相关论文: Phenomenological Arrhenius Analyses in Plasmon-Enh…
The possibility of studying non-thermal electron energization in laser-driven plasma experiments of magnetic reconnection is studied using two- and three-dimensional particle-in-cell simulations. It is demonstrated that non-thermal…
Thermodynamic characteristics of the radiation of condensed combustion products presented in the form of agglomerates of metal-oxide nanoparticles demonstrate deviations from the classical Planck's law. We propose to interpret these…
Generation of energetic (hot) electrons is an intrinsic property of any plasmonic nanostructure under illumination. Simultaneously, a striking advantage of metal nanocrystals over semiconductors lies in their very large absorption cross…
Understanding the interplay between illumination and the electron distribution in metallic nanostructures is a crucial step towards developing applications such as plasmonic photo-catalysis for green fuels, nano-scale photo-detection and…
The use of nanoplasmonics to control light and heat close to the thermodynamic limit enables exciting opportunities in the field of plasmonic catalysis. The decay of plasmonic excitations creates highly nonequilibrium distributions of hot…
We solve the Maxwell and heat equations self-consistently for metal nanoparticles under intense continuous wave (CW) illumination. Unlike previous studies, we rely on {\em experimentally}-measured data for the metal permittivity for…
In this paper we discuss the field enhancement due to surface plasmons resonances of metallic nanostructures, in particular nano spheres on top of a metal, and find maximum field enhancement of the order of 10^2, intensities enhancement of…
Investigating nanoplasmonics using time-dependent approaches permits shedding light on the dynamic optical properties of plasmonic structures, which are intrinsically connected with their potential applications in photochemistry and…
Catalytically active enzymes have recently been observed to exhibit enhanced diffusion. In a recent work [C. Riedel et al., Nature 517, 227 (2015)], it has been suggested that this phenomenon is correlated with the degree of exothermicity…
In this paper, we investigate the photothermal effects of the plasmon resonance. Metal nanoparticles efficiently generate heat in the presence of electromagnetic radiation. The process is strongly enhanced when a fixed frequency of the…
Metal photoluminescence (MPL) originates from radiative recombination of photoexcited core holes and conduction band electrons. In metal nanostructures, MPL is enhanced due to the surface plasmon local field effect. We identify another…
The fluorescence of organic fluorophore molecules is enhanced when they are placed in contact with certain metals (Al, Ag, Cu, Au, etc.) whose surface plasmon waves couple into the radiative modes of the molecules and increase the radiative…
Plasmonics, the science and technology of the interaction of light with metallic objects, is fundamentally changing the way we can detect, generate and manipulate light. Although the field is progressing swiftly, thanks to the availability…
Plasmonic materials have got wide attention as a potential candidate for light driven catalysis of chemical conversions by harnessing solar energy to reduce the environmental issues generated by fossil fuels-based bulk chemical industries.…
Plasmonic absorption of light can lead to significant local heating in metallic nanostructures, an effect that defines the sub-field of thermoplasmonics and has been leveraged in diverse applications from biomedical technology to…
Recently, we have shown that thermal effects play a crucial role in speeding up the rate of bond-dissociation reactions. This was done by applying a simple temperature-shifted Arrhenius Law to the experimental data, corroborated with…
We combine ab-initio calculations based on many-body perturbation theory and the cumulant expansion with angle-resolved photoemission spectroscopy (ARPES) to quantify the electron-plasmon interaction in the highly-doped semiconducting…
We describe the process of Foerster transfer between semiconductor nanoparticles in the presence of a metal subsystem (metal nanocrystals). In the presence of metal nanocrystals, the Foerster process can become faster and more long-range.…
Nonlinear electron emission processes induced by surface plasmon oscillations have been studied both experimentally and theoretically. The measured above-threshold electron spectra extend up to energies whose appearance cannot be explained…
Gas phase thermal isomerization rates of trans-stilbene at 300 K obey the Arrhenius law. In solution the rates increase ten-fold and depend only very weakly on excitation wavelength or intramolecular temperature. Both observations are…