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Generation of circularly-polarized high-harmonics with the same helicity to all orders is indispensable for chiral-sensitive spectroscopy with attosecond temporal resolution. Solid-state samples have added a valuable asset in controlling…

光学 · 物理学 2023-06-06 Navdeep Rana , M. S. Mrudul , Gopal Dixit

The design and fabrication of phononic crystals (PnCs) hold the key to control the propagation of heat and sound at the nanoscale. However, there is a lack of experimental studies addressing the impact of order/disorder on the phononic…

A recent paper reported elliptically polarized high-order harmonics from aligned N$_2$ using a linearly polarized driving field [X. Zhou \emph{et al.}, Phys. Rev. Lett. \textbf{102}, 073902 (2009)]. This observation cannot be explained in…

原子物理 · 物理学 2010-03-29 Adam Etches , Christian Bruun Madsen , Lars Bojer Madsen

We studied the high-order harmonic generation (HHG) from 2D solid materials in circularly and bichromatic circularly polarized laser fields numerically by simulating the dynamics of single-active-electron processes in 2D periodic…

光学 · 物理学 2018-10-23 Guang-Rui Jia , Xin-Qiang Wang , Tao-Yuan Du , Xiao-Huan Huang , Xue-Bin Bian

High-order harmonics generated by bicircular laser field have helicities which alternate between $+1$ and $-1$. In order to generate circularly polarized high-harmonic pulses, which are important for applications, it is necessary to achieve…

原子物理 · 物理学 2018-09-26 Dejan B. Milošević

Symmetries are so involved in crystallographic detail that it is indispensable when crystal cell or lattice is mentioned. For nanocrystals, however, many are 'systemic symmetries', meaning that the whole structures of nanocrystal particles…

介观与纳米尺度物理 · 物理学 2011-12-13 Yan Zhou , Junyan Zhang , Bin Zhang , Jutao Jin , Aimin Liang , Yuqing Da , Jiangong Li

We investigate the polarization properties of high harmonic generation from polar molecules with a linearly polarized field. It is found that elliptically polarized harmonics are observed in a wide spectral range from the plateau to the…

光学 · 物理学 2011-12-06 Meiyan Qin , Xiaosong Zhu , Qingbin Zhang , Weiyi Hong , Peixiang Lu

We investigate the influence of intense, elliptically polarized driving fields on high-order harmonic spectra from aligned diatomic molecules. We derive a generalized two-center interference condition for elliptically polarized fields,…

原子物理 · 物理学 2015-06-16 T. Das , B. B. Augstein , C. Figueira de Morisson Faria

The polarization matrix ($2\times2$) obtained from two component eigen-spinors of spherical harmonics help us to evaluate the differential matrix $N$ of the anisotropic optical medium. The geometric phase is realized through {\it helicity}…

光学 · 物理学 2007-05-23 Dipti Banerjee

Disorder in crystals is rarely random, and instead involves local correlations whose presence and nature are hidden from conventional crystallographic probes. This hidden order can sometimes be controlled, but its importance for physical…

材料科学 · 物理学 2023-10-05 Nikolaj Roth , Andrew L. Goodwin

Polarization-resolved second-harmonic spectra are obtained from the resonant modes of a two-dimensional planar photonic crystal microcavity patterned in a free-standing InP slab. The photonic crystal microcavity is comprised of a single…

High harmonic generation (HHG) in crystals has revealed a wealth of perspectives such as all-optical mapping of the electronic band structure, ultrafast quantum information and the creation of novel all-solid-state attosecond sources.…

We study the ellipticity of high-order harmonics emitted from CO$_2$ molecule driven by linearly polarized laser fields using numerical simulations within the time-dependent density functional theory. We find that the overall ellipticity of…

原子与分子团簇 · 物理学 2024-09-17 Andres Mora , Lauren Bauerle , Yuqing Xia , Agnieszka Jaron

Polarized and azimuthal dependencies of optical second harmonics generation (SHG) at the surface of noncentrosymmetric semiconductor crystals have been measured on polished surfaces of ZnSe(100), using a fundamental wavelength of 1.06$\mu…

光学 · 物理学 2007-05-23 Xiangyang Song , Arnold Neumann , Rein Maripuu , Kai Siegbahn

The generation of high-order harmonics in finite, hexagonal nanoribbons is simulated. Ribbons with armchair and zig-zag edges are investigated by using a tight-binding approach with only nearest neighbor hopping. By turning an alternating…

介观与纳米尺度物理 · 物理学 2024-03-12 Hannah Jürß , Dieter Bauer

We demonstrated nonperturbative high harmonics induced by intense mid-infrared light up to 18th order that well exceed the material bandgap in monolayer transition metal dichalcogenides. The intensities of the even-order high-harmonic…

介观与纳米尺度物理 · 物理学 2019-08-20 Naotaka Yoshikawa , Kohei Nagai , Kento Uchida , Yuhei Takaguchi , Shogo Sasaki , Yasumitsu Miyata , Koichiro Tanaka

We observe the generation of high harmonics in the plane perpendicular to the driving laser polarization and show that these are driven by the spin-orbit interaction. Using R-Matrix with time-dependence theory, we demonstrate that for…

High order harmonic generation from clusters is a controversial topic: conflicting theories exist, with different explanations for similar experimental observations. From an experimental point of view, separating the contributions from…

原子与分子团簇 · 物理学 2015-06-12 H. Ruf , C. Handschin , R. Cireasa , N. Thiré , A. Ferré , S. Petit , D. Descamps , E. Mével , E. Constant , V. Blanchet , B. Fabre , Y. Mairesse

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

原子物理 · 物理学 2018-05-18 Peter Mulholland , Daniel Dundas

Second harmonic generation in a two dimensional nonlinear quasi-crystal is demonstrated for the first time. Temperature and wavelength tuning of the crystal reveal the uniformity of the pattern while angle tuning reveals the dense nature of…

光学 · 物理学 2007-05-23 Neil Broderick , Anna Peacock , Katia Gallo , Ruth Lewen , Radu Bratfalean