相关论文: Laser-induced dynamics of molecules with strong nu…
An extended version of the antisymmetrized molecular dynamics to study structure of $p$-$sd$ shell hypernuclei is developed. By using an effective $\Lambda N$ interaction, we investigate energy curves of $^9_\Lambda$Be, $^{13}_\Lambda$C and…
The impact of nonadiabatic laser-induced molecular alignment on filamentation is numerically studied. Weak and strong field model of impulsive molecular alignment are compared in the context of nonlinear pulse propagation. It is shown that…
Recently it has been experimentally demonstrated that certain glasses display an unexpected magnetic field dependence of the dielectric constant. In particular, the echo technique experiments have shown that the echo amplitude depends on…
Rotation of molecules embedded in He nanodroplets is explored by a combination of fs laser-induced alignment experiments and angulon quasiparticle theory. We demonstrate that at low fluence of the fs alignment pulse, the molecule and its…
Nuclear magnetic resonance relaxometry represents a powerful tool for extracting dynamic information. Yet, obtaining links to molecular motion is challenging for many ions that relax through the quadrupolar mechanism, which is mediated by…
The strong coupling between intense laser fields and valence electrons in molecules causes a distortion of the potential energy hypersurfaces which determine the motion of nuclei in a molecule and influences possible reaction pathways. The…
The use of strong-field (i.e. intensities in excess of 10^13 Wcm-2) few-cycle ultrafast (durations of 10 femtoseconds or less) laser pulses to create, manipulate and image vibrational wavepackets is investigated. Quasi-classical modelling…
Strong magnetic fields have a large impact on the dynamics of molecules. In addition to the changes of the electronic structure, the nuclei are exposed to the Lorentz force with the magnetic field being screened by the electrons. In this…
A strong inhomogeneous static electric field is used to spatially disperse a rotationally cold supersonic beam of 2,6-difluoroiodobenzene molecules according to their rotational quantum state. The molecules in the lowest lying rotational…
Electric quadrupole (E2) matrix elements provide a measure of nuclear deformation and related collective structure. Ground-state quadrupole moments in particular are known to high precision in many p-shell nuclei. While the experimental…
We demonstrate experimentally a method of varying the degree of directionality in laser-induced molecular rotation. To control the ratio between the number of clockwise and counter-clockwise rotating molecules (with respect to a fixed…
Torque is ubiquitous in many molecular systems, including collisions, chemical reactions, vibrations, electronic excitations and especially rotor molecules. We present a straightforward theoretical method based on forces acting on atoms and…
Nuclei with a quadrupole deformation such as $^{177}$Hf have enhanced weak quadrupole moment which induces the tensor weak electron-nucleus interaction in atoms and molecules. Corresponding parity non-conserving (PNC) effect is strongly…
We introduce and experimentally demonstrate a method, where the two intrinsic time scales of a molecule, the slow nuclear motion and the fast electronic motion, are simultaneously measured in a photo-electron photo-ion coincidence…
Nuclei exhibit both single-particle and collective degrees of freedom, with the latter often subdivided into vibrational and rotational motions. Experimentally identifying the relative roles of these collective modes is extremely…
Most atomic nuclei exhibit ellipsoidal shapes characterized by quadrupole deformation $\beta_2$ and triaxiality $\gamma$, and sometimes even a pear-like octupole deformation $\beta_3$. The STAR experiment introduced a new…
The standard tunneling model describes quite satisfactorily the thermal properties of amorphous solids at temperatures $T<1K$ in terms of an ensemble of two-level systems possessing logarithmically uniform distribution over their tunneling…
Interaction of a strong laser pulse with matter transfers not only energy but also linear momentum of the photons. Recent experimental advances have made it possible to detect the small amount of linear momentum delivered to the…
Nuclei with spin $I \ge 1$ have a weak quadrupole moment which leads to tensor contribution to the parity non-conserving interaction between nuclei and electrons. We calculate this contribution for Yb$^+$, Fr and Ra$^+$ and found it to be…
Low-lying quadrupole shape dynamics is a typical manifestation of large amplitude collective motion in finite nuclei. To describe the dynamics on a microscopic foundation, we have formulated a consistent scheme in which the Bohr collective…