相关论文: Modeling of Ex-Situ Dissolution for Geologic Seque…
Understanding the similarities and differences of the long term impact of different carbon dioxide removal (CDR) techniques is essential in determining the most effective and sustainable strategies to mitigate climate change. In particular,…
Electrochemical conversion of CO2 (CO2R) into fuels and chemicals can both reduce CO2 emissions and allow for clean manufacturing in the scenario of significant expansion of renewable power generation. However, large-scale process…
We present a computational study into the adsorption properties of CO$_2$ on amorphous and crystalline water surfaces under astrophysically relevant conditions. Water and carbon dioxide are two of the most dominant species in the icy…
We present design methods and insights for CO2 capture, transport, and storage systems for clusters of industrial facilities, with a case-study focus on the state of Louisiana. Our analytical framework includes: (1) evaluating the scale and…
Mineral dissolution in porous media coupled with single- or multi-phase flows is pervasive in natural and engineering systems including carbon capture and sequestration (CCS) and acid stimulation in reservoir engineering. Dissolution of…
To limit global warming to pre-industrial levels, global governments, industry and academia are taking aggressive efforts to reduce carbon emissions. The evaluation of anthropogenic carbon dioxide (CO$_2$) emissions, however, depends on the…
The chemistry of carbon in aqueous fluids at extreme pressure and temperature conditions is of great importance to Earth's deep carbon cycle, which substantially affects the carbon budget at Earth's surface and global climate change. At…
The electrochemical reduction of atmospheric CO$_2$ into high-energy molecules with renewable energy is a promising avenue for energy storage that can take advantage of existing infrastructure especially in areas where sustainable…
Climate change is a rapidly accelerating problem that requires fast and large-scale carbon sequestration to prevent catastrophe. This paper proposes a novel approach to use explosives for large-scale carbon sequestration. Combining the…
The conversion of CO2 into high-value chemicals through a photoreduction reaction in water is a promising route to reduce the dependence on fossil fuels. Ag nanoparticles can drive this reaction via localized surface plasmon resonance, but…
Carbon capture and storage (CCS) technology has been applied successfully in recent decades to reduce carbon emissions and alleviate global warming. In this regard, shale reservoirs present tremendous potential for carbon dioxide (CO2)…
Increasing anthropogenic carbon dioxide (CO$_2$) emissions have led to rising global temperatures and climate change. Using earth-abundant metal-oxide catalysts such as Cu$_2$O for reducing CO$_2$ through RWGS reaction seems lucrative. In…
Carbon nanoonions are novel carbon nanoestructures that have potential applications in fields like electronics and chemical catalysis. Here we report a very simple but effective method of purifying carbon nanoonions produced by submerged…
Addressing climate change calls for action to control CO$_2$ pollution. Direct air and ocean capture offer a solution to this challenge. Making carbon capture competitive with alternatives, such as forestation and mineralisation, requires…
We describe a new principle - the Alkalinity Concentration Swing (ACS) - for direct air capture of carbon dioxide driven by concentrating an alkaline solution that has been exposed to the atmosphere and loaded with dissolved inorganic…
Absorption lines from molecular hydrogen ($\rm H_2$) in the spectra of background sources are a powerful probe of the physical conditions in intervening cold neutral medium. At high redshift, $z>2$, $\rm H_2$ lines are conveniently shifted…
We extend an existing thermophysical activity model of comet 67P/Churyumov-Gerasimenko to include pressure buildup inside the pebbles making up the nucleus. We test various quantities of H$_{2}$O and CO$_{2}$, in order to simulate the…
Microbially induced calcite precipitation (MICP) is a technology for sealing leakage paths to ensure the safe storage of CO$_2$ in geological formations. In this work we introduce a numerical simulator of MICP for field-scale studies. This…
We study by kinetic Monte Carlo simulations the dynamic behavior of a Ziff-Gulari-Barshad (ZGB) model for the catalytic oxidation of CO on a surface. It is well known that the ZGB model presents a continuous transition between an oxygen…
The carbon capture, utilization, and storage (CCUS) framework is an essential component in reducing greenhouse gas emissions, with its success hinging on the comprehensive knowledge of subsurface geology and geomechanics. Passive seismic…