glassy slow dynamics characterized…

软凝聚态物质 · 物理学 2015-05-19 Atsushi Ikeda , Kunimasa Miyazaki

Orientational relaxation (OR) in a viscous, glassy liquid is investigated by carrying out extensive NPT molecular dynamics simulations of isolated ellipsoids in a glass forming binary mixture. Near the glass transition, the OR occurs mainly…

软凝聚态物质 · 物理学 2016-08-31 S. Bhattacharyya , A. Mukherjee , B. Bagchi

We use X-ray tomography to investigate the translational and rotational dynamical heterogeneities of a three dimensional hard ellipsoids granular packing driven by oscillatory shear. We find that particles which translate quickly form…

无序系统与神经网络 · 物理学 2018-07-11 Binquan Kou , Yixin Cao , Jindong Li , Chengjie Xia , Zhifeng Li , Haipeng Dong , Ang Zhang , Jie Zhang , Walter Kob , Yujie Wang

We study the dynamics of a one-dimensional fluid of orientable hard rectangles with a non-coarse-grained microscopic mechanism of facilitation. The length occupied by a rectangle depends on its orientation, which is coupled to an external…

无序系统与神经网络 · 物理学 2011-12-09 Jeferson J. Arenzon , Deepak Dhar , Ronald Dickman

We study the dynamics of monodisperse hard ellipsoids via a new event-driven molecular dynamics algorithm as a function of volume fraction $\phi$ and aspect ratio $X_0$. We evaluate the translational $D_{trans}$ and the rotational $D_{rot}$…

软凝聚态物质 · 物理学 2009-11-13 C. De Michele , R. Schilling , F. Sciortino

We present molecular dynamics simulations of the motion of a single rigid rod in a disordered static 2d-array of disk-like obstacles. Two different configurations have been used for the latter: A completely random one, and which thus has an…

软凝聚态物质 · 物理学 2009-11-11 Angel J. Moreno , Walter Kob

We observe the translational and rotational diffusion of dimer tracer particles in quasi-2D colloidal samples. The dimers are in dense samples of two different sizes of spherical colloidal particles, with the area fraction ${\phi}$ of the…

软凝聚态物质 · 物理学 2017-10-05 Skanda Vivek , Eric R. Weeks

Molecular dynamics simulations are performed to investigate heterogeneous dynamics in amorphous glassy materials under oscillatory shear strain. We consider three-dimensional binary Lennard-Jones mixture well below the glass transition…

软凝聚态物质 · 物理学 2013-05-10 Nikolai V. Priezjev

Structural relaxation in binary hard spherical particles has been shown recently to exhibit a wealth of remarkable features when size disparity or mixture's composition is varied. In this paper, we test whether or not similar dynamical…

软凝聚态物质 · 物理学 2014-12-03 Wen-Sheng Xu , Zhao-Yan Sun , Li-Jia An

We numerically study the equilibrium relaxation dynamics of a two-dimensional Mari-Kurchan glass model. The tree-like structure of particle interactions forbids both non-trivial structural motifs and the emergence of a complex free-energy…

无序系统与神经网络 · 物理学 2022-06-27 Yoshihiko Nishikawa , Atsushi Ikeda , Ludovic Berthier

Exploring structural order in disordered systems including liquids and glasses is an intriguing but challenging issue in condensed matter physics. Here we construct a new parameter based on the angular distribution function of particles and…

软凝聚态物质 · 物理学 2018-06-11 Xiunan Yang , Wei-Hua Wang , Ke Chen

We propose a dynamic Kerr effect experiment for the distinction between dynamic heterogeneous and homogeneous relaxation in glassy systems. The possibility of this distinction is due to the inherent nonlinearity of the Kerr effect signal.…

软凝聚态物质 · 物理学 2009-11-11 Uli Haeberle , Gregor Diezemann

Using Density Functional Theory we theoretically study the orientational properties of uniform phases of hard kites -- two isosceles triangles joined by their common base. Two approximations are used: Scaled Particle Theory, and a new…

软凝聚态物质 · 物理学 2020-11-25 Yuri Martínez-Ratón , Enrique Velasco
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