相关论文: Pulse dependence of prevalent pathways in xenon dr…
When atoms and molecules are irradiated by an x-ray free-electron laser (XFEL), they are highly ionized via a sequence of one-photon ionization and relaxation processes. To describe the ionization dynamics during XFEL pulses, a rate…
We study the interaction of a heteronuclear diatomic molecule, carbon monoxide, with a free-electron laser (FEL) pulse. We compute the ion yields and the intermediate states by which the ion yields are populated. We do so using rate…
A simple model for sequential multiphoton ionization by ultra-intense x-rays is presented. The derived scaling of the ion yield with pulse energy quantitatively reproduces the experimental data, which shows that the ion yield increases…
We explore the interactions between Argon and extreme ultraviolet (XUV) laser pulses across photon energies of 200 eV, 260 eV, and 315 eV, scrutinizing the influence of photon energy on Argon ion yields and unraveling the associated…
We investigate the interaction of Xe with isolated attosecond XUV pulses. Specifically, we calculate the ion yields and determine the pathways leading to the formation of ionic charged states up to Xe$^{5+}$. To do so, in our formulation we…
The dependency on the excitation energy of ultrafast multi-photon ionization of xenon by intense, short extreme ultraviolet pulses (XUV) was investigated in the vicinity of the 4$d$ 'giant' resonance using ion time-of-flight spectroscopy.…
We report on tunnel ionization of Xe by 2-cycle, intense, infrared laser pulses and its dependence on carrier-envelope-phase (CEP). At low values of optical field ($E$), the ionization yield is maximum for cos-like pulses with the…
Carrier envelope phase (CEP) stabilized 5 fs and 22 fs pulses of intense 800 nm light are used to probe the strong-field ionization dynamics of multielectron entities, xenon and carbon disulfide. We compare ion yields obtained with and…
Intense, ultrashort pulses of 800 nm laser light (12 fs, $\sim$4 optical cycles) of peak intensity 5$\times$10$^{14}$ W cm$^{-2}$ have been used to irradiate gas-phase Xe$_n$ clusters ($n$=500-25,000) so as to induce multiple ionization and…
Intense, 100 fs laser pulses at 3.2 and 3.6 um are used to generate, by multi-photon ionization, broadband wave packets with up to 400 eV of kinetic energy and charge states up to Xe+6. The multiple ionization pathways are well described by…
We have investigated multiphoton multiple ionization dynamics of argon and xenon atoms using a new x-ray free electron laser (XFEL) facility, SPring-8 Angstrom Compact free electron LAser (SACLA) in Japan, and identified that highly charged…
We have developed a Monte Carlo model for studying the local degradation of electrons in the energy range 9-10000 eV in xenon gas. Analytically fitted form of electron impact cross sections for elastic and various inelastic processes are…
The ionization of xenon atoms subjected to 42fs, 800nm pulses of radiation from a Ti:Sapphire laser was investigated. In our experiments a maximum laser intensity of $\sim2\times 10^{15} \textrm{W}/\textrm{cm}^2$ was used. Xenon ions were…
We present experimental results for the ionization of aniline and benzene molecules subjected to intense ultrashort laser pulses. Measured parent molecular ions yields were obtained using a recently developed technique capable of…
We present a theoretical framework to describe state-resolved ionization dynamics of neon atoms driven by ultraintense x-ray free-electron-laser pulses. In general, x-ray multiphoton ionization dynamics of atoms have been described by…
Strong-field ionization can induce electron motion in both the continuum and the valence shell of the parent ion. Here, we explore their interplay by studying laser-induced electron diffraction (LIED) patterns arising from interaction with…
We investigate the formation of multiple-core-hole states of molecular nitrogen interacting with a free-electron laser pulse. We obtain bound and continuum molecular orbitals in the single-center expansion scheme and use these orbitals to…
We analyze the photoelectron angular distribution in two-pathway interference between non\-resonant one-photon and resonant two-photon ionization of neon. We consider a bichromatic femtosecond XUV pulse whose fundamental frequency is tuned…
In a recent experiment at the VUV free-electron laser facility at DESY in Hamburg, the generation of multiply charged ions in a gas of atomic xenon was observed. This paper develops a theoretical description of multiphoton ionization of…
The multiphoton ionization rate of molecules depends on the alignment of the molecular axis with respect to the ionizing laser polarization. By studying molecular frame photo-electron angular distributions from N$_2$, O$_2$ and benzene, we…