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One of the most striking manifestations of electronic properties of topological insulators is the dependence of the photocurrent direction on the helicity of circularly polarized optical excitation. The helicity dependent photocurrents,…

Chirality manifests across multiple scales, yielding unique phenomena that break mirror symmetry. In chiral materials, unexpectedly large spin-filtering or photogalvanic effects have been observed even in materials composed of light…

Chiral topological semimetals are materials that break both inversion and mirror symmetries. They host interesting phenomena such as the quantized circular photogalvanic effect (CPGE) and the chiral magnetic effect. In this work, we report…

Novel topological phases of matter are fruitful platforms for the discovery of unconventional electromagnetic phenomena. Higher-fold topology is one example, where the low-energy description goes beyond Standard Model analogs. Despite…

Chiral perovskites are emerging semiconducting materials with broken symmetry that can selectively absorb and emit circularly polarized light. However, most of the chiral perovskites are typically low-dimensional structures with limited…

Bulk photovoltaic effect is a non-linear response in noncentrosymmetric materials that converts light into DC current. In this work, we investigate the optical linear and non-linear responses in a chalcopyrite semiconductor ZnGeP$_2$. We…

材料科学 · 物理学 2024-10-15 Banasree Sadhukhan

The absence of mirror symmetry, or chirality, is behind striking natural phenomena found in systems as diverse as DNA and crystalline solids. A remarkable example occurs when chiral semimetals with topologically protected band degeneracies…

Higher-fold chiral fermions that go beyond two-fold Weyl fermions have recently been reported in crystalline systems. Here, we focus on such excitations in several binary, ternary and quaternary alloys/compounds with CoGe, BiSbPt and KMgBO3…

材料科学 · 物理学 2020-11-30 Chanchal K. Barman , Chiranjit Mondal , Sumiran Pujari , Biswarup Pathak , Aftab Alam

We studied the linear electro-optic effect of chiral topological semimetal RhSi which is characterized by high-fold chiral fermions separated in energy space. We identify that the general second order conductivity…

光学 · 物理学 2021-10-25 Zhi Li , Yuewen Gao , Yu Gu , Shengli Zhang , Toshiaki Iitaka , W. M. Liu

Topological semimetals in crystals with a chiral structure (which possess a handedness due to a lack of mirror and inversion symmetries) are expected to display numerous exotic physical phenomena, including fermionic excitations with large…

This paper presents a study of dc photocurrents in biased insulators to the third order in the electric field. We find three photocurrents which are characterized by physical divergences of the third-order free-electron polarization…

介观与纳米尺度物理 · 物理学 2019-08-07 Benjamin M. Fregoso

Two-dimensional ferroelectrics have recently emerged as a promising avenue for next-generation optoelectronic and photovoltaic devices. Due to the intrinsic absence of inversion symmetry, 2D ferroelectrics exhibit bulk photovoltaic effect…

材料科学 · 物理学 2025-12-08 Francesco Delodovici , Brahim Dkhil , Charles Paillard

Chiral multifold fermions in solids exhibit unique band structures and topological properties, making them ideal for exploring fundamental physical phenomena related to nontrivial topology, chirality, and symmetry breaking. However, the…

The nonlinear optical responses from topological semimetals are crucial in both understanding the fundamental properties of quantum materials and designing next-generation light-sensors or solar-cells. However, previous work was focusing on…

Chirality arises from the asymmetry of matters, where two counterparts are the mirror image of each other. The interaction between circular-polarization light and quantum materials is enhanced in chiral space groups due to the structural…

介观与纳米尺度物理 · 物理学 2023-09-13 Chang Niu , Shouyuan Huang , Neil Ghosh , Pukun Tan , Mingyi Wang , Wenzhuo Wu , Xianfan Xu , Peide D. Ye

Topological semimetals in chiral crystals, which possess both structural handedness and band crossings (or nodes) with topological chiral charge, exhibit many exotic physical properties. Here we demonstrate that the structural and…

介观与纳米尺度物理 · 物理学 2025-02-21 Mingxiang Pan , Hui Zeng , Erqing Wang , Huaqing Huang

In recent years, a type of topological semimetals (TSMs) that can host new fermions with high-fold degeneracy has attracted considerable interest. Among them, ones with chiral structrue particularly catch our attention. Such chiral…

材料科学 · 物理学 2024-04-29 Yan Wang , Xiaosong Bai , Wujun Shi , Wenjian Liu , Qiunan Xu

Chiral crystals are materials whose lattice structure has a well-defined handedness due to the lack of inversion, mirror, or other roto-inversion symmetries. These crystals represent a broad, important class of quantum materials; their…

So far, the circular photogalvanic effect (CPGE) is the only possible quantized signal in Weyl semimetals. With inversion and mirror symmetries broken, Weyl and multifold fermions in band structures with opposite chiralities can stay at…

材料科学 · 物理学 2020-10-07 Congcong Le , Yang Zhang , Claudia Felser , Yan Sun

The quantum behaviour of electrons in materials lays the foundation for modern electronic and information technology. Quantum materials with novel electronic and optical properties have been proposed as the next frontier, but much remains…

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