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Harmonic generation provides an efficient tool for the study of ultrafast nonlinear dynamics. We report on time-resolved optical-pump terahertz-harmonic-generation spectroscopic investigation of ultrafast nonlinearity in a prototypical…

We report on terahertz high-harmonic generation in a Dirac semimetal as a function of the driving-pulse ellipticity and on a theoretical study of the field-driven intraband kinetics of massless Dirac fermions.Very efficient control of…

Engineered micro- or nano-structures based on nonlinear optical materials offer versatile opportunities for optoelectronic applications. While extensive efforts have been devoted to design tailored microcavities to promote and increase the…

We report strong terahertz (~10^12 Hz) high harmonic generation in thin films of Cd3As2, a three-dimensional Dirac semimetal at room temperature. The third harmonics is detectable with tabletop light source and can be as strong as 100 V/cm…

Two-dimensional (2D) materials with zero band gap exhibit remarkable electronic properties with wide tunability. High harmonic generation (HHG) in such materials offers unique platforms to develop novel optoelectronic devices at nanoscale,…

光学 · 物理学 2019-02-22 Rui Qin , Zi-Yu Chen

We explore anomalous high-harmonic generation in a model that realizes a transition from a broken time-reversal symmetry Weyl-semimetal to a semi-Dirac regime, i.e. a gapless semimetal with dispersion that is parabolic in one direction and…

介观与纳米尺度物理 · 物理学 2024-05-17 Luka Medic , Jernej Mravlje , Anton Ramšak , Tomaž Rejec

Frequency multiplication of terahertz signals on a solid state platform is highly sought-after for the next generation of high-speed electronics and the creation of frequency combs. Solutions to efficiently generate extreme harmonics (up to…

光学 · 物理学 2021-02-25 J. Lim , Y. S. Ang , F. J. G. de Abajó , I. Kaminer , L. K. Ang , L. J. Wong

In this paper, the nonlinear interaction of Weyl semimetal (WSM) with a strong driving electromagnetic wave-field is investigated. In the scope of the structure-gauge invariant low-energy nonlinear electrodynamic theory, the…

介观与纳米尺度物理 · 物理学 2022-06-22 H. K. Avetissian , V. N. Avetisyan , B. R. Avchyan , G. F. Mkrtchian

The generation of high-order harmonics in bulk solids subjected to intense ultrashort laser pulses has opened up new avenues for research in extreme nonlinear optics and light-matter interaction on sub-cycle timescales. Despite significant…

We investigate high-harmonic generation in closed systems, using the two-level atom as a simplified model. By means of a windowed Fourier transform of the time-dependent dipole acceleration, we extract the main contributions to this process…

原子物理 · 物理学 2007-05-23 C. Figueira de Morisson Faria , I Rotter

High-harmonic generation (HHG), the hallmark effect of attosecond science, is a nonperturbative nonlinear process leading to the emission of high-harmonic light from gases and solids. In gases, extreme driving laser pulse intensities can…

3D Dirac semimetals (DSMs) are promising materials for terahertz high harmonic generation (HHG). We show that 3D DSMs' high nonlinearity opens up a regime of nonlinear optics where extreme subwavelength current density features develop…

光学 · 物理学 2021-06-21 Jeremy Lim , Yee Sin Ang , Lay Kee Ang , Liang Jie Wong

Time-domain analysis of harmonic fields with sub-cycle resolution is now experimentally viable due to the emergence of sensitive, on-chip techniques for petahertz-scale optical-field sampling. We demonstrate how such a time-domain,…

Recent years have witnessed significant developments in the study of nonlinear properties of various optical materials at the nanoscale. However, in most cases experimental results on harmonic generation from nanostructured materials are…

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

强关联电子 · 物理学 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

High-harmonic generation in solids by intense laser pulses provides a fascinating platform for studying material properties and ultra-fast electron dynamics, where its coherent character is a central aspect. Using the semiconductor Bloch…

介观与纳米尺度物理 · 物理学 2026-01-22 Wolfgang Hogger , Alexander Riedel , Debadrito Roy , Angelika Knothe , Cosimo Gorini , Juan-Diego Urbina , Klaus Richter

We propose an analytical approach to high-harmonic generation (HHG) for nonperturbative low-frequency and high-intensity fields based on the (Jeffreys-)Wentzel-Kramers-Brillouin (WKB) approximation. By properly taking into account Stokes…

强关联电子 · 物理学 2022-01-05 Hidetoshi Taya , Masaru Hongo , Tatsuhiko N. Ikeda

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

We study high-order harmonic generation by optically driven one- and two-dimensional hydrogenlike atoms formed by Coulomb imurities in graphene. The time-dependent Dirac equations with Coulomb plus time-periodic monochromatic field…

介观与纳米尺度物理 · 物理学 2025-04-07 S. Rakhmanov , K. Matchonov , H. Yusupov , K. Nasriddinov , D. Matrasulov

Optical harmonic generation occurs when high intensity light ($>10^{10}$W/m$^{2}$) interacts with a nonlinear material. Electrical control of the nonlinear optical response enables applications such as gate-tunable switches and frequency…

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