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In frustrated Ising magnets, classical spin liquids (CSLs) with macroscopic ground-state degeneracy can survive against conventional magnetic order, as exemplified by systems on triangular, kagome and pyrochlore lattices at zero field. Here…

The search for quantum spin liquids (QSL) -- topological magnets with fractionalized excitations -- has been a central theme in condensed matter and materials physics. While theories are no longer in short supply, tracking down materials…

Three-dimensionally (3D) frustrated magnets generally exist in the magnetic diamond and pyrochlore lattices, in which quantum fluctuations suppress magnetic orders and generate highly entangled ground states (GS). LiYbSe2 in a previously…

A decade ago, Alexei Kitaev proposed an exactly solvable $S$ = 1/2 model on a two-dimensional honeycomb lattice, where the spins fractionalize into Majorana fermions and form a topological quantum spin liquid (QSL) in the ground state. It…

强关联电子 · 物理学 2022-01-21 Hidenori Takagi , Tomohiro Takayama , George Jackeli , Giniyat Khaliullin , Stephen E. Nagler

The most fascinating feature of certain two-dimensional (2D) gapless quantum spin liquid (QSL) is that their spinon excitations behave like the fermionic carriers of a paramagnetic metal. The spinon Fermi surface is then expected to produce…

强关联电子 · 物理学 2020-09-17 N. Li , Q. Huang , X. Y. Yue , W. J. Chu , Q. Chen , E. S. Choi , X. Zhao , H. D. Zhou , X. F. Sun

Actively shought since the turn of the century, two-dimensional quantum spin liquids (QSLs) are exotic phases of matter where magnetic moments remain disordered even at extremely low temperatures. Despite ongoing searches, QSLs remain…

强关联电子 · 物理学 2015-07-22 Juan Carrasquilla , Zhihao Hao , Roger G. Melko

Spin-1/2 kagome-lattice Heisenberg antiferromagnet is theoretically known to have a quantum spin liquid ground state, one of the frontiers of condensed matter physics. The search for the model substances has been continued for a long time,…

强关联电子 · 物理学 2024-08-21 Hidekazu Tanaka

The kagome Heisenberg antiferromagnet formed by frustrated spins arranged in a lattice of corner-sharing triangles is a prime candidate for hosting a quantum spin liquid (QSL) ground state consisting of entangled spin singlets. But the…

The two-dimensional (2D) spin-1/2 kagome Heisenberg antiferromagnet is believed to host quantum spin liquid (QSL) states with no magnetic order, but its ground state remains largely elusive. An important outstanding question concerns the…

强关联电子 · 物理学 2024-05-30 S. Suetsugu , T. Asaba , Y. Kasahara , Y. Kohsaka , K. Totsuka , B. Li , Y. Zhao , Y. Li , M. Tokunaga , Y. Matsuda

Recent experiments suggest a quantum spin liquid ground state in the material PbCuTe$_2$O$_6$, where $S=1/2$ moments are coupled by antiferromagnetic Heisenberg interactions into a three dimensional structure of corner sharing triangles…

强关联电子 · 物理学 2021-09-15 Li Ern Chern , Yong Baek Kim

Fifty years after Anderson's resonating valence-bond proposal, the spin-1/2 triangular-lattice Heisenberg antiferromagnet (TLHAF) remains the ultimate platform to explore highly entangled quantum spin states in proximity to magnetic order.…

We investigate the ground-state and the finite-temperature properties of the bond-random $s=1/2$ Heisenberg model on a square lattice with frustrating nearest- and next-nearest-neighbor antiferromagnetic interactions, $J_1$ and $J_2$, by…

强关联电子 · 物理学 2018-10-26 Kazuki Uematsu , Hikaru Kawamura

Triangular lattice antiferromagnets are prototypes for frustrated magnetism and may potentially realize novel quantum magnetic states such as a quantum spin liquid ground state. A recent work suggests NdTa$_7$O$_{19}$ with rare-earth…

We present a neutron diffraction study of NaYbO$_2$, a candidate quantum spin liquid compound hosting a geometrically frustrated triangular lattice of magnetic Yb$^{3+}$ ions. We observe diffuse magnetic scattering that persists to at least…

The ground state of the spin$-1/2$ kagome antiferromagnet remains uncertain despite decades of active research. Here we step aside from this debated question to address the ground-state nature of a related, and potentially just as rich,…

强关联电子 · 物理学 2019-12-11 Tristan Lugan , L. D. C Jaubert , Arnaud Ralko

We report gapless quantum spin liquid behavior in the layered triangular Sr$_{3}$CuSb$_{2}$O$_{9}$ (SCSO) system. X-ray diffraction shows superlattice reflections associated with atomic site ordering into triangular Cu planes well-separated…

Ba3IrTi2O9 crystallizes in a hexagonal structure consisting of a layered triangular arrangement of Ir4+ (Jeff=1/2). Magnetic susceptibility and heat capacity data show no magnetic ordering down to 0.35K inspite of a strong magnetic coupling…

强关联电子 · 物理学 2012-10-29 Tusharkanti Dey , A. V. Mahajan , P. Khuntia , M. Baenitz , B. Koteswararao , F. C. Chou

Recently several triangular-lattice magnets with delafossite structure have been found to display spin-liquid behavior down to the lowest temperatures. Remarkably, applying a magnetic field destroys the spin liquid which then gives way to…

强关联电子 · 物理学 2024-07-09 Santanu Dey , Joseph Maciejko , Matthias Vojta

The quantum antiferromagnet on the pyrochlore lattice offers an archetypal frustrated system, which potentially realizes a quantum spin liquid characterized by the absence of standard spontaneous symmetry breaking even at zero temperature,…

强关联电子 · 物理学 2023-11-21 Rico Pohle , Youhei Yamaji , Masatoshi Imada

Recently, a number of experiments indicate the possible presence of spin liquid phases in quantum magnets with spin-1/2 and spin-1 moments sitting on triangular-lattice-based structures in Ba3CuSb2O9 and Ba3NiSb2O9 respectively. In relation…

强关联电子 · 物理学 2013-06-04 Kyusung Hwang , Tyler Dodds , Subhro Bhattacharjee , Yong Baek Kim